Crack formation and self-closing in shrinkable, granular packings

Many clays, soils, biological tissues, foods, and coatings are shrinkable, granular materials: they are composed of packed, hydrated grains that shrink when dried. In many cases, these packings crack during drying, critically hindering applications. However, while cracking has been widely studied fo...

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Bibliographic Details
Published in:Soft matter 2019, Vol.15 (23), p.4689-472
Main Authors: Cho, H. Jeremy, Lu, Nancy B, Howard, Michael P, Adams, Rebekah A, Datta, Sujit S
Format: Article
Language:English
Subjects:
Atrophy
Beads
Capillarity
Clay
Continuum modeling
Cracks
Drying
Evolution
Gels
Granular materials
Hydrogels
Shrinkage
Soil shrinkage
Substrates
Tissues
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Summary:Many clays, soils, biological tissues, foods, and coatings are shrinkable, granular materials: they are composed of packed, hydrated grains that shrink when dried. In many cases, these packings crack during drying, critically hindering applications. However, while cracking has been widely studied for bulk gels and packings of non-shrinkable grains, little is known about how packings of shrinkable grains crack. Here, we elucidate how grain shrinkage alters cracking during drying. Using experiments with model shrinkable hydrogel beads, we show that differential shrinkage can dramatically alter crack evolution during drying-in some cases, even causing cracks to spontaneously "self-close". In other cases, packings shrink without cracking or crack irreversibly. We developed both granular and continuum models to quantify the interplay between grain shrinkage, poromechanics, packing size, drying rate, capillarity, and substrate friction on cracking. Guided by the theory, we also found that cracking can be completely altered by varying the spatial profile of drying. Our work elucidates the rich physics underlying cracking in shrinkable, granular packings, and yields new strategies for controlling crack evolution. We show that differential shrinkage can dramatically alter cracking-even enabling cracks to self-close-during drying in shrinkable, granular packings.
ISSN:1744-683X
1744-6848
DOI:10.1039/c9sm00731h