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Development of a detection method for {244}Pu by resonance ionization mass spectrometry
The long-lived actinide {sup 244}Pu (t{sub 1/2} = 81 Myr) is expected to be present in the Interstellar Medium from fresh r-process nucleosynthesis or in direct ejecta from supernovae. Deposition onto Earth may result in traces of live {sup 244}Pu in suitable reservoirs. We are developing a method f...
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Published in: | New astronomy reviews 2006-10, Vol.50 (7-8) |
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creator | Ofan, A. Ahmad, I. Greene, J. P. Paul, M. Savina, M. R. |
description | The long-lived actinide {sup 244}Pu (t{sub 1/2} = 81 Myr) is expected to be present in the Interstellar Medium from fresh r-process nucleosynthesis or in direct ejecta from supernovae. Deposition onto Earth may result in traces of live {sup 244}Pu in suitable reservoirs. We are developing a method for {sup 244}Pu detection based on resonance ionization mass spectroscopy. Using Gd as a proxy, we determine an overall efficiency of 0.5% in conditions applicable to the detection of Pu, and present preliminary results on Pu detection. |
doi_str_mv | 10.1016/j.newar.2006.06.066 |
format | article |
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P. ; Paul, M. ; Savina, M. R.</creator><creatorcontrib>Ofan, A. ; Ahmad, I. ; Greene, J. P. ; Paul, M. ; Savina, M. R. ; Argonne National Lab. (ANL), Argonne, IL (United States)</creatorcontrib><description>The long-lived actinide {sup 244}Pu (t{sub 1/2} = 81 Myr) is expected to be present in the Interstellar Medium from fresh r-process nucleosynthesis or in direct ejecta from supernovae. Deposition onto Earth may result in traces of live {sup 244}Pu in suitable reservoirs. We are developing a method for {sup 244}Pu detection based on resonance ionization mass spectroscopy. Using Gd as a proxy, we determine an overall efficiency of 0.5% in conditions applicable to the detection of Pu, and present preliminary results on Pu detection.</description><identifier>ISSN: 1387-6473</identifier><identifier>EISSN: 1872-9630</identifier><identifier>DOI: 10.1016/j.newar.2006.06.066</identifier><language>eng</language><publisher>United States</publisher><subject>ACTINIDES ; CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS ; DEPOSITION ; DETECTION ; EFFICIENCY ; IONIZATION ; MASS SPECTROSCOPY ; NUCLEOSYNTHESIS ; R PROCESS ; RESONANCE ; RESONANCE IONIZATION MASS SPECTROSCOPY ; SPECTROSCOPY ; SUPERNOVAE</subject><ispartof>New astronomy reviews, 2006-10, Vol.50 (7-8)</ispartof><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>230,314,780,784,885,27924,27925</link.rule.ids><backlink>$$Uhttps://www.osti.gov/biblio/1026633$$D View this record in Osti.gov$$Hfree_for_read</backlink></links><search><creatorcontrib>Ofan, A.</creatorcontrib><creatorcontrib>Ahmad, I.</creatorcontrib><creatorcontrib>Greene, J. 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R.</creatorcontrib><creatorcontrib>Argonne National Lab. (ANL), Argonne, IL (United States)</creatorcontrib><collection>OSTI.GOV</collection><jtitle>New astronomy reviews</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Ofan, A.</au><au>Ahmad, I.</au><au>Greene, J. P.</au><au>Paul, M.</au><au>Savina, M. R.</au><aucorp>Argonne National Lab. (ANL), Argonne, IL (United States)</aucorp><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Development of a detection method for {244}Pu by resonance ionization mass spectrometry</atitle><jtitle>New astronomy reviews</jtitle><date>2006-10</date><risdate>2006</risdate><volume>50</volume><issue>7-8</issue><issn>1387-6473</issn><eissn>1872-9630</eissn><abstract>The long-lived actinide {sup 244}Pu (t{sub 1/2} = 81 Myr) is expected to be present in the Interstellar Medium from fresh r-process nucleosynthesis or in direct ejecta from supernovae. Deposition onto Earth may result in traces of live {sup 244}Pu in suitable reservoirs. We are developing a method for {sup 244}Pu detection based on resonance ionization mass spectroscopy. Using Gd as a proxy, we determine an overall efficiency of 0.5% in conditions applicable to the detection of Pu, and present preliminary results on Pu detection.</abstract><cop>United States</cop><doi>10.1016/j.newar.2006.06.066</doi></addata></record> |
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subjects | ACTINIDES CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS DEPOSITION DETECTION EFFICIENCY IONIZATION MASS SPECTROSCOPY NUCLEOSYNTHESIS R PROCESS RESONANCE RESONANCE IONIZATION MASS SPECTROSCOPY SPECTROSCOPY SUPERNOVAE |
title | Development of a detection method for {244}Pu by resonance ionization mass spectrometry |
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