Loading…
Second-order nonlinear optical metamaterials: ABC-type nanolaminates
We demonstrate a concept for second-order nonlinear metamaterials that can be obtained from non-metallic centrosymmetric constituents with inherently low optical absorption. The concept is based on iterative atomic-layer deposition of three different materials, A = Al2O3, B = TiO2, and C = HfO2. The...
Saved in:
| Published in: | Applied physics letters 2015-09, Vol.107 (12) |
|---|---|
| Main Authors: | , , , , , , , , , |
| Format: | Article |
| Language: | English |
| Subjects: | |
| Citations: | Items that this one cites Items that cite this one |
| Online Access: | Get full text |
| Tags: |
Add Tag
No Tags, Be the first to tag this record!
|
| cited_by | cdi_FETCH-LOGICAL-c285t-99cbc9018ae40fd2865f5237fed96755bc2bec3f45803ac39e149cadd0fd2bfd3 |
|---|---|
| cites | cdi_FETCH-LOGICAL-c285t-99cbc9018ae40fd2865f5237fed96755bc2bec3f45803ac39e149cadd0fd2bfd3 |
| container_end_page | |
| container_issue | 12 |
| container_start_page | |
| container_title | Applied physics letters |
| container_volume | 107 |
| creator | Alloatti, L. Kieninger, C. Froelich, A. Lauermann, M. Frenzel, T. Köhnle, K. Freude, W. Leuthold, J. Wegener, M. Koos, C. |
| description | We demonstrate a concept for second-order nonlinear metamaterials that can be obtained from non-metallic centrosymmetric constituents with inherently low optical absorption. The concept is based on iterative atomic-layer deposition of three different materials, A = Al2O3, B = TiO2, and C = HfO2. The centrosymmetry of the resulting ABC stack is broken since the ABC and the inverted CBA sequences are not equivalent—a necessary condition for non-zero second-order nonlinearity. In our experiments, we find that the bulk second-order nonlinear susceptibility depends on the density of interfaces, leading to a nonlinear susceptibility of 0.26 pm/V at a wavelength of 800 nm. ABC-type nanolaminates can be deposited on virtually any substrate and offer a promising route towards engineering of second-order optical nonlinearities at both infrared and visible wavelengths. |
| doi_str_mv | 10.1063/1.4931492 |
| format | article |
| fullrecord | <record><control><sourceid>proquest_osti_</sourceid><recordid>TN_cdi_osti_scitechconnect_22482119</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2124098010</sourcerecordid><originalsourceid>FETCH-LOGICAL-c285t-99cbc9018ae40fd2865f5237fed96755bc2bec3f45803ac39e149cadd0fd2bfd3</originalsourceid><addsrcrecordid>eNpFkE1LAzEQhoMoWKsH_8GCJw9bM8l-xVtt_YKCB_UcssksbtlN1iQ99N-b0oKnYXgfhmdeQm6BLoBW_AEWheBQCHZGZkDrOucAzTmZUUp5XokSLslVCNu0lozzGVl_onbW5M4b9Jl1dugtKp-5KfZaDdmIUY0qou_VEB6z5dMqj_sJM6usG9TY25SFa3LRpRhvTnNOvl-ev1Zv-ebj9X213OSaNWXMhdCtFhQahQXtDGuqsksWdYdGVHVZtpq1qHlXlA3lSnOB6RGtjDnAbWf4nNwd77oQexl0H1H_JH2LOkrGioYBiH9q8u53hyHKrdt5m8QkA1ZQ0VCgibo_Utq7EDx2cvL9qPxeApWHKiXIU5X8D4TeZRM</addsrcrecordid><sourcetype>Open Access Repository</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2124098010</pqid></control><display><type>article</type><title>Second-order nonlinear optical metamaterials: ABC-type nanolaminates</title><source>American Institute of Physics:Jisc Collections:Transitional Journals Agreement 2021-23 (Reading list)</source><source>AIP Journals (American Institute of Physics)</source><creator>Alloatti, L. ; Kieninger, C. ; Froelich, A. ; Lauermann, M. ; Frenzel, T. ; Köhnle, K. ; Freude, W. ; Leuthold, J. ; Wegener, M. ; Koos, C.</creator><creatorcontrib>Alloatti, L. ; Kieninger, C. ; Froelich, A. ; Lauermann, M. ; Frenzel, T. ; Köhnle, K. ; Freude, W. ; Leuthold, J. ; Wegener, M. ; Koos, C.</creatorcontrib><description>We demonstrate a concept for second-order nonlinear metamaterials that can be obtained from non-metallic centrosymmetric constituents with inherently low optical absorption. The concept is based on iterative atomic-layer deposition of three different materials, A = Al2O3, B = TiO2, and C = HfO2. The centrosymmetry of the resulting ABC stack is broken since the ABC and the inverted CBA sequences are not equivalent—a necessary condition for non-zero second-order nonlinearity. In our experiments, we find that the bulk second-order nonlinear susceptibility depends on the density of interfaces, leading to a nonlinear susceptibility of 0.26 pm/V at a wavelength of 800 nm. ABC-type nanolaminates can be deposited on virtually any substrate and offer a promising route towards engineering of second-order optical nonlinearities at both infrared and visible wavelengths.</description><identifier>ISSN: 0003-6951</identifier><identifier>EISSN: 1077-3118</identifier><identifier>DOI: 10.1063/1.4931492</identifier><language>eng</language><publisher>Melville: American Institute of Physics</publisher><subject>ABSORPTION ; ALUMINIUM OXIDES ; Aluminum oxide ; Applied physics ; Bulk density ; CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS ; DEPOSITS ; Hafnium oxide ; HAFNIUM OXIDES ; INTERFACES ; ITERATIVE METHODS ; METAMATERIALS ; Nonlinear optics ; NONLINEAR PROBLEMS ; Nonlinearity ; Sequences ; SUBSTRATES ; Titanium dioxide ; TITANIUM OXIDES ; WAVELENGTHS</subject><ispartof>Applied physics letters, 2015-09, Vol.107 (12)</ispartof><rights>2015 AIP Publishing LLC.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c285t-99cbc9018ae40fd2865f5237fed96755bc2bec3f45803ac39e149cadd0fd2bfd3</citedby><cites>FETCH-LOGICAL-c285t-99cbc9018ae40fd2865f5237fed96755bc2bec3f45803ac39e149cadd0fd2bfd3</cites><orcidid>0000-0002-1245-4179</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>230,314,780,782,784,885,27924,27925</link.rule.ids><backlink>$$Uhttps://www.osti.gov/biblio/22482119$$D View this record in Osti.gov$$Hfree_for_read</backlink></links><search><creatorcontrib>Alloatti, L.</creatorcontrib><creatorcontrib>Kieninger, C.</creatorcontrib><creatorcontrib>Froelich, A.</creatorcontrib><creatorcontrib>Lauermann, M.</creatorcontrib><creatorcontrib>Frenzel, T.</creatorcontrib><creatorcontrib>Köhnle, K.</creatorcontrib><creatorcontrib>Freude, W.</creatorcontrib><creatorcontrib>Leuthold, J.</creatorcontrib><creatorcontrib>Wegener, M.</creatorcontrib><creatorcontrib>Koos, C.</creatorcontrib><title>Second-order nonlinear optical metamaterials: ABC-type nanolaminates</title><title>Applied physics letters</title><description>We demonstrate a concept for second-order nonlinear metamaterials that can be obtained from non-metallic centrosymmetric constituents with inherently low optical absorption. The concept is based on iterative atomic-layer deposition of three different materials, A = Al2O3, B = TiO2, and C = HfO2. The centrosymmetry of the resulting ABC stack is broken since the ABC and the inverted CBA sequences are not equivalent—a necessary condition for non-zero second-order nonlinearity. In our experiments, we find that the bulk second-order nonlinear susceptibility depends on the density of interfaces, leading to a nonlinear susceptibility of 0.26 pm/V at a wavelength of 800 nm. ABC-type nanolaminates can be deposited on virtually any substrate and offer a promising route towards engineering of second-order optical nonlinearities at both infrared and visible wavelengths.</description><subject>ABSORPTION</subject><subject>ALUMINIUM OXIDES</subject><subject>Aluminum oxide</subject><subject>Applied physics</subject><subject>Bulk density</subject><subject>CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS</subject><subject>DEPOSITS</subject><subject>Hafnium oxide</subject><subject>HAFNIUM OXIDES</subject><subject>INTERFACES</subject><subject>ITERATIVE METHODS</subject><subject>METAMATERIALS</subject><subject>Nonlinear optics</subject><subject>NONLINEAR PROBLEMS</subject><subject>Nonlinearity</subject><subject>Sequences</subject><subject>SUBSTRATES</subject><subject>Titanium dioxide</subject><subject>TITANIUM OXIDES</subject><subject>WAVELENGTHS</subject><issn>0003-6951</issn><issn>1077-3118</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2015</creationdate><recordtype>article</recordtype><recordid>eNpFkE1LAzEQhoMoWKsH_8GCJw9bM8l-xVtt_YKCB_UcssksbtlN1iQ99N-b0oKnYXgfhmdeQm6BLoBW_AEWheBQCHZGZkDrOucAzTmZUUp5XokSLslVCNu0lozzGVl_onbW5M4b9Jl1dugtKp-5KfZaDdmIUY0qou_VEB6z5dMqj_sJM6usG9TY25SFa3LRpRhvTnNOvl-ev1Zv-ebj9X213OSaNWXMhdCtFhQahQXtDGuqsksWdYdGVHVZtpq1qHlXlA3lSnOB6RGtjDnAbWf4nNwd77oQexl0H1H_JH2LOkrGioYBiH9q8u53hyHKrdt5m8QkA1ZQ0VCgibo_Utq7EDx2cvL9qPxeApWHKiXIU5X8D4TeZRM</recordid><startdate>20150921</startdate><enddate>20150921</enddate><creator>Alloatti, L.</creator><creator>Kieninger, C.</creator><creator>Froelich, A.</creator><creator>Lauermann, M.</creator><creator>Frenzel, T.</creator><creator>Köhnle, K.</creator><creator>Freude, W.</creator><creator>Leuthold, J.</creator><creator>Wegener, M.</creator><creator>Koos, C.</creator><general>American Institute of Physics</general><scope>AAYXX</scope><scope>CITATION</scope><scope>8FD</scope><scope>H8D</scope><scope>L7M</scope><scope>OTOTI</scope><orcidid>https://orcid.org/0000-0002-1245-4179</orcidid></search><sort><creationdate>20150921</creationdate><title>Second-order nonlinear optical metamaterials: ABC-type nanolaminates</title><author>Alloatti, L. ; Kieninger, C. ; Froelich, A. ; Lauermann, M. ; Frenzel, T. ; Köhnle, K. ; Freude, W. ; Leuthold, J. ; Wegener, M. ; Koos, C.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c285t-99cbc9018ae40fd2865f5237fed96755bc2bec3f45803ac39e149cadd0fd2bfd3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2015</creationdate><topic>ABSORPTION</topic><topic>ALUMINIUM OXIDES</topic><topic>Aluminum oxide</topic><topic>Applied physics</topic><topic>Bulk density</topic><topic>CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS</topic><topic>DEPOSITS</topic><topic>Hafnium oxide</topic><topic>HAFNIUM OXIDES</topic><topic>INTERFACES</topic><topic>ITERATIVE METHODS</topic><topic>METAMATERIALS</topic><topic>Nonlinear optics</topic><topic>NONLINEAR PROBLEMS</topic><topic>Nonlinearity</topic><topic>Sequences</topic><topic>SUBSTRATES</topic><topic>Titanium dioxide</topic><topic>TITANIUM OXIDES</topic><topic>WAVELENGTHS</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Alloatti, L.</creatorcontrib><creatorcontrib>Kieninger, C.</creatorcontrib><creatorcontrib>Froelich, A.</creatorcontrib><creatorcontrib>Lauermann, M.</creatorcontrib><creatorcontrib>Frenzel, T.</creatorcontrib><creatorcontrib>Köhnle, K.</creatorcontrib><creatorcontrib>Freude, W.</creatorcontrib><creatorcontrib>Leuthold, J.</creatorcontrib><creatorcontrib>Wegener, M.</creatorcontrib><creatorcontrib>Koos, C.</creatorcontrib><collection>CrossRef</collection><collection>Technology Research Database</collection><collection>Aerospace Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>OSTI.GOV</collection><jtitle>Applied physics letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Alloatti, L.</au><au>Kieninger, C.</au><au>Froelich, A.</au><au>Lauermann, M.</au><au>Frenzel, T.</au><au>Köhnle, K.</au><au>Freude, W.</au><au>Leuthold, J.</au><au>Wegener, M.</au><au>Koos, C.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Second-order nonlinear optical metamaterials: ABC-type nanolaminates</atitle><jtitle>Applied physics letters</jtitle><date>2015-09-21</date><risdate>2015</risdate><volume>107</volume><issue>12</issue><issn>0003-6951</issn><eissn>1077-3118</eissn><abstract>We demonstrate a concept for second-order nonlinear metamaterials that can be obtained from non-metallic centrosymmetric constituents with inherently low optical absorption. The concept is based on iterative atomic-layer deposition of three different materials, A = Al2O3, B = TiO2, and C = HfO2. The centrosymmetry of the resulting ABC stack is broken since the ABC and the inverted CBA sequences are not equivalent—a necessary condition for non-zero second-order nonlinearity. In our experiments, we find that the bulk second-order nonlinear susceptibility depends on the density of interfaces, leading to a nonlinear susceptibility of 0.26 pm/V at a wavelength of 800 nm. ABC-type nanolaminates can be deposited on virtually any substrate and offer a promising route towards engineering of second-order optical nonlinearities at both infrared and visible wavelengths.</abstract><cop>Melville</cop><pub>American Institute of Physics</pub><doi>10.1063/1.4931492</doi><orcidid>https://orcid.org/0000-0002-1245-4179</orcidid></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 0003-6951 |
| ispartof | Applied physics letters, 2015-09, Vol.107 (12) |
| issn | 0003-6951 1077-3118 |
| language | eng |
| recordid | cdi_osti_scitechconnect_22482119 |
| source | American Institute of Physics:Jisc Collections:Transitional Journals Agreement 2021-23 (Reading list); AIP Journals (American Institute of Physics) |
| subjects | ABSORPTION ALUMINIUM OXIDES Aluminum oxide Applied physics Bulk density CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS DEPOSITS Hafnium oxide HAFNIUM OXIDES INTERFACES ITERATIVE METHODS METAMATERIALS Nonlinear optics NONLINEAR PROBLEMS Nonlinearity Sequences SUBSTRATES Titanium dioxide TITANIUM OXIDES WAVELENGTHS |
| title | Second-order nonlinear optical metamaterials: ABC-type nanolaminates |
| url | http://sfxeu10.hosted.exlibrisgroup.com/loughborough?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2024-12-23T08%3A52%3A58IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_osti_&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Second-order%20nonlinear%20optical%20metamaterials:%20ABC-type%20nanolaminates&rft.jtitle=Applied%20physics%20letters&rft.au=Alloatti,%20L.&rft.date=2015-09-21&rft.volume=107&rft.issue=12&rft.issn=0003-6951&rft.eissn=1077-3118&rft_id=info:doi/10.1063/1.4931492&rft_dat=%3Cproquest_osti_%3E2124098010%3C/proquest_osti_%3E%3Cgrp_id%3Ecdi_FETCH-LOGICAL-c285t-99cbc9018ae40fd2865f5237fed96755bc2bec3f45803ac39e149cadd0fd2bfd3%3C/grp_id%3E%3Coa%3E%3C/oa%3E%3Curl%3E%3C/url%3E&rft_id=info:oai/&rft_pqid=2124098010&rft_id=info:pmid/&rfr_iscdi=true |