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Exhaustive Screening of Long-Term Pollutants in Riverbank Sediments of the Wurm River, Germany
Fluvial sediments can act as archives for long-term pollution. However, in environmental studies, often only preselected contaminants and, therefore, only a limited part of the pollution are considered. Herein, geochemical investigations of riverbank samples of the Wurm River (catchment
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| Published in: | Water, air, and soil pollution air, and soil pollution, 2018-06, Vol.229 (6), p.1-23, Article 197 |
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| container_title | Water, air, and soil pollution |
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| creator | Hagemann, Lukas Buchty-Lemke, Michael Lehmkuhl, Frank Alzer, Jannika Kümmerle, Eberhard Andreas Schwarzbauer, Jan |
| description | Fluvial sediments can act as archives for long-term pollution. However, in environmental studies, often only preselected contaminants and, therefore, only a limited part of the pollution are considered. Herein, geochemical investigations of riverbank samples of the Wurm River (catchment |
| doi_str_mv | 10.1007/s11270-018-3843-9 |
| format | article |
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2
) depict the anthropogenic impact of the city Aachen (250,000 inhabitants) to its main outlet resulting in an exhaustive list of present pollutants including their concentrations. The study is based on 14 riverbank sediment samples at eight sampling sites on a 7.6-km-long segment of the Wurm River. The sediment samples were analyzed for grain size composition (laser diffraction particle size analyzer), total organic carbon (TOC), trace element inventory (X-ray fluorescence), and organic compounds (chromatography-mass spectrometry). Here, we report quantitative data for 71 persistent organic substances as well as six trace elements (Cu, Zn, As, Ba, Hg, and Pb) entering the Wurm River due to domestic and industrial emissions. In general, a slight decline of, e.g., PTEs, DDX, and PCB concentrations with decreasing sampling depth points to a steady improvement of conditions. Whereas no clear trends can be seen for organic pollutants along the investigated reach with increasing distance to the main source of pollution (Aachen city). As obtained concentrations for organic pollutants indicate a rather low level of pollution, trace element values exceed geogenic background values by far. Furthermore, we used selected compounds as time markers for a rough estimation of sedimentation rates. Obtained values point to a highly complex morphodynamic regime with changing sedimentation rates (0.6 to 3.0 cm a
−1
) within barely 100 m of river course.</description><identifier>ISSN: 0049-6979</identifier><identifier>EISSN: 1573-2932</identifier><identifier>DOI: 10.1007/s11270-018-3843-9</identifier><language>eng</language><publisher>Cham: Springer International Publishing</publisher><subject>Anthropogenic factors ; Archives ; Atmospheric Protection/Air Quality Control/Air Pollution ; Catchment area ; Climate Change/Climate Change Impacts ; Contaminants ; Depth perception ; Earth and Environmental Science ; Environment ; Environmental monitoring ; Environmental studies ; Fluorescence ; Fluvial sedimentation ; Fluvial sediments ; Geochemistry ; Geomorphology ; Human influences ; Hydrogeology ; Industrial emissions ; Lasers ; Lead ; Low level ; Mass spectrometry ; Mass spectroscopy ; Mercury ; Mercury (metal) ; Organic carbon ; Organic compounds ; Outlets ; PCB ; Pollutants ; Pollution ; Pollution levels ; Pollution sources ; Polychlorinated biphenyls ; River banks ; River catchments ; Riverbanks ; Rivers ; Sampling ; Sediment ; Sediment samplers ; Sediment samples ; Sedimentation ; Sedimentation & deposition ; Sedimentation rates ; Sediments ; Sediments (Geology) ; Size distribution ; Soil Science & Conservation ; Total organic carbon ; Trace elements ; Water analysis ; Water pollution ; Water Quality/Water Pollution ; X ray fluorescence analysis ; X-ray fluorescence ; Zinc</subject><ispartof>Water, air, and soil pollution, 2018-06, Vol.229 (6), p.1-23, Article 197</ispartof><rights>Springer International Publishing AG, part of Springer Nature 2018</rights><rights>COPYRIGHT 2018 Springer</rights><rights>Water, Air, & Soil Pollution is a copyright of Springer, (2018). All Rights Reserved.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c355t-e1f3dca8a9e78410598bfdf5406dd53791a68547273121ef075c9dff9f80e8cd3</citedby><cites>FETCH-LOGICAL-c355t-e1f3dca8a9e78410598bfdf5406dd53791a68547273121ef075c9dff9f80e8cd3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://www.proquest.com/docview/2049796715/fulltextPDF?pq-origsite=primo$$EPDF$$P50$$Gproquest$$H</linktopdf><linktohtml>$$Uhttps://www.proquest.com/docview/2049796715?pq-origsite=primo$$EHTML$$P50$$Gproquest$$H</linktohtml><link.rule.ids>314,780,784,11688,27924,27925,36060,44363,74895</link.rule.ids></links><search><creatorcontrib>Hagemann, Lukas</creatorcontrib><creatorcontrib>Buchty-Lemke, Michael</creatorcontrib><creatorcontrib>Lehmkuhl, Frank</creatorcontrib><creatorcontrib>Alzer, Jannika</creatorcontrib><creatorcontrib>Kümmerle, Eberhard Andreas</creatorcontrib><creatorcontrib>Schwarzbauer, Jan</creatorcontrib><title>Exhaustive Screening of Long-Term Pollutants in Riverbank Sediments of the Wurm River, Germany</title><title>Water, air, and soil pollution</title><addtitle>Water Air Soil Pollut</addtitle><description>Fluvial sediments can act as archives for long-term pollution. However, in environmental studies, often only preselected contaminants and, therefore, only a limited part of the pollution are considered. Herein, geochemical investigations of riverbank samples of the Wurm River (catchment < 400 km
2
) depict the anthropogenic impact of the city Aachen (250,000 inhabitants) to its main outlet resulting in an exhaustive list of present pollutants including their concentrations. The study is based on 14 riverbank sediment samples at eight sampling sites on a 7.6-km-long segment of the Wurm River. The sediment samples were analyzed for grain size composition (laser diffraction particle size analyzer), total organic carbon (TOC), trace element inventory (X-ray fluorescence), and organic compounds (chromatography-mass spectrometry). Here, we report quantitative data for 71 persistent organic substances as well as six trace elements (Cu, Zn, As, Ba, Hg, and Pb) entering the Wurm River due to domestic and industrial emissions. In general, a slight decline of, e.g., PTEs, DDX, and PCB concentrations with decreasing sampling depth points to a steady improvement of conditions. Whereas no clear trends can be seen for organic pollutants along the investigated reach with increasing distance to the main source of pollution (Aachen city). As obtained concentrations for organic pollutants indicate a rather low level of pollution, trace element values exceed geogenic background values by far. Furthermore, we used selected compounds as time markers for a rough estimation of sedimentation rates. Obtained values point to a highly complex morphodynamic regime with changing sedimentation rates (0.6 to 3.0 cm a
−1
) within barely 100 m of river course.</description><subject>Anthropogenic factors</subject><subject>Archives</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Catchment area</subject><subject>Climate Change/Climate Change Impacts</subject><subject>Contaminants</subject><subject>Depth perception</subject><subject>Earth and Environmental Science</subject><subject>Environment</subject><subject>Environmental monitoring</subject><subject>Environmental studies</subject><subject>Fluorescence</subject><subject>Fluvial sedimentation</subject><subject>Fluvial sediments</subject><subject>Geochemistry</subject><subject>Geomorphology</subject><subject>Human influences</subject><subject>Hydrogeology</subject><subject>Industrial emissions</subject><subject>Lasers</subject><subject>Lead</subject><subject>Low level</subject><subject>Mass spectrometry</subject><subject>Mass spectroscopy</subject><subject>Mercury</subject><subject>Mercury 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Germany</atitle><jtitle>Water, air, and soil pollution</jtitle><stitle>Water Air Soil Pollut</stitle><date>2018-06-01</date><risdate>2018</risdate><volume>229</volume><issue>6</issue><spage>1</spage><epage>23</epage><pages>1-23</pages><artnum>197</artnum><issn>0049-6979</issn><eissn>1573-2932</eissn><abstract>Fluvial sediments can act as archives for long-term pollution. However, in environmental studies, often only preselected contaminants and, therefore, only a limited part of the pollution are considered. Herein, geochemical investigations of riverbank samples of the Wurm River (catchment < 400 km
2
) depict the anthropogenic impact of the city Aachen (250,000 inhabitants) to its main outlet resulting in an exhaustive list of present pollutants including their concentrations. The study is based on 14 riverbank sediment samples at eight sampling sites on a 7.6-km-long segment of the Wurm River. The sediment samples were analyzed for grain size composition (laser diffraction particle size analyzer), total organic carbon (TOC), trace element inventory (X-ray fluorescence), and organic compounds (chromatography-mass spectrometry). Here, we report quantitative data for 71 persistent organic substances as well as six trace elements (Cu, Zn, As, Ba, Hg, and Pb) entering the Wurm River due to domestic and industrial emissions. In general, a slight decline of, e.g., PTEs, DDX, and PCB concentrations with decreasing sampling depth points to a steady improvement of conditions. Whereas no clear trends can be seen for organic pollutants along the investigated reach with increasing distance to the main source of pollution (Aachen city). As obtained concentrations for organic pollutants indicate a rather low level of pollution, trace element values exceed geogenic background values by far. Furthermore, we used selected compounds as time markers for a rough estimation of sedimentation rates. Obtained values point to a highly complex morphodynamic regime with changing sedimentation rates (0.6 to 3.0 cm a
−1
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| ispartof | Water, air, and soil pollution, 2018-06, Vol.229 (6), p.1-23, Article 197 |
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| subjects | Anthropogenic factors Archives Atmospheric Protection/Air Quality Control/Air Pollution Catchment area Climate Change/Climate Change Impacts Contaminants Depth perception Earth and Environmental Science Environment Environmental monitoring Environmental studies Fluorescence Fluvial sedimentation Fluvial sediments Geochemistry Geomorphology Human influences Hydrogeology Industrial emissions Lasers Lead Low level Mass spectrometry Mass spectroscopy Mercury Mercury (metal) Organic carbon Organic compounds Outlets PCB Pollutants Pollution Pollution levels Pollution sources Polychlorinated biphenyls River banks River catchments Riverbanks Rivers Sampling Sediment Sediment samplers Sediment samples Sedimentation Sedimentation & deposition Sedimentation rates Sediments Sediments (Geology) Size distribution Soil Science & Conservation Total organic carbon Trace elements Water analysis Water pollution Water Quality/Water Pollution X ray fluorescence analysis X-ray fluorescence Zinc |
| title | Exhaustive Screening of Long-Term Pollutants in Riverbank Sediments of the Wurm River, Germany |
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