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Large-area epitaxial growth of MoSe2 via an incandescent molybdenum source

We have developed an incandescent Mo source to fabricate large-area single-crystalline MoSe2 thin films. The as-grown MoSe2 thin films were characterized using transmission electron microscopy, energy dispersive X-ray spectroscopy, atomic force microscopy, Raman spectroscopy, photoluminescence, refl...

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Bibliographic Details
Published in:arXiv.org 2017-06
Main Authors: Cheng, Man-Kit, Liang, Jing, Ying-Hoi Lai, Liang-Xi, Pang, Liu, Yi, Shen, Junying, Hou, Jianqiang, Qing Lin He, Xu, Bochao, Chen, Junshu, Wang, Gan, Liu, Chang, Lortz, Rolf, Sou, Iam-Keong
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Language:English
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Summary:We have developed an incandescent Mo source to fabricate large-area single-crystalline MoSe2 thin films. The as-grown MoSe2 thin films were characterized using transmission electron microscopy, energy dispersive X-ray spectroscopy, atomic force microscopy, Raman spectroscopy, photoluminescence, reflection high energy electron diffraction (RHEED) and angular resolved photoemission spectroscopy (ARPES). A new Raman characteristic peak at 1591 cm-1 was identified. Results from Raman spectroscopy, photoluminescence, RHEED and ARPES studies consistently reveal that large-area single crystalline mono-layer of MoSe2 could be achieved by this technique. This technique enjoys several advantages over conventional approaches and could be extended to the growth of other two-dimensional layered materials containing a low-vapor-pressure element.
ISSN:2331-8422