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Impurity-induced changes of overlayer symmetry and of phase transitions

We show in a Low Energy Electron Diffraction (LEED) experiment that small concentrations of oxygen atoms (2 to 12% of a monolayer) added to half a monolayer of Sr on Mo(112), ordered in a $c(2\times 2)$ structure, do not destroy order, but introduce new correlations with different translational symm...

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Bibliographic Details
Published in:Europhysics letters 2001-10, Vol.56 (1), p.67-73
Main Authors: Godzik, G, Pfnür, H, Lyuksyutov, I. F
Format: Article
Language:English
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Summary:We show in a Low Energy Electron Diffraction (LEED) experiment that small concentrations of oxygen atoms (2 to 12% of a monolayer) added to half a monolayer of Sr on Mo(112), ordered in a $c(2\times 2)$ structure, do not destroy order, but introduce new correlations with different translational symmetry. Thus incommensurate structures with domain walls are formed and the $c(2\times 2)$ is finally transformed into a $p(2\times 1)$ structure. Temperature-driven transitions at constant average densities from incommensurate to short-range order and finally to long-range order at high temperature can be described by simultaneous melting and domain wall evaporation.
ISSN:0295-5075
1286-4854
DOI:10.1209/epl/i2001-00488-0