Time-resolved Auger–Meitner spectroscopy of the photodissociation dynamics of CS2

The photodissociation dynamics of UV excited CS2 are investigated using time-resolved Auger-Meitner (AM) spectroscopy. AM decay is initiated by inner-shell ionisation with a femtosecond duration x-ray (179.9 eV) probe generated by the FERMI free electron laser. The time-delayed x-ray probe removes a...

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Published in:Journal of physics. B, Atomic, molecular, and optical physics Atomic, molecular, and optical physics, 2024-11, Vol.57 (21)
Main Authors: Thompson, Henry J, Plekan, Oksana, Bonanomi, Matteo, Pal, Nitish, Allum, Felix, Brynes, Alexander D, Coreno, Marcello, Coriani, Sonia, Danailov, Miltcho B, Decleva, Piero, Demidovich, Alexander, Devetta, Michele, Faccialà, Davide, Feifel, Raimund, Forbes, Ruaridh, Grazioli, Cesare, Holland, David M P, Piseri, Paolo, Prince, Kevin C, Rolles, Daniel, Schuurman, Michael S, Simoncig, Alberto, Squibb, Richard J, Tenorio, Bruno N C, Vozzi, Caterina, Zangrando, Marco, Callegari, Carlo, Minns, Russell S, Di Fraia, Michele
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Language:English
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Atom and Molecular Physics and Optics
Atom- och molekylfysik och optik
Auger spectroscopy
free electron lasers
time-resolved x-ray spectroscopy
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container_title Journal of physics. B, Atomic, molecular, and optical physics
container_volume 57
creator Thompson, Henry J
Plekan, Oksana
Bonanomi, Matteo
Pal, Nitish
Allum, Felix
Brynes, Alexander D
Coreno, Marcello
Coriani, Sonia
Danailov, Miltcho B
Decleva, Piero
Demidovich, Alexander
Devetta, Michele
Faccialà, Davide
Feifel, Raimund
Forbes, Ruaridh
Grazioli, Cesare
Holland, David M P
Piseri, Paolo
Prince, Kevin C
Rolles, Daniel
Schuurman, Michael S
Simoncig, Alberto
Squibb, Richard J
Tenorio, Bruno N C
Vozzi, Caterina
Zangrando, Marco
Callegari, Carlo
Minns, Russell S
Di Fraia, Michele
description The photodissociation dynamics of UV excited CS2 are investigated using time-resolved Auger-Meitner (AM) spectroscopy. AM decay is initiated by inner-shell ionisation with a femtosecond duration x-ray (179.9 eV) probe generated by the FERMI free electron laser. The time-delayed x-ray probe removes an electron from the S(2p) orbital leading to secondary emission of a high energy electron through AM decay. We monitor the electron kinetic energy of the AM emission as a function of pump-probe delay and observe time-dependent changes in the spectrum that correlate with the formation of bound, excited-state CS2 molecules at early times, and CS + S fragments on the picosecond timescale. The results are analysed based on a simplified kinetic scheme that provides a time constant for dissociation of approximately 1.2 ps, in agreement with previous time-resolved x-ray photoelectron spectroscopy measurements.
doi_str_mv 10.1088/1361-6455/ad7e89
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subjects Atom and Molecular Physics and Optics
Atom- och molekylfysik och optik
Auger spectroscopy
free electron lasers
time-resolved x-ray spectroscopy
title Time-resolved Auger–Meitner spectroscopy of the photodissociation dynamics of CS2
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