28.3% efficient perovskite-silicon tandem solar cells with mixed self-assembled monolayers

A certified 28.3% efficient monolithic perovskite-silicon tandem (PST) solar cell with a mixed self-assembled monolayer (SAM) containing carbazole cores with H-ligands (2PACz) and methoxy-ligands (MeO-2PACz) is reported. Our analysis revealed that there existed uncovered areas of MeO-2PACz on indium...

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Published in:Applied physics express 2022-07, Vol.15 (7), p.76503
Main Authors: Mishima, Ryota, Hino, Masashi, Kanematsu, Masanori, Kishimoto, Kazuhisa, Ishibashi, Hirotaka, Konishi, Katsunori, Okamoto, Shimpei, Irie, Toru, Fujimoto, Takahisa, Yoshida, Wataru, Uzu, Hisashi, Adachi, Daisuke, Yamamoto, Kenji
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monolithic perovskite-silicon tandem solar cell
perovskite solar cell
self-assembled monolayer
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cited_by cdi_FETCH-LOGICAL-c316t-7ac9cc4a755cef189f330e74719c9ba2cf3fa2903ce7dcb7db64f577c17a2e5b3
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container_end_page
container_issue 7
container_start_page 76503
container_title Applied physics express
container_volume 15
creator Mishima, Ryota
Hino, Masashi
Kanematsu, Masanori
Kishimoto, Kazuhisa
Ishibashi, Hirotaka
Konishi, Katsunori
Okamoto, Shimpei
Irie, Toru
Fujimoto, Takahisa
Yoshida, Wataru
Uzu, Hisashi
Adachi, Daisuke
Yamamoto, Kenji
description A certified 28.3% efficient monolithic perovskite-silicon tandem (PST) solar cell with a mixed self-assembled monolayer (SAM) containing carbazole cores with H-ligands (2PACz) and methoxy-ligands (MeO-2PACz) is reported. Our analysis revealed that there existed uncovered areas of MeO-2PACz on indium tin oxide, which would be caused by the steric effect, and they were filled with 2PACz in the mixed SAM, leading to the improvement of fill factors in the PST cells. This result was explained by the passivation qualities as hole transport layers and the local interaction between methoxy ligands and perovskite materials.
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subjects monolithic perovskite-silicon tandem solar cell
perovskite solar cell
self-assembled monolayer
title 28.3% efficient perovskite-silicon tandem solar cells with mixed self-assembled monolayers
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