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Moisture assisted perovskite film growth for high performance solar cells

Moisture is assumed to be detrimental to organometal trihalide perovskite, as excess water can damage the crystallinity of the perovskite structure. Here, we report a growth mode for via thermal annealing of the perovskite precursor film in a humid environment (e.g., ambient air) to greatly improve...

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Published in:	Applied physics letters 2014-11, Vol.105 (18)
Main Authors:	You, Jingbi, Yang, Yang (Michael), Hong, Ziruo, Song, Tze-Bin, Meng, Lei, Liu, Yongsheng, Jiang, Chengyang, Zhou, Huanping, Chang, Wei-Hsuan, Li, Gang, Yang, Yang
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Language:	English
Subjects:	Applied physics Carrier mobility Energy conversion efficiency Film growth Maximum power Moisture Optoelectronics Perovskite structure Perovskites Photovoltaic cells Photovoltaic conversion Service life assessment Solar cells Structural damage Water damage
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container_issue	18
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container_title	Applied physics letters
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creator	You, Jingbi Yang, Yang (Michael) Hong, Ziruo Song, Tze-Bin Meng, Lei Liu, Yongsheng Jiang, Chengyang Zhou, Huanping Chang, Wei-Hsuan Li, Gang Yang, Yang
description	Moisture is assumed to be detrimental to organometal trihalide perovskite, as excess water can damage the crystallinity of the perovskite structure. Here, we report a growth mode for via thermal annealing of the perovskite precursor film in a humid environment (e.g., ambient air) to greatly improve the film quality, grain size, carrier mobility, and lifetime. Our method produces devices with maximum power conversion efficiency of 17.1% and a fill factor of 80%, revealing a promising route to achieve high quality perovskite polycrystalline films with superior optoelectronic properties that can pave the way towards efficient photovoltaic conversion.
doi_str_mv	10.1063/1.4901510
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source	American Institute of Physics:Jisc Collections:Transitional Journals Agreement 2021-23 (Reading list); AIP Journals (American Institute of Physics)
subjects	Applied physics Carrier mobility Energy conversion efficiency Film growth Maximum power Moisture Optoelectronics Perovskite structure Perovskites Photovoltaic cells Photovoltaic conversion Service life assessment Solar cells Structural damage Water damage
title	Moisture assisted perovskite film growth for high performance solar cells
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