Electronic four-particle correlations in semiconductors: Renormalization of coherent pump-probe oscillations

The nonlinear optical response of excitons in a single ZnSe quantum well is investigated by pump-probe measurements. In the counter-circular polarization configuration at negative delay, {delta}t, spectral oscillations are observed the period E{sub PP} of which is energy dependent. Whereas at energi...

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Published in:Physical review. B, Condensed matter and materials physics Condensed matter and materials physics, 2000-03, Vol.61 (12)
Main Authors: Neukirch, U., Bolton, S. R., Sham, L. J., Chemla, D. S.
Format: Article
Language:English
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CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY
ELECTRONIC STRUCTURE
EXCITONS
EXPERIMENTAL DATA
FREQUENCY MIXING
MATERIALS SCIENCE
NONLINEAR OPTICS
OPTICAL PROPERTIES
SEMICONDUCTOR MATERIALS
THIN FILMS
ZINC SELENIDES
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creator Neukirch, U.
Bolton, S. R.
Sham, L. J.
Chemla, D. S.
description The nonlinear optical response of excitons in a single ZnSe quantum well is investigated by pump-probe measurements. In the counter-circular polarization configuration at negative delay, {delta}t, spectral oscillations are observed the period E{sub PP} of which is energy dependent. Whereas at energies above the 1S exciton the usual E{sub PP}=h/|{delta}t| dependence is found, the period strongly deviates from that value at energies below the exciton. Model calculations reveal that this behavior is caused by the bound biexciton state in the four-particle correlations. (c) 2000 The American Physical Society.
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subjects CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY
ELECTRONIC STRUCTURE
EXCITONS
EXPERIMENTAL DATA
FREQUENCY MIXING
MATERIALS SCIENCE
NONLINEAR OPTICS
OPTICAL PROPERTIES
SEMICONDUCTOR MATERIALS
THIN FILMS
ZINC SELENIDES
title Electronic four-particle correlations in semiconductors: Renormalization of coherent pump-probe oscillations
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