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Time-reversal symmetry breaking superconductivity between twisted cuprate superconductors
Twisted interfaces between stacked van der Waals (vdW) cuprate crystals present a platform for engineering superconducting order parameters by adjusting stacking angles. Employing a cryogenic assembly technique, we construct twisted vdW Josephson junctions (JJ) at atomically sharp interfaces between...
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Published in: | Science (American Association for the Advancement of Science) 2023-12, Vol.382 (6677), p.eabl8371-1427 |
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creator | Zhao, S Y Frank Cui, Xiaomeng Volkov, Pavel A Yoo, Hyobin Lee, Sangmin Gardener, Jules A Akey, Austin J Engelke, Rebecca Ronen, Yuval Zhong, Ruidan Gu, Genda Plugge, Stephan Tummuru, Tarun Kim, Miyoung Franz, Marcel Pixley, Jedediah H Poccia, Nicola Kim, Philip |
description | Twisted interfaces between stacked van der Waals (vdW) cuprate crystals present a platform for engineering superconducting order parameters by adjusting stacking angles. Employing a cryogenic assembly technique, we construct twisted vdW Josephson junctions (JJ) at atomically sharp interfaces between Bi
Sr
CaCu
O
crystals with quality approaching the limit set by intrinsic JJ. Near 45° twist angle, we observe fractional Shapiro steps and Fraunhofer patterns, consistent with the existence of two degenerate Josephson ground states related by time-reversal symmetry (TRS). By programming the JJ current bias sequence, we controllably break TRS to place the JJ into either of the two ground states, realizing reversible Josephson diodes without external magnetic fields. Our results open a path to engineering topological devices at higher temperatures. |
doi_str_mv | 10.1126/science.abl8371 |
format | article |
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Sr
CaCu
O
crystals with quality approaching the limit set by intrinsic JJ. Near 45° twist angle, we observe fractional Shapiro steps and Fraunhofer patterns, consistent with the existence of two degenerate Josephson ground states related by time-reversal symmetry (TRS). By programming the JJ current bias sequence, we controllably break TRS to place the JJ into either of the two ground states, realizing reversible Josephson diodes without external magnetic fields. Our results open a path to engineering topological devices at higher temperatures.</description><identifier>ISSN: 0036-8075</identifier><identifier>EISSN: 1095-9203</identifier><identifier>DOI: 10.1126/science.abl8371</identifier><identifier>PMID: 38060675</identifier><language>eng</language><publisher>United States: The American Association for the Advancement of Science</publisher><subject>Bismuth ; Broken symmetry ; CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY ; Coupling ; Graphene ; Order parameters ; Superconductivity ; Superconductors ; Superlattices ; Transition metal compounds ; Two dimensional materials</subject><ispartof>Science (American Association for the Advancement of Science), 2023-12, Vol.382 (6677), p.eabl8371-1427</ispartof><rights>Copyright © 2023 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c352t-43cfe9c560ab6b1a08ea2aa51366a82cf8e9bc637759f41f152ac34efe03e02d3</citedby><cites>FETCH-LOGICAL-c352t-43cfe9c560ab6b1a08ea2aa51366a82cf8e9bc637759f41f152ac34efe03e02d3</cites><orcidid>0000-0002-4844-2030 ; 0000-0001-7982-0113 ; 0000-0002-3109-640X ; 0000-0002-1249-6053 ; 0000-0001-7586-9788 ; 0000-0002-2824-2154 ; 0000-0002-1515-8076 ; 0009-0001-7196-2763 ; 0000-0002-2427-2591 ; 0000-0001-5151-1706 ; 0000-0002-9886-3255 ; 0000-0003-0608-0016 ; 0000-0001-6848-3190 ; 0000-0003-4922-6812 ; 0000-0001-8632-6711 ; 0000-0002-8039-9482 ; 0000-0002-8255-0086 ; 0000000179820113 ; 0000000224272591 ; 0000000215158076 ; 0000000186326711 ; 0000000349226812 ; 0000000151511706 ; 0009000171962763 ; 0000000280399482 ; 0000000212496053 ; 0000000282550086 ; 0000000175869788 ; 0000000298863255 ; 0000000168483190 ; 0000000306080016 ; 0000000248442030 ; 000000023109640X ; 0000000228242154</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>230,314,780,784,885,2884,2885,27924,27925</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/38060675$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink><backlink>$$Uhttps://www.osti.gov/servlets/purl/2203268$$D View this record in Osti.gov$$Hfree_for_read</backlink></links><search><creatorcontrib>Zhao, S Y Frank</creatorcontrib><creatorcontrib>Cui, Xiaomeng</creatorcontrib><creatorcontrib>Volkov, Pavel A</creatorcontrib><creatorcontrib>Yoo, Hyobin</creatorcontrib><creatorcontrib>Lee, Sangmin</creatorcontrib><creatorcontrib>Gardener, Jules A</creatorcontrib><creatorcontrib>Akey, Austin J</creatorcontrib><creatorcontrib>Engelke, Rebecca</creatorcontrib><creatorcontrib>Ronen, Yuval</creatorcontrib><creatorcontrib>Zhong, Ruidan</creatorcontrib><creatorcontrib>Gu, Genda</creatorcontrib><creatorcontrib>Plugge, Stephan</creatorcontrib><creatorcontrib>Tummuru, Tarun</creatorcontrib><creatorcontrib>Kim, Miyoung</creatorcontrib><creatorcontrib>Franz, Marcel</creatorcontrib><creatorcontrib>Pixley, Jedediah H</creatorcontrib><creatorcontrib>Poccia, Nicola</creatorcontrib><creatorcontrib>Kim, Philip</creatorcontrib><creatorcontrib>Brookhaven National Laboratory (BNL), Upton, NY (United States)</creatorcontrib><title>Time-reversal symmetry breaking superconductivity between twisted cuprate superconductors</title><title>Science (American Association for the Advancement of Science)</title><addtitle>Science</addtitle><description>Twisted interfaces between stacked van der Waals (vdW) cuprate crystals present a platform for engineering superconducting order parameters by adjusting stacking angles. Employing a cryogenic assembly technique, we construct twisted vdW Josephson junctions (JJ) at atomically sharp interfaces between Bi
Sr
CaCu
O
crystals with quality approaching the limit set by intrinsic JJ. Near 45° twist angle, we observe fractional Shapiro steps and Fraunhofer patterns, consistent with the existence of two degenerate Josephson ground states related by time-reversal symmetry (TRS). By programming the JJ current bias sequence, we controllably break TRS to place the JJ into either of the two ground states, realizing reversible Josephson diodes without external magnetic fields. Our results open a path to engineering topological devices at higher temperatures.</description><subject>Bismuth</subject><subject>Broken symmetry</subject><subject>CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY</subject><subject>Coupling</subject><subject>Graphene</subject><subject>Order parameters</subject><subject>Superconductivity</subject><subject>Superconductors</subject><subject>Superlattices</subject><subject>Transition metal compounds</subject><subject>Two dimensional 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Miyoung</au><au>Franz, Marcel</au><au>Pixley, Jedediah H</au><au>Poccia, Nicola</au><au>Kim, Philip</au><aucorp>Brookhaven National Laboratory (BNL), Upton, NY (United States)</aucorp><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Time-reversal symmetry breaking superconductivity between twisted cuprate superconductors</atitle><jtitle>Science (American Association for the Advancement of Science)</jtitle><addtitle>Science</addtitle><date>2023-12-22</date><risdate>2023</risdate><volume>382</volume><issue>6677</issue><spage>eabl8371</spage><epage>1427</epage><pages>eabl8371-1427</pages><issn>0036-8075</issn><eissn>1095-9203</eissn><abstract>Twisted interfaces between stacked van der Waals (vdW) cuprate crystals present a platform for engineering superconducting order parameters by adjusting stacking angles. Employing a cryogenic assembly technique, we construct twisted vdW Josephson junctions (JJ) at atomically sharp interfaces between Bi
Sr
CaCu
O
crystals with quality approaching the limit set by intrinsic JJ. Near 45° twist angle, we observe fractional Shapiro steps and Fraunhofer patterns, consistent with the existence of two degenerate Josephson ground states related by time-reversal symmetry (TRS). By programming the JJ current bias sequence, we controllably break TRS to place the JJ into either of the two ground states, realizing reversible Josephson diodes without external magnetic fields. Our results open a path to engineering topological devices at higher temperatures.</abstract><cop>United States</cop><pub>The American Association for the Advancement of Science</pub><pmid>38060675</pmid><doi>10.1126/science.abl8371</doi><tpages>6</tpages><orcidid>https://orcid.org/0000-0002-4844-2030</orcidid><orcidid>https://orcid.org/0000-0001-7982-0113</orcidid><orcidid>https://orcid.org/0000-0002-3109-640X</orcidid><orcidid>https://orcid.org/0000-0002-1249-6053</orcidid><orcidid>https://orcid.org/0000-0001-7586-9788</orcidid><orcidid>https://orcid.org/0000-0002-2824-2154</orcidid><orcidid>https://orcid.org/0000-0002-1515-8076</orcidid><orcidid>https://orcid.org/0009-0001-7196-2763</orcidid><orcidid>https://orcid.org/0000-0002-2427-2591</orcidid><orcidid>https://orcid.org/0000-0001-5151-1706</orcidid><orcidid>https://orcid.org/0000-0002-9886-3255</orcidid><orcidid>https://orcid.org/0000-0003-0608-0016</orcidid><orcidid>https://orcid.org/0000-0001-6848-3190</orcidid><orcidid>https://orcid.org/0000-0003-4922-6812</orcidid><orcidid>https://orcid.org/0000-0001-8632-6711</orcidid><orcidid>https://orcid.org/0000-0002-8039-9482</orcidid><orcidid>https://orcid.org/0000-0002-8255-0086</orcidid><orcidid>https://orcid.org/0000000179820113</orcidid><orcidid>https://orcid.org/0000000224272591</orcidid><orcidid>https://orcid.org/0000000215158076</orcidid><orcidid>https://orcid.org/0000000186326711</orcidid><orcidid>https://orcid.org/0000000349226812</orcidid><orcidid>https://orcid.org/0000000151511706</orcidid><orcidid>https://orcid.org/0009000171962763</orcidid><orcidid>https://orcid.org/0000000280399482</orcidid><orcidid>https://orcid.org/0000000212496053</orcidid><orcidid>https://orcid.org/0000000282550086</orcidid><orcidid>https://orcid.org/0000000175869788</orcidid><orcidid>https://orcid.org/0000000298863255</orcidid><orcidid>https://orcid.org/0000000168483190</orcidid><orcidid>https://orcid.org/0000000306080016</orcidid><orcidid>https://orcid.org/0000000248442030</orcidid><orcidid>https://orcid.org/000000023109640X</orcidid><orcidid>https://orcid.org/0000000228242154</orcidid><oa>free_for_read</oa></addata></record> |
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identifier | ISSN: 0036-8075 |
ispartof | Science (American Association for the Advancement of Science), 2023-12, Vol.382 (6677), p.eabl8371-1427 |
issn | 0036-8075 1095-9203 |
language | eng |
recordid | cdi_osti_scitechconnect_2203268 |
source | American Association for the Advancement of Science; Alma/SFX Local Collection |
subjects | Bismuth Broken symmetry CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY Coupling Graphene Order parameters Superconductivity Superconductors Superlattices Transition metal compounds Two dimensional materials |
title | Time-reversal symmetry breaking superconductivity between twisted cuprate superconductors |
url | http://sfxeu10.hosted.exlibrisgroup.com/loughborough?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2024-12-20T18%3A05%3A07IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_osti_&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Time-reversal%20symmetry%20breaking%20superconductivity%20between%20twisted%20cuprate%20superconductors&rft.jtitle=Science%20(American%20Association%20for%20the%20Advancement%20of%20Science)&rft.au=Zhao,%20S%20Y%20Frank&rft.aucorp=Brookhaven%20National%20Laboratory%20(BNL),%20Upton,%20NY%20(United%20States)&rft.date=2023-12-22&rft.volume=382&rft.issue=6677&rft.spage=eabl8371&rft.epage=1427&rft.pages=eabl8371-1427&rft.issn=0036-8075&rft.eissn=1095-9203&rft_id=info:doi/10.1126/science.abl8371&rft_dat=%3Cproquest_osti_%3E2902971323%3C/proquest_osti_%3E%3Cgrp_id%3Ecdi_FETCH-LOGICAL-c352t-43cfe9c560ab6b1a08ea2aa51366a82cf8e9bc637759f41f152ac34efe03e02d3%3C/grp_id%3E%3Coa%3E%3C/oa%3E%3Curl%3E%3C/url%3E&rft_id=info:oai/&rft_pqid=2904231820&rft_id=info:pmid/38060675&rfr_iscdi=true |