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Threshold ionization spectroscopy of H2O, HDO and D2O and low-lying vibrational levels of HDO+ and D2O
Rotationally resolved photoelectron spectra of jet-cooled H 2 O, HDO and D 2 O have been recorded near the origin of the photoionising transition following single-photon ionization using the complementary techniques of mass-analysed threshold-ionization (MATI) and pulsed-field-ionization zero-kineti...
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| Published in: | Molecular physics 2015-12, Vol.113 (24), p.3918-3924 |
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| Format: | Article |
| Language: | English |
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| container_end_page | 3924 |
| container_issue | 24 |
| container_start_page | 3918 |
| container_title | Molecular physics |
| container_volume | 113 |
| creator | Lauzin, Clément Jacovella, Ugo Merkt, Frédéric |
| description | Rotationally resolved photoelectron spectra of jet-cooled H
2
O, HDO and D
2
O have been recorded near the origin of the
photoionising transition following single-photon ionization using the complementary techniques of mass-analysed threshold-ionization (MATI) and pulsed-field-ionization zero-kinetic-energy (PFI-ZEKE) photoelectron spectroscopy. A gas mixture of H
2
O, HDO and D
2
O with Ar was obtained by mixing H
2
O (ℓ) and D
2
O (ℓ) in a reservoir and bubbling Ar gas through the mixture. To unambiguously assign the photoelectron bands to H
2
O, HDO or D
2
O, the PFI-ZEKE photoelectron spectra of the mixture were compared to MATI spectra and to spectra of H
2
O. Analysis of the rotational structure of the origin bands (v
+
1
= 0, v
2
+
= 0, v
+
3
= 0) ← (v
1
= 0, v
2
= 0, v
3
= 0) of H
2
O, HDO and D
2
O and of the transitions to the (010), (020) and (100) levels of D
2
O
+
and the first excited level of the O-D stretching mode of HDO
+
provided new information on the photoionization dynamics of water and the energy level structure of HDO
+
and D
2
O
+
. |
| doi_str_mv | 10.1080/00268976.2015.1049971 |
| format | article |
| fullrecord | <record><control><sourceid>proquest_infor</sourceid><recordid>TN_cdi_proquest_journals_1749007522</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>3895404771</sourcerecordid><originalsourceid>FETCH-LOGICAL-i217t-47ff653ccf06652e220d246d55d43bb9862374fde84ef904d2c7e8f693868cb03</originalsourceid><addsrcrecordid>eNo1kF1LwzAUhoMoOKc_QQh4qZ0nH03aO2VTJwx6M69D1ySuIzYz6Tbmr7fdx9ULh-d9OTwI3RMYEcjgGYCKLJdiRIGk3YnnuSQXaECYoAkDml2iQc8kPXSNbmJcAYAAAgNk58tg4tI7jWvf1H9l2wWOa1O1wcfKr_fYWzylxROeTgpcNhpP6DGd3yVuXzffeFsvwqFYOuzM1rh4KE2Kx3PhFl3Z0kVzd8oh-np_m4-nyaz4-By_zpKaEtkmXForUlZVFoRIqaEUNOVCp6nmbLHIM0GZ5FabjBubA9e0kiazImeZyKoFsCF6OO6ug__dmNiqld-E7q-oiOQ5gEwp7aiXI1U31oefcueD06ot984HG8qmqqNiBFRvV53tqt6uOtll_y2ka14</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>1749007522</pqid></control><display><type>article</type><title>Threshold ionization spectroscopy of H2O, HDO and D2O and low-lying vibrational levels of HDO+ and D2O</title><source>Taylor and Francis Science and Technology Collection</source><creator>Lauzin, Clément ; Jacovella, Ugo ; Merkt, Frédéric</creator><creatorcontrib>Lauzin, Clément ; Jacovella, Ugo ; Merkt, Frédéric</creatorcontrib><description>Rotationally resolved photoelectron spectra of jet-cooled H
2
O, HDO and D
2
O have been recorded near the origin of the
photoionising transition following single-photon ionization using the complementary techniques of mass-analysed threshold-ionization (MATI) and pulsed-field-ionization zero-kinetic-energy (PFI-ZEKE) photoelectron spectroscopy. A gas mixture of H
2
O, HDO and D
2
O with Ar was obtained by mixing H
2
O (ℓ) and D
2
O (ℓ) in a reservoir and bubbling Ar gas through the mixture. To unambiguously assign the photoelectron bands to H
2
O, HDO or D
2
O, the PFI-ZEKE photoelectron spectra of the mixture were compared to MATI spectra and to spectra of H
2
O. Analysis of the rotational structure of the origin bands (v
+
1
= 0, v
2
+
= 0, v
+
3
= 0) ← (v
1
= 0, v
2
= 0, v
3
= 0) of H
2
O, HDO and D
2
O and of the transitions to the (010), (020) and (100) levels of D
2
O
+
and the first excited level of the O-D stretching mode of HDO
+
provided new information on the photoionization dynamics of water and the energy level structure of HDO
+
and D
2
O
+
.</description><identifier>ISSN: 0026-8976</identifier><identifier>EISSN: 1362-3028</identifier><identifier>DOI: 10.1080/00268976.2015.1049971</identifier><language>eng</language><publisher>Abingdon: Taylor & Francis</publisher><subject>Lying ; MATI ; PFI-ZEKE photoelectron spectroscopy ; Spectrum analysis ; water</subject><ispartof>Molecular physics, 2015-12, Vol.113 (24), p.3918-3924</ispartof><rights>2015 Taylor & Francis 2015</rights><rights>2015 Taylor & Francis</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,27922,27923</link.rule.ids></links><search><creatorcontrib>Lauzin, Clément</creatorcontrib><creatorcontrib>Jacovella, Ugo</creatorcontrib><creatorcontrib>Merkt, Frédéric</creatorcontrib><title>Threshold ionization spectroscopy of H2O, HDO and D2O and low-lying vibrational levels of HDO+ and D2O</title><title>Molecular physics</title><description>Rotationally resolved photoelectron spectra of jet-cooled H
2
O, HDO and D
2
O have been recorded near the origin of the
photoionising transition following single-photon ionization using the complementary techniques of mass-analysed threshold-ionization (MATI) and pulsed-field-ionization zero-kinetic-energy (PFI-ZEKE) photoelectron spectroscopy. A gas mixture of H
2
O, HDO and D
2
O with Ar was obtained by mixing H
2
O (ℓ) and D
2
O (ℓ) in a reservoir and bubbling Ar gas through the mixture. To unambiguously assign the photoelectron bands to H
2
O, HDO or D
2
O, the PFI-ZEKE photoelectron spectra of the mixture were compared to MATI spectra and to spectra of H
2
O. Analysis of the rotational structure of the origin bands (v
+
1
= 0, v
2
+
= 0, v
+
3
= 0) ← (v
1
= 0, v
2
= 0, v
3
= 0) of H
2
O, HDO and D
2
O and of the transitions to the (010), (020) and (100) levels of D
2
O
+
and the first excited level of the O-D stretching mode of HDO
+
provided new information on the photoionization dynamics of water and the energy level structure of HDO
+
and D
2
O
+
.</description><subject>Lying</subject><subject>MATI</subject><subject>PFI-ZEKE photoelectron spectroscopy</subject><subject>Spectrum analysis</subject><subject>water</subject><issn>0026-8976</issn><issn>1362-3028</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2015</creationdate><recordtype>article</recordtype><recordid>eNo1kF1LwzAUhoMoOKc_QQh4qZ0nH03aO2VTJwx6M69D1ySuIzYz6Tbmr7fdx9ULh-d9OTwI3RMYEcjgGYCKLJdiRIGk3YnnuSQXaECYoAkDml2iQc8kPXSNbmJcAYAAAgNk58tg4tI7jWvf1H9l2wWOa1O1wcfKr_fYWzylxROeTgpcNhpP6DGd3yVuXzffeFsvwqFYOuzM1rh4KE2Kx3PhFl3Z0kVzd8oh-np_m4-nyaz4-By_zpKaEtkmXForUlZVFoRIqaEUNOVCp6nmbLHIM0GZ5FabjBubA9e0kiazImeZyKoFsCF6OO6ug__dmNiqld-E7q-oiOQ5gEwp7aiXI1U31oefcueD06ot984HG8qmqqNiBFRvV53tqt6uOtll_y2ka14</recordid><startdate>20151217</startdate><enddate>20151217</enddate><creator>Lauzin, Clément</creator><creator>Jacovella, Ugo</creator><creator>Merkt, Frédéric</creator><general>Taylor & Francis</general><general>Taylor & Francis Ltd</general><scope>7U5</scope><scope>8FD</scope><scope>H8D</scope><scope>L7M</scope></search><sort><creationdate>20151217</creationdate><title>Threshold ionization spectroscopy of H2O, HDO and D2O and low-lying vibrational levels of HDO+ and D2O</title><author>Lauzin, Clément ; Jacovella, Ugo ; Merkt, Frédéric</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-i217t-47ff653ccf06652e220d246d55d43bb9862374fde84ef904d2c7e8f693868cb03</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2015</creationdate><topic>Lying</topic><topic>MATI</topic><topic>PFI-ZEKE photoelectron spectroscopy</topic><topic>Spectrum analysis</topic><topic>water</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Lauzin, Clément</creatorcontrib><creatorcontrib>Jacovella, Ugo</creatorcontrib><creatorcontrib>Merkt, Frédéric</creatorcontrib><collection>Solid State and Superconductivity Abstracts</collection><collection>Technology Research Database</collection><collection>Aerospace Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Molecular physics</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Lauzin, Clément</au><au>Jacovella, Ugo</au><au>Merkt, Frédéric</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Threshold ionization spectroscopy of H2O, HDO and D2O and low-lying vibrational levels of HDO+ and D2O</atitle><jtitle>Molecular physics</jtitle><date>2015-12-17</date><risdate>2015</risdate><volume>113</volume><issue>24</issue><spage>3918</spage><epage>3924</epage><pages>3918-3924</pages><issn>0026-8976</issn><eissn>1362-3028</eissn><abstract>Rotationally resolved photoelectron spectra of jet-cooled H
2
O, HDO and D
2
O have been recorded near the origin of the
photoionising transition following single-photon ionization using the complementary techniques of mass-analysed threshold-ionization (MATI) and pulsed-field-ionization zero-kinetic-energy (PFI-ZEKE) photoelectron spectroscopy. A gas mixture of H
2
O, HDO and D
2
O with Ar was obtained by mixing H
2
O (ℓ) and D
2
O (ℓ) in a reservoir and bubbling Ar gas through the mixture. To unambiguously assign the photoelectron bands to H
2
O, HDO or D
2
O, the PFI-ZEKE photoelectron spectra of the mixture were compared to MATI spectra and to spectra of H
2
O. Analysis of the rotational structure of the origin bands (v
+
1
= 0, v
2
+
= 0, v
+
3
= 0) ← (v
1
= 0, v
2
= 0, v
3
= 0) of H
2
O, HDO and D
2
O and of the transitions to the (010), (020) and (100) levels of D
2
O
+
and the first excited level of the O-D stretching mode of HDO
+
provided new information on the photoionization dynamics of water and the energy level structure of HDO
+
and D
2
O
+
.</abstract><cop>Abingdon</cop><pub>Taylor & Francis</pub><doi>10.1080/00268976.2015.1049971</doi><tpages>7</tpages><oa>free_for_read</oa></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 0026-8976 |
| ispartof | Molecular physics, 2015-12, Vol.113 (24), p.3918-3924 |
| issn | 0026-8976 1362-3028 |
| language | eng |
| recordid | cdi_proquest_journals_1749007522 |
| source | Taylor and Francis Science and Technology Collection |
| subjects | Lying MATI PFI-ZEKE photoelectron spectroscopy Spectrum analysis water |
| title | Threshold ionization spectroscopy of H2O, HDO and D2O and low-lying vibrational levels of HDO+ and D2O |
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