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Electronic structure of warm dense copper studied by ultrafast x-ray absorption spectroscopy

We use time-resolved x-ray absorption spectroscopy to investigate the unoccupied electronic density of states of warm dense copper that is produced isochorically through the absorption of an ultrafast optical pulse. The temperature of the superheated electron-hole plasma, which ranges from 4000 to 1...

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Published in:Physical review letters 2011-04, Vol.106 (16), p.167601-167601, Article 167601
Main Authors: Cho, B I, Engelhorn, K, Correa, A A, Ogitsu, T, Weber, C P, Lee, H J, Feng, J, Ni, P A, Ping, Y, Nelson, A J, Prendergast, D, Lee, R W, Falcone, R W, Heimann, P A
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cited_by cdi_FETCH-LOGICAL-c504t-af5b798e131e4bc1a9e578e814598f395c0ead452f0c509644a86fe0471b9dd33
cites cdi_FETCH-LOGICAL-c504t-af5b798e131e4bc1a9e578e814598f395c0ead452f0c509644a86fe0471b9dd33
container_end_page 167601
container_issue 16
container_start_page 167601
container_title Physical review letters
container_volume 106
creator Cho, B I
Engelhorn, K
Correa, A A
Ogitsu, T
Weber, C P
Lee, H J
Feng, J
Ni, P A
Ping, Y
Nelson, A J
Prendergast, D
Lee, R W
Falcone, R W
Heimann, P A
description We use time-resolved x-ray absorption spectroscopy to investigate the unoccupied electronic density of states of warm dense copper that is produced isochorically through the absorption of an ultrafast optical pulse. The temperature of the superheated electron-hole plasma, which ranges from 4000 to 10 000 K, was determined by comparing the measured x-ray absorption spectrum with a simulation. The electronic structure of warm dense copper is adequately described with the high temperature electronic density of state calculated by the density functional theory. The dynamics of the electron temperature is consistent with a two-temperature model, while a temperature-dependent electron-phonon coupling parameter is necessary.
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title Electronic structure of warm dense copper studied by ultrafast x-ray absorption spectroscopy
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