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Investigation of the neutron activation of endohedral rare earth metallofullerenes
Endohedral lanthanide metallofullerenes and their water-soluble biocompatible derivatives have been synthesized. The effect that fast-neutron irradiation has on the stability and nuclear physical properties of endohedral metallofullerenes that are used as magnetocontrast materials ( 46 Sc, 140 La, 1...
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Published in: | Crystallography reports 2011-12, Vol.56 (7), p.1192-1196 |
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container_end_page | 1196 |
container_issue | 7 |
container_start_page | 1192 |
container_title | Crystallography reports |
container_volume | 56 |
creator | Shilin, V. A. Lebedev, V. T. Kolesnik, S. G. Kozlov, V. S. Grushko, Yu. S. Sedov, V. P. Kukorenko, V. V. |
description | Endohedral lanthanide metallofullerenes and their water-soluble biocompatible derivatives have been synthesized. The effect that fast-neutron irradiation has on the stability and nuclear physical properties of endohedral metallofullerenes that are used as magnetocontrast materials (
46
Sc,
140
La,
141
Nd,
153
Sm,
152
Eu,
154
Eu,
153
Sm,
160
Tb,
169
Yb,
170
Tm (isomers I and III), and
177
Lu) is studied. Our hypothesis, according to which carbon-shell relaxation is based on the fast nonradiative processes of an electron shake-off type, is confirmed. |
doi_str_mv | 10.1134/S1063774511070339 |
format | article |
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46
Sc,
140
La,
141
Nd,
153
Sm,
152
Eu,
154
Eu,
153
Sm,
160
Tb,
169
Yb,
170
Tm (isomers I and III), and
177
Lu) is studied. Our hypothesis, according to which carbon-shell relaxation is based on the fast nonradiative processes of an electron shake-off type, is confirmed.</description><identifier>ISSN: 1063-7745</identifier><identifier>EISSN: 1562-689X</identifier><identifier>DOI: 10.1134/S1063774511070339</identifier><language>eng</language><publisher>Dordrecht: SP MAIK Nauka/Interperiodica</publisher><subject>CARBON ; Crystallography and Scattering Methods ; EUROPIUM 152 ; EUROPIUM 154 ; FAST NEUTRONS ; INORGANIC, ORGANIC, PHYSICAL AND ANALYTICAL CHEMISTRY ; IRRADIATION ; ISOMERS ; LANTHANUM 140 ; LUTETIUM 177 ; Nanomaterials and Ceramics ; NEODYMIUM 141 ; NEUTRON ACTIVATION ANALYSIS ; PHYSICAL PROPERTIES ; Physics ; Physics and Astronomy ; RADIATION CHEMISTRY, RADIOCHEMISTRY AND NUCLEAR CHEMISTRY ; RARE EARTH COMPLEXES ; RELAXATION ; SAMARIUM 153 ; SCANDIUM 46 ; STABILITY ; TERBIUM 160 ; THULIUM 170 ; YTTERBIUM 169</subject><ispartof>Crystallography reports, 2011-12, Vol.56 (7), p.1192-1196</ispartof><rights>Pleiades Publishing, Ltd. 2011</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c316t-392cb566c8d92b856c33bf0634a15e0ae0211d252ccfa895bc8b2c63d440c3b53</citedby><cites>FETCH-LOGICAL-c316t-392cb566c8d92b856c33bf0634a15e0ae0211d252ccfa895bc8b2c63d440c3b53</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>230,314,780,784,885,27924,27925</link.rule.ids><backlink>$$Uhttps://www.osti.gov/biblio/22054217$$D View this record in Osti.gov$$Hfree_for_read</backlink></links><search><creatorcontrib>Shilin, V. A.</creatorcontrib><creatorcontrib>Lebedev, V. T.</creatorcontrib><creatorcontrib>Kolesnik, S. G.</creatorcontrib><creatorcontrib>Kozlov, V. S.</creatorcontrib><creatorcontrib>Grushko, Yu. S.</creatorcontrib><creatorcontrib>Sedov, V. P.</creatorcontrib><creatorcontrib>Kukorenko, V. V.</creatorcontrib><title>Investigation of the neutron activation of endohedral rare earth metallofullerenes</title><title>Crystallography reports</title><addtitle>Crystallogr. Rep</addtitle><description>Endohedral lanthanide metallofullerenes and their water-soluble biocompatible derivatives have been synthesized. The effect that fast-neutron irradiation has on the stability and nuclear physical properties of endohedral metallofullerenes that are used as magnetocontrast materials (
46
Sc,
140
La,
141
Nd,
153
Sm,
152
Eu,
154
Eu,
153
Sm,
160
Tb,
169
Yb,
170
Tm (isomers I and III), and
177
Lu) is studied. Our hypothesis, according to which carbon-shell relaxation is based on the fast nonradiative processes of an electron shake-off type, is confirmed.</description><subject>CARBON</subject><subject>Crystallography and Scattering Methods</subject><subject>EUROPIUM 152</subject><subject>EUROPIUM 154</subject><subject>FAST NEUTRONS</subject><subject>INORGANIC, ORGANIC, PHYSICAL AND ANALYTICAL CHEMISTRY</subject><subject>IRRADIATION</subject><subject>ISOMERS</subject><subject>LANTHANUM 140</subject><subject>LUTETIUM 177</subject><subject>Nanomaterials and Ceramics</subject><subject>NEODYMIUM 141</subject><subject>NEUTRON ACTIVATION ANALYSIS</subject><subject>PHYSICAL PROPERTIES</subject><subject>Physics</subject><subject>Physics and Astronomy</subject><subject>RADIATION CHEMISTRY, RADIOCHEMISTRY AND NUCLEAR CHEMISTRY</subject><subject>RARE EARTH COMPLEXES</subject><subject>RELAXATION</subject><subject>SAMARIUM 153</subject><subject>SCANDIUM 46</subject><subject>STABILITY</subject><subject>TERBIUM 160</subject><subject>THULIUM 170</subject><subject>YTTERBIUM 169</subject><issn>1063-7745</issn><issn>1562-689X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2011</creationdate><recordtype>article</recordtype><recordid>eNp9UE1LxDAQDaLguvoDvBU8VzNJk7ZHWfxYWBD8AG8lnU63XbqJJNkF_72RFS-Cp5nhvTe89xi7BH4NIIubF-BalmWhAHjJpayP2AyUFrmu6vfjtCc4_8ZP2VkIG855VUExY89Lu6cQx7WJo7OZ67M4UGZpF306DcZx_4uQ7dxAnTdT5o2njIyPQ7alaKbJ9btpIk-Wwjk76c0U6OJnztnb_d3r4jFfPT0sF7erHCXomMtaYKu0xqqrRVspjVK2fbJZGFDEDXEB0AklEHtT1arFqhWoZVcUHGWr5JxdHf665L8JOEbCAZ21hLERgqtCQJlYcGChdyF46psPP26N_2yAN9_VNX-qSxpx0ITEtWvyzcbtvE1h_hF9AfJecPU</recordid><startdate>20111201</startdate><enddate>20111201</enddate><creator>Shilin, V. A.</creator><creator>Lebedev, V. T.</creator><creator>Kolesnik, S. G.</creator><creator>Kozlov, V. S.</creator><creator>Grushko, Yu. S.</creator><creator>Sedov, V. P.</creator><creator>Kukorenko, V. V.</creator><general>SP MAIK Nauka/Interperiodica</general><scope>AAYXX</scope><scope>CITATION</scope><scope>OTOTI</scope></search><sort><creationdate>20111201</creationdate><title>Investigation of the neutron activation of endohedral rare earth metallofullerenes</title><author>Shilin, V. A. ; Lebedev, V. T. ; Kolesnik, S. G. ; Kozlov, V. S. ; Grushko, Yu. S. ; Sedov, V. P. ; Kukorenko, V. V.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c316t-392cb566c8d92b856c33bf0634a15e0ae0211d252ccfa895bc8b2c63d440c3b53</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2011</creationdate><topic>CARBON</topic><topic>Crystallography and Scattering Methods</topic><topic>EUROPIUM 152</topic><topic>EUROPIUM 154</topic><topic>FAST NEUTRONS</topic><topic>INORGANIC, ORGANIC, PHYSICAL AND ANALYTICAL CHEMISTRY</topic><topic>IRRADIATION</topic><topic>ISOMERS</topic><topic>LANTHANUM 140</topic><topic>LUTETIUM 177</topic><topic>Nanomaterials and Ceramics</topic><topic>NEODYMIUM 141</topic><topic>NEUTRON ACTIVATION ANALYSIS</topic><topic>PHYSICAL PROPERTIES</topic><topic>Physics</topic><topic>Physics and Astronomy</topic><topic>RADIATION CHEMISTRY, RADIOCHEMISTRY AND NUCLEAR CHEMISTRY</topic><topic>RARE EARTH COMPLEXES</topic><topic>RELAXATION</topic><topic>SAMARIUM 153</topic><topic>SCANDIUM 46</topic><topic>STABILITY</topic><topic>TERBIUM 160</topic><topic>THULIUM 170</topic><topic>YTTERBIUM 169</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Shilin, V. A.</creatorcontrib><creatorcontrib>Lebedev, V. T.</creatorcontrib><creatorcontrib>Kolesnik, S. G.</creatorcontrib><creatorcontrib>Kozlov, V. S.</creatorcontrib><creatorcontrib>Grushko, Yu. S.</creatorcontrib><creatorcontrib>Sedov, V. P.</creatorcontrib><creatorcontrib>Kukorenko, V. V.</creatorcontrib><collection>CrossRef</collection><collection>OSTI.GOV</collection><jtitle>Crystallography reports</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Shilin, V. A.</au><au>Lebedev, V. T.</au><au>Kolesnik, S. G.</au><au>Kozlov, V. S.</au><au>Grushko, Yu. S.</au><au>Sedov, V. P.</au><au>Kukorenko, V. V.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Investigation of the neutron activation of endohedral rare earth metallofullerenes</atitle><jtitle>Crystallography reports</jtitle><stitle>Crystallogr. Rep</stitle><date>2011-12-01</date><risdate>2011</risdate><volume>56</volume><issue>7</issue><spage>1192</spage><epage>1196</epage><pages>1192-1196</pages><issn>1063-7745</issn><eissn>1562-689X</eissn><abstract>Endohedral lanthanide metallofullerenes and their water-soluble biocompatible derivatives have been synthesized. The effect that fast-neutron irradiation has on the stability and nuclear physical properties of endohedral metallofullerenes that are used as magnetocontrast materials (
46
Sc,
140
La,
141
Nd,
153
Sm,
152
Eu,
154
Eu,
153
Sm,
160
Tb,
169
Yb,
170
Tm (isomers I and III), and
177
Lu) is studied. Our hypothesis, according to which carbon-shell relaxation is based on the fast nonradiative processes of an electron shake-off type, is confirmed.</abstract><cop>Dordrecht</cop><pub>SP MAIK Nauka/Interperiodica</pub><doi>10.1134/S1063774511070339</doi><tpages>5</tpages></addata></record> |
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language | eng |
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source | Springer Nature |
subjects | CARBON Crystallography and Scattering Methods EUROPIUM 152 EUROPIUM 154 FAST NEUTRONS INORGANIC, ORGANIC, PHYSICAL AND ANALYTICAL CHEMISTRY IRRADIATION ISOMERS LANTHANUM 140 LUTETIUM 177 Nanomaterials and Ceramics NEODYMIUM 141 NEUTRON ACTIVATION ANALYSIS PHYSICAL PROPERTIES Physics Physics and Astronomy RADIATION CHEMISTRY, RADIOCHEMISTRY AND NUCLEAR CHEMISTRY RARE EARTH COMPLEXES RELAXATION SAMARIUM 153 SCANDIUM 46 STABILITY TERBIUM 160 THULIUM 170 YTTERBIUM 169 |
title | Investigation of the neutron activation of endohedral rare earth metallofullerenes |
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