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An Effective Asphalt UV Blocking Material Based on Host-Guest Schiff Base/Layered Double Hydroxides
The development of asphalt-based UV blocking materials is important to extend the alphalt lifespan in road construction. In this work, we put forward that the fabrication of host-guest system can be an effective way to obtain UV blocking materials. Firstly, a new anionic Schiff base, N,N'bis(salicyl...
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Published in: | Chinese journal of chemistry 2017-11, Vol.35 (11), p.1701-1705 |
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creator | Xia, Chunhui Gao, Rui Li, Kaitao Yang, Yang Lin, Yanjun Yan, Dongpeng |
description | The development of asphalt-based UV blocking materials is important to extend the alphalt lifespan in road construction. In this work, we put forward that the fabrication of host-guest system can be an effective way to obtain UV blocking materials. Firstly, a new anionic Schiff base, N,N'bis(salicylidine)-4,4'-diaminostilbene-2,2'-disulfonic acid (SDSD), has been synthesized, which was intercalated into Zn-Al-LDH by anion-exchange method. FT-IR and XRD illustrate the layered organic-inorganic composite, Zn-Al-SDSD-LDH, has been successfully synthesized with high crystallinity. Laser particle size analyzer, SEM and TEM show that particle size distributions of Zn-Al-SDSD-LDH is in the range 100--500 nm. UV-vis absorption spectra show that Zn-Al-SDSD-LDH has better UV absorption than the pristine Zn-Al-LDH and SDSD. Furthermore, the mixture of asphalt and 3 wt% Zn-Al-SDSD-LDH presents enhanced UV blocking property relative to the pristine asphalt after irradiating by UV spray accelerated weathering test. Therefore, this work not only develops a new type of host-guest Zn-Al-SDSD- LDH, but also confirms it can be an effective asphalt UV blocking material for practical application. |
doi_str_mv | 10.1002/cjoc.201700136 |
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In this work, we put forward that the fabrication of host-guest system can be an effective way to obtain UV blocking materials. Firstly, a new anionic Schiff base, N,N'bis(salicylidine)-4,4'-diaminostilbene-2,2'-disulfonic acid (SDSD), has been synthesized, which was intercalated into Zn-Al-LDH by anion-exchange method. FT-IR and XRD illustrate the layered organic-inorganic composite, Zn-Al-SDSD-LDH, has been successfully synthesized with high crystallinity. Laser particle size analyzer, SEM and TEM show that particle size distributions of Zn-Al-SDSD-LDH is in the range 100--500 nm. UV-vis absorption spectra show that Zn-Al-SDSD-LDH has better UV absorption than the pristine Zn-Al-LDH and SDSD. Furthermore, the mixture of asphalt and 3 wt% Zn-Al-SDSD-LDH presents enhanced UV blocking property relative to the pristine asphalt after irradiating by UV spray accelerated weathering test. Therefore, this work not only develops a new type of host-guest Zn-Al-SDSD- LDH, but also confirms it can be an effective asphalt UV blocking material for practical application.</description><identifier>ISSN: 1001-604X</identifier><identifier>EISSN: 1614-7065</identifier><identifier>DOI: 10.1002/cjoc.201700136</identifier><language>eng</language><publisher>Weinheim: WILEY-VCH Verlag GmbH & Co. KGaA</publisher><subject>Absorption ; Absorption spectra ; Accelerated tests ; Aluminum ; Anion exchanging ; Asphalt ; Composite materials ; Fabrication ; Host-guest materials ; Hydroxides ; Imines ; layered double hydroxides ; Life span ; Particle size ; Road construction ; Schiff base ; Synthesis ; Ultraviolet radiation ; UV blocking ; Weathering ; Zinc</subject><ispartof>Chinese journal of chemistry, 2017-11, Vol.35 (11), p.1701-1705</ispartof><rights>2017 SIOC, CAS, Shanghai, & WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim</rights><rights>2017 SIOC, CAS, Shanghai & WILEY-VCH Verlag GmbH & Co. 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In this work, we put forward that the fabrication of host-guest system can be an effective way to obtain UV blocking materials. Firstly, a new anionic Schiff base, N,N'bis(salicylidine)-4,4'-diaminostilbene-2,2'-disulfonic acid (SDSD), has been synthesized, which was intercalated into Zn-Al-LDH by anion-exchange method. FT-IR and XRD illustrate the layered organic-inorganic composite, Zn-Al-SDSD-LDH, has been successfully synthesized with high crystallinity. Laser particle size analyzer, SEM and TEM show that particle size distributions of Zn-Al-SDSD-LDH is in the range 100--500 nm. UV-vis absorption spectra show that Zn-Al-SDSD-LDH has better UV absorption than the pristine Zn-Al-LDH and SDSD. Furthermore, the mixture of asphalt and 3 wt% Zn-Al-SDSD-LDH presents enhanced UV blocking property relative to the pristine asphalt after irradiating by UV spray accelerated weathering test. 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Therefore, this work not only develops a new type of host-guest Zn-Al-SDSD- LDH, but also confirms it can be an effective asphalt UV blocking material for practical application.</abstract><cop>Weinheim</cop><pub>WILEY-VCH Verlag GmbH & Co. KGaA</pub><doi>10.1002/cjoc.201700136</doi><tpages>5</tpages></addata></record> |
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subjects | Absorption Absorption spectra Accelerated tests Aluminum Anion exchanging Asphalt Composite materials Fabrication Host-guest materials Hydroxides Imines layered double hydroxides Life span Particle size Road construction Schiff base Synthesis Ultraviolet radiation UV blocking Weathering Zinc |
title | An Effective Asphalt UV Blocking Material Based on Host-Guest Schiff Base/Layered Double Hydroxides |
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