Electric Field Controlled Magnetic Anisotropy in a Single Molecule

We have measured quantum transport through an individual Fe\(_4\) single-molecule magnet embedded in a three-terminal device geometry. The characteristic zero-field splittings of adjacent charge states and their magnetic field evolution are observed in inelastic tunneling spectroscopy. We demonstrat...

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Published in:arXiv.org 2010-09
Main Authors: Zyazin, Alexander S, Johan W G van den Berg, Osorio, Edgar A, Herre S J van der Zant, Konstantinidis, Nikolaos P, Leijnse, Martin, Wegewijs, Maarten R, May, Falk, Hofstetter, Walter, Danieli, Chiara, Cornia, Andrea
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Language:English
Subjects:
Electric fields
Magnetic anisotropy
Magnetic properties
Magnetism
Quantum transport
Subtraction
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creator Zyazin, Alexander S
Johan W G van den Berg
Osorio, Edgar A
Herre S J van der Zant
Konstantinidis, Nikolaos P
Leijnse, Martin
Wegewijs, Maarten R
May, Falk
Hofstetter, Walter
Danieli, Chiara
Cornia, Andrea
description We have measured quantum transport through an individual Fe\(_4\) single-molecule magnet embedded in a three-terminal device geometry. The characteristic zero-field splittings of adjacent charge states and their magnetic field evolution are observed in inelastic tunneling spectroscopy. We demonstrate that the molecule retains its magnetic properties, and moreover, that the magnetic anisotropy is significantly enhanced by reversible electron addition / subtraction controlled with the gate voltage. Single-molecule magnetism can thus be electrically controlled.
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subjects Electric fields
Magnetic anisotropy
Magnetic properties
Magnetism
Quantum transport
Subtraction
title Electric Field Controlled Magnetic Anisotropy in a Single Molecule
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