Pulse-fluence-specified optimal control simulation with applications to molecular orientation and spin-isomer-selective molecular alignment

We propose an optimal control simulation with specified pulse fluence and amplitude. The simulation is applied to the orientation control of CO molecules to examine the optimal combination of THz and laser pulses, and to discriminate nuclear-spin isomers of 14N2 as spatially anisotropic distribution...

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Bibliographic Details
Main Authors: Yoshida, Masataka, Nakashima, Kaoru, Ohtsuki, Yukiyoshi
Format: Conference Proceeding
Language:English
Subjects:
ALIGNMENT
AMPLITUDES
ANISOTROPY
CARBON MONOXIDE
CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS
Control simulation
DISTRIBUTION
Fluence
ISOMERS
LASER RADIATION
MOLECULES
NITROGEN 14
OPTIMAL CONTROL
PULSES
SIMULATION
SPIN
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Summary:We propose an optimal control simulation with specified pulse fluence and amplitude. The simulation is applied to the orientation control of CO molecules to examine the optimal combination of THz and laser pulses, and to discriminate nuclear-spin isomers of 14N2 as spatially anisotropic distributions.
ISSN:0094-243X
1551-7616
DOI:10.1063/1.4938840