The Study of Self-Oscillations During CH4 Oxidation Over Ni by the Pulse Method: Is it Possible?

For the first time, the pulse method has been applied to the study of the self-oscillatory behaviour. For methane oxidation over Ni foil the response to a sequence of equal pulses has been strictly periodic. The pulse method allowed to obtain some new information about the origin of oscillations in...

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Bibliographic Details
Published in:Catalysis letters 2017-10, Vol.147 (10), p.2664-2673
Main Authors: Bychkov, V. Yu, Tulenin, Yu. P., Slinko, M. M., Gorenberg, A. Ya, Korchak, V. N.
Format: Article
Language:English
Subjects:
Catalysis
Chemistry
Chemistry and Materials Science
Industrial Chemistry/Chemical Engineering
Metal foils
Methane
Organometallic Chemistry
Oscillations
Oxidation
Physical Chemistry
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Summary:For the first time, the pulse method has been applied to the study of the self-oscillatory behaviour. For methane oxidation over Ni foil the response to a sequence of equal pulses has been strictly periodic. The pulse method allowed to obtain some new information about the origin of oscillations in this reaction. Graphical Abstract
ISSN:1011-372X
1572-879X
DOI:10.1007/s10562-017-2167-5