Advances in Stabilizing 'Layered-Layered' xLi2MnO3·(1-x)LiMO2 (M=Mn, Ni, Co) Electrodes with a Spinel Component

Composite electrode structures with layered and spinel components have been investigated to evaluate the possibility of arresting or suppressing the voltage fade observed on cycling high capacity, lithium- and manganese-rich 'layered-layered' xLi2MnO3*(1-x)LiMO2 (M=Mn, Ni, Co) electrodes i...

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Published in:Journal of the Electrochemical Society 2014-01, Vol.161 (14), p.A2160-A2167
Main Authors: Long, Brandon R., Croy, Jason R., Park, Joong Sun, Wen, Jianguo, Miller, Dean J., Thackeray, Michael M.
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container_issue 14
container_start_page A2160
container_title Journal of the Electrochemical Society
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creator Long, Brandon R.
Croy, Jason R.
Park, Joong Sun
Wen, Jianguo
Miller, Dean J.
Thackeray, Michael M.
description Composite electrode structures with layered and spinel components have been investigated to evaluate the possibility of arresting or suppressing the voltage fade observed on cycling high capacity, lithium- and manganese-rich 'layered-layered' xLi2MnO3*(1-x)LiMO2 (M=Mn, Ni, Co) electrodes in lithium cells. Control of the spinel content in 'layered-layered-spinel' electrode materials and regulating the electrochemical voltage window of the lithium cells enables a capacity of approximately 190 mAh/g with little voltage fade. The results bode well for enhancing the electrochemical properties and structural stability of composite electrode structures on long-term cycling in lithium-ion batteries.
doi_str_mv 10.1149/2.0681414jes
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title Advances in Stabilizing 'Layered-Layered' xLi2MnO3·(1-x)LiMO2 (M=Mn, Ni, Co) Electrodes with a Spinel Component
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