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Year-round chemical aerosol records in continental Antarctica obtained by automatic samplings
Aimed at year-round recording of the chemical aerosol composition in central Antarctica, an unattended operating aerosol sampler was successfully deployed at the EPICA deep drilling site in Dronning Maud Land (Kohnen Station). Analyses of teflon/nylon filter packs consecutively collected over bi-wee...
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Published in: | Tellus. Series B, Chemical and physical meteorology Chemical and physical meteorology, 2007-09, Vol.59 (4), p.755-765 |
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cites | cdi_FETCH-LOGICAL-c5163-1e0b0a29d2ad5bf6e1f7de7defe8375dab7f0a358f9082c6cd2c4b0bf122a6073 |
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container_title | Tellus. Series B, Chemical and physical meteorology |
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creator | Weller, Rolf Wagenbach, Dietmar |
description | Aimed at year-round recording of the chemical aerosol composition in central Antarctica, an unattended operating aerosol sampler was successfully deployed at the EPICA deep drilling site in Dronning Maud Land (Kohnen Station). Analyses of teflon/nylon filter packs consecutively collected over bi-weekly intervals during the February 2003 to December 2005 period allowed to evaluate seasonal concentration variations of methane sulphonate (MS), Cl
-
, NO
3
-
, non-sea salt (nss-)SO
4
2-
and Na
+
, while NH
4
+
and mineral dust related ion results remained below detection limits. For MS and nss-SO
4
2-
distinct late summer maxima around 44 and 200 ng m
-3
, respectively, were found, while (total) NO
3
-
showed a broad November maximum of about 52 ng m
-3
. In contrast, the highest concentrations of Na
+
with peak values of up to 160 ng m
-3
were observed during the winter half year. The seasonality of these species broadly coincided with long-term observations at the coastal Neumayer Station, including surprisingly comparable NO
3
-
levels. However, the biogenic sulphur and sea salt concentrations were lower at Kohnen by typically a factor of 2-3 and 10, respectively. The arrival of sea ice derived sea salt particles at Kohnen could not clearly detected, since even during mid-winter the nss-SO
4
2-
to Na
+
ratio was generally too high to unambiguously identify a sulphur depleted sea salt SO
4
2-
fraction. |
doi_str_mv | 10.1111/j.1600-0889.2007.00293.x |
format | article |
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-
, NO
3
-
, non-sea salt (nss-)SO
4
2-
and Na
+
, while NH
4
+
and mineral dust related ion results remained below detection limits. For MS and nss-SO
4
2-
distinct late summer maxima around 44 and 200 ng m
-3
, respectively, were found, while (total) NO
3
-
showed a broad November maximum of about 52 ng m
-3
. In contrast, the highest concentrations of Na
+
with peak values of up to 160 ng m
-3
were observed during the winter half year. The seasonality of these species broadly coincided with long-term observations at the coastal Neumayer Station, including surprisingly comparable NO
3
-
levels. However, the biogenic sulphur and sea salt concentrations were lower at Kohnen by typically a factor of 2-3 and 10, respectively. The arrival of sea ice derived sea salt particles at Kohnen could not clearly detected, since even during mid-winter the nss-SO
4
2-
to Na
+
ratio was generally too high to unambiguously identify a sulphur depleted sea salt SO
4
2-
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-
, NO
3
-
, non-sea salt (nss-)SO
4
2-
and Na
+
, while NH
4
+
and mineral dust related ion results remained below detection limits. For MS and nss-SO
4
2-
distinct late summer maxima around 44 and 200 ng m
-3
, respectively, were found, while (total) NO
3
-
showed a broad November maximum of about 52 ng m
-3
. In contrast, the highest concentrations of Na
+
with peak values of up to 160 ng m
-3
were observed during the winter half year. The seasonality of these species broadly coincided with long-term observations at the coastal Neumayer Station, including surprisingly comparable NO
3
-
levels. However, the biogenic sulphur and sea salt concentrations were lower at Kohnen by typically a factor of 2-3 and 10, respectively. The arrival of sea ice derived sea salt particles at Kohnen could not clearly detected, since even during mid-winter the nss-SO
4
2-
to Na
+
ratio was generally too high to unambiguously identify a sulphur depleted sea salt SO
4
2-
fraction.</description><subject>Aerosols</subject><subject>Antarctica</subject><subject>Chemical composition and interactions. Ionic interactions and processes</subject><subject>Concentration (composition)</subject><subject>Earth, ocean, space</subject><subject>Exact sciences and technology</subject><subject>External geophysics</subject><subject>Marine</subject><subject>Maxima</subject><subject>Meteorology</subject><subject>Particles and aerosols</subject><subject>Sampling</subject><subject>Stations</subject><subject>Sulfur</subject><subject>Sulphur</subject><issn>0280-6509</issn><issn>1600-0889</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2007</creationdate><recordtype>article</recordtype><sourceid>0YH</sourceid><recordid>eNqNkE1v1DAQhi0EEsuW_-ALiEvC2GkcW-JSVuVDqsSlHHqorIk_wCsnXuys2v33eNkCN6htja2Z952xHkIog5bV9XbbMgHQgJSq5QBDC8BV194_Ias_hadkBVxCI3pQz8mLUrYAcN4rsSK3Nw5zk9N-ttR8d1MwGCm6nEqKNDuTsi00zNSkeQmzm5davqgxm6VKaRoXrGlLxwPF_ZImrGlacNrFMH8rZ-SZx1jcy4d7Tb5-uLzefGquvnz8vLm4akzPRNcwByMgV5aj7UcvHPODdfV4J7uhtzgOHrDrpVcguRHGcnM-wugZ5yhg6Nbk9anvLqcfe1cWPYViXIw4u7QvmoMY6u6q8M0_hUz0rFPDUOOayJPUVBglO693OUyYD5qBPqLXW30krI-E9RG9_oVe31frq4cpWCpPn3E2ofz1S6WUHHjVvTvp7kJ0h0f319eX7-uj2jcne5h9yhPepRytXvAQU_49s_vvZ38Cv3euNQ</recordid><startdate>200709</startdate><enddate>200709</enddate><creator>Weller, Rolf</creator><creator>Wagenbach, Dietmar</creator><general>Taylor & Francis</general><general>Blackwell Publishing Ltd</general><general>Blackwell</general><scope>0YH</scope><scope>IQODW</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>8FD</scope><scope>H8D</scope><scope>L7M</scope><scope>7TG</scope><scope>7TV</scope><scope>7UA</scope><scope>C1K</scope><scope>F1W</scope><scope>H96</scope><scope>KL.</scope><scope>L.G</scope></search><sort><creationdate>200709</creationdate><title>Year-round chemical aerosol records in continental Antarctica obtained by automatic samplings</title><author>Weller, Rolf ; Wagenbach, Dietmar</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c5163-1e0b0a29d2ad5bf6e1f7de7defe8375dab7f0a358f9082c6cd2c4b0bf122a6073</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2007</creationdate><topic>Aerosols</topic><topic>Antarctica</topic><topic>Chemical composition and interactions. Ionic interactions and processes</topic><topic>Concentration (composition)</topic><topic>Earth, ocean, space</topic><topic>Exact sciences and technology</topic><topic>External geophysics</topic><topic>Marine</topic><topic>Maxima</topic><topic>Meteorology</topic><topic>Particles and aerosols</topic><topic>Sampling</topic><topic>Stations</topic><topic>Sulfur</topic><topic>Sulphur</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Weller, Rolf</creatorcontrib><creatorcontrib>Wagenbach, Dietmar</creatorcontrib><collection>Taylor & Francis Open Access</collection><collection>Pascal-Francis</collection><collection>CrossRef</collection><collection>Technology Research Database</collection><collection>Aerospace Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>Meteorological & Geoastrophysical Abstracts</collection><collection>Pollution Abstracts</collection><collection>Water Resources Abstracts</collection><collection>Environmental Sciences and Pollution Management</collection><collection>ASFA: Aquatic Sciences and Fisheries Abstracts</collection><collection>Aquatic Science & Fisheries Abstracts (ASFA) 2: Ocean Technology, Policy & Non-Living Resources</collection><collection>Meteorological & Geoastrophysical Abstracts - Academic</collection><collection>Aquatic Science & Fisheries Abstracts (ASFA) Professional</collection><jtitle>Tellus. Series B, Chemical and physical meteorology</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Weller, Rolf</au><au>Wagenbach, Dietmar</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Year-round chemical aerosol records in continental Antarctica obtained by automatic samplings</atitle><jtitle>Tellus. Series B, Chemical and physical meteorology</jtitle><date>2007-09</date><risdate>2007</risdate><volume>59</volume><issue>4</issue><spage>755</spage><epage>765</epage><pages>755-765</pages><issn>0280-6509</issn><eissn>1600-0889</eissn><coden>TSBMD7</coden><abstract>Aimed at year-round recording of the chemical aerosol composition in central Antarctica, an unattended operating aerosol sampler was successfully deployed at the EPICA deep drilling site in Dronning Maud Land (Kohnen Station). Analyses of teflon/nylon filter packs consecutively collected over bi-weekly intervals during the February 2003 to December 2005 period allowed to evaluate seasonal concentration variations of methane sulphonate (MS), Cl
-
, NO
3
-
, non-sea salt (nss-)SO
4
2-
and Na
+
, while NH
4
+
and mineral dust related ion results remained below detection limits. For MS and nss-SO
4
2-
distinct late summer maxima around 44 and 200 ng m
-3
, respectively, were found, while (total) NO
3
-
showed a broad November maximum of about 52 ng m
-3
. In contrast, the highest concentrations of Na
+
with peak values of up to 160 ng m
-3
were observed during the winter half year. The seasonality of these species broadly coincided with long-term observations at the coastal Neumayer Station, including surprisingly comparable NO
3
-
levels. However, the biogenic sulphur and sea salt concentrations were lower at Kohnen by typically a factor of 2-3 and 10, respectively. The arrival of sea ice derived sea salt particles at Kohnen could not clearly detected, since even during mid-winter the nss-SO
4
2-
to Na
+
ratio was generally too high to unambiguously identify a sulphur depleted sea salt SO
4
2-
fraction.</abstract><cop>Oxford, UK</cop><pub>Taylor & Francis</pub><doi>10.1111/j.1600-0889.2007.00293.x</doi><tpages>11</tpages><oa>free_for_read</oa></addata></record> |
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ispartof | Tellus. Series B, Chemical and physical meteorology, 2007-09, Vol.59 (4), p.755-765 |
issn | 0280-6509 1600-0889 |
language | eng |
recordid | cdi_pascalfrancis_primary_18999872 |
source | Taylor & Francis Open Access |
subjects | Aerosols Antarctica Chemical composition and interactions. Ionic interactions and processes Concentration (composition) Earth, ocean, space Exact sciences and technology External geophysics Marine Maxima Meteorology Particles and aerosols Sampling Stations Sulfur Sulphur |
title | Year-round chemical aerosol records in continental Antarctica obtained by automatic samplings |
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