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Green one-pot preparation of carbon dots (CD)-embedded cellulose transparent film for Fe3+ indicator using ionic liquid
In this study, carbon dots (CD)-embedded film was successfully fabricated for Fe 3+ sensing via a one-pot process. The carbon dots for Fe 3+ ion detection were synthesized using the cellulose/ionic liquid solution for different treatment times. With the increase of the treatment time, the N-doped gr...
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| Published in: | Cellulose (London) 2020-05, Vol.27 (8), p.4609-4621 |
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| Main Authors: | , , , |
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| Language: | English |
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| cites | cdi_FETCH-LOGICAL-c286t-7049f10a30e39abfaed299ceb5b30522a5d7f672f5df19314a4b1b8ab8aa328c3 |
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| container_issue | 8 |
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| container_title | Cellulose (London) |
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| creator | Woo, Jeongyeon Song, Younghan Ahn, Jungbin Kim, Hyungsup |
| description | In this study, carbon dots (CD)-embedded film was successfully fabricated for Fe
3+
sensing via a one-pot process. The carbon dots for Fe
3+
ion detection were synthesized using the cellulose/ionic liquid solution for different treatment times. With the increase of the treatment time, the N-doped graphitic structure in the core and the functional groups on the surface were highly developed in the carbon dots. The properties and structures of the carbon dots were characterized using TEM, UV–Vis spectroscopy, XPS, IR, TCSPC, and PL spectroscopy. The carbon dots prepared by 12 h treatment showed a high quantum yield of 28.4%, and the superior stability for long-term storage, UV exposure, ionic strength, and pH change. The carbon dots in the film, as well as in the aqueous dispersion, revealed highly selective detection toward Fe
3+
. The CD-embedded cellulose film can be used as a Fe
3+
indicating film with good reusability, outstanding transparency, and high photostability.
Graphic abstract |
| doi_str_mv | 10.1007/s10570-020-03099-5 |
| format | article |
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3+
sensing via a one-pot process. The carbon dots for Fe
3+
ion detection were synthesized using the cellulose/ionic liquid solution for different treatment times. With the increase of the treatment time, the N-doped graphitic structure in the core and the functional groups on the surface were highly developed in the carbon dots. The properties and structures of the carbon dots were characterized using TEM, UV–Vis spectroscopy, XPS, IR, TCSPC, and PL spectroscopy. The carbon dots prepared by 12 h treatment showed a high quantum yield of 28.4%, and the superior stability for long-term storage, UV exposure, ionic strength, and pH change. The carbon dots in the film, as well as in the aqueous dispersion, revealed highly selective detection toward Fe
3+
. The CD-embedded cellulose film can be used as a Fe
3+
indicating film with good reusability, outstanding transparency, and high photostability.
Graphic abstract</description><identifier>ISSN: 0969-0239</identifier><identifier>EISSN: 1572-882X</identifier><identifier>DOI: 10.1007/s10570-020-03099-5</identifier><language>eng</language><publisher>Dordrecht: Springer Netherlands</publisher><subject>Bioorganic Chemistry ; Carbon ; Carbon dots ; Cellulose ; Ceramics ; Chemical synthesis ; Chemistry ; Chemistry and Materials Science ; Composites ; Ferric ions ; Functional groups ; Glass ; Graphitic structure ; Infrared spectroscopy ; Ionic liquids ; Ions ; Natural Materials ; Organic Chemistry ; Original Research ; Physical Chemistry ; Polymer Sciences ; Spectrum analysis ; Sustainable Development</subject><ispartof>Cellulose (London), 2020-05, Vol.27 (8), p.4609-4621</ispartof><rights>Springer Nature B.V. 2020</rights><rights>Springer Nature B.V. 2020.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c286t-7049f10a30e39abfaed299ceb5b30522a5d7f672f5df19314a4b1b8ab8aa328c3</citedby><cites>FETCH-LOGICAL-c286t-7049f10a30e39abfaed299ceb5b30522a5d7f672f5df19314a4b1b8ab8aa328c3</cites><orcidid>0000-0002-9326-9943</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,27924,27925</link.rule.ids></links><search><creatorcontrib>Woo, Jeongyeon</creatorcontrib><creatorcontrib>Song, Younghan</creatorcontrib><creatorcontrib>Ahn, Jungbin</creatorcontrib><creatorcontrib>Kim, Hyungsup</creatorcontrib><title>Green one-pot preparation of carbon dots (CD)-embedded cellulose transparent film for Fe3+ indicator using ionic liquid</title><title>Cellulose (London)</title><addtitle>Cellulose</addtitle><description>In this study, carbon dots (CD)-embedded film was successfully fabricated for Fe
3+
sensing via a one-pot process. The carbon dots for Fe
3+
ion detection were synthesized using the cellulose/ionic liquid solution for different treatment times. With the increase of the treatment time, the N-doped graphitic structure in the core and the functional groups on the surface were highly developed in the carbon dots. The properties and structures of the carbon dots were characterized using TEM, UV–Vis spectroscopy, XPS, IR, TCSPC, and PL spectroscopy. The carbon dots prepared by 12 h treatment showed a high quantum yield of 28.4%, and the superior stability for long-term storage, UV exposure, ionic strength, and pH change. The carbon dots in the film, as well as in the aqueous dispersion, revealed highly selective detection toward Fe
3+
. The CD-embedded cellulose film can be used as a Fe
3+
indicating film with good reusability, outstanding transparency, and high photostability.
Graphic abstract</description><subject>Bioorganic Chemistry</subject><subject>Carbon</subject><subject>Carbon dots</subject><subject>Cellulose</subject><subject>Ceramics</subject><subject>Chemical synthesis</subject><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Composites</subject><subject>Ferric ions</subject><subject>Functional groups</subject><subject>Glass</subject><subject>Graphitic structure</subject><subject>Infrared spectroscopy</subject><subject>Ionic liquids</subject><subject>Ions</subject><subject>Natural Materials</subject><subject>Organic Chemistry</subject><subject>Original Research</subject><subject>Physical Chemistry</subject><subject>Polymer Sciences</subject><subject>Spectrum analysis</subject><subject>Sustainable Development</subject><issn>0969-0239</issn><issn>1572-882X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2020</creationdate><recordtype>article</recordtype><recordid>eNp9kE9LxDAQxYMouK5-AU8BL4pU86dpm6OsrgoLXhS8hbSZLFm6TTdJEb-90RW8CTNMMnnvBX4InVNyQwmpbyMloiYFYbk5kbIQB2hGRc2KpmHvh2hGZCXzM5fH6CTGDSFE1ozO0MdjABiwH6AYfcJjgFEHnZzPO4s7Hdp8Mj5FfLm4vypg24IxYHAHfT_1PgJOQQ8xm2BI2Lp-i60PeAn8GrvBuE6nfJ2iG9Y4h7oO9243OXOKjqzuI5z9zjl6Wz68Lp6K1cvj8-JuVXSsqVJRk1JaSjQnwKVurQbDpOygFS0ngjEtTG2rmllhLJWclrpsadvoXJqzpuNzdLHPHYPfTRCT2vgpDPlLlWGUZSNF1WQV26u64GMMYNUY3FaHT0WJ-gas9oBVBqx-ACuRTXxvilk8rCH8Rf_j-gIil38i</recordid><startdate>20200501</startdate><enddate>20200501</enddate><creator>Woo, Jeongyeon</creator><creator>Song, Younghan</creator><creator>Ahn, Jungbin</creator><creator>Kim, Hyungsup</creator><general>Springer Netherlands</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>AFKRA</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>HCIFZ</scope><scope>KB.</scope><scope>PDBOC</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><orcidid>https://orcid.org/0000-0002-9326-9943</orcidid></search><sort><creationdate>20200501</creationdate><title>Green one-pot preparation of carbon dots (CD)-embedded cellulose transparent film for Fe3+ indicator using ionic liquid</title><author>Woo, Jeongyeon ; Song, Younghan ; Ahn, Jungbin ; Kim, Hyungsup</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c286t-7049f10a30e39abfaed299ceb5b30522a5d7f672f5df19314a4b1b8ab8aa328c3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2020</creationdate><topic>Bioorganic Chemistry</topic><topic>Carbon</topic><topic>Carbon dots</topic><topic>Cellulose</topic><topic>Ceramics</topic><topic>Chemical synthesis</topic><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Composites</topic><topic>Ferric ions</topic><topic>Functional groups</topic><topic>Glass</topic><topic>Graphitic structure</topic><topic>Infrared spectroscopy</topic><topic>Ionic liquids</topic><topic>Ions</topic><topic>Natural Materials</topic><topic>Organic Chemistry</topic><topic>Original Research</topic><topic>Physical Chemistry</topic><topic>Polymer Sciences</topic><topic>Spectrum analysis</topic><topic>Sustainable Development</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Woo, Jeongyeon</creatorcontrib><creatorcontrib>Song, Younghan</creatorcontrib><creatorcontrib>Ahn, Jungbin</creatorcontrib><creatorcontrib>Kim, Hyungsup</creatorcontrib><collection>CrossRef</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central</collection><collection>AUTh Library subscriptions: ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Materials Science Collection</collection><collection>ProQuest Central</collection><collection>SciTech Premium Collection</collection><collection>Materials Science Database</collection><collection>Materials science collection</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><jtitle>Cellulose (London)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Woo, Jeongyeon</au><au>Song, Younghan</au><au>Ahn, Jungbin</au><au>Kim, Hyungsup</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Green one-pot preparation of carbon dots (CD)-embedded cellulose transparent film for Fe3+ indicator using ionic liquid</atitle><jtitle>Cellulose (London)</jtitle><stitle>Cellulose</stitle><date>2020-05-01</date><risdate>2020</risdate><volume>27</volume><issue>8</issue><spage>4609</spage><epage>4621</epage><pages>4609-4621</pages><issn>0969-0239</issn><eissn>1572-882X</eissn><abstract>In this study, carbon dots (CD)-embedded film was successfully fabricated for Fe
3+
sensing via a one-pot process. The carbon dots for Fe
3+
ion detection were synthesized using the cellulose/ionic liquid solution for different treatment times. With the increase of the treatment time, the N-doped graphitic structure in the core and the functional groups on the surface were highly developed in the carbon dots. The properties and structures of the carbon dots were characterized using TEM, UV–Vis spectroscopy, XPS, IR, TCSPC, and PL spectroscopy. The carbon dots prepared by 12 h treatment showed a high quantum yield of 28.4%, and the superior stability for long-term storage, UV exposure, ionic strength, and pH change. The carbon dots in the film, as well as in the aqueous dispersion, revealed highly selective detection toward Fe
3+
. The CD-embedded cellulose film can be used as a Fe
3+
indicating film with good reusability, outstanding transparency, and high photostability.
Graphic abstract</abstract><cop>Dordrecht</cop><pub>Springer Netherlands</pub><doi>10.1007/s10570-020-03099-5</doi><tpages>13</tpages><orcidid>https://orcid.org/0000-0002-9326-9943</orcidid></addata></record> |
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| ispartof | Cellulose (London), 2020-05, Vol.27 (8), p.4609-4621 |
| issn | 0969-0239 1572-882X |
| language | eng |
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| source | Springer Nature |
| subjects | Bioorganic Chemistry Carbon Carbon dots Cellulose Ceramics Chemical synthesis Chemistry Chemistry and Materials Science Composites Ferric ions Functional groups Glass Graphitic structure Infrared spectroscopy Ionic liquids Ions Natural Materials Organic Chemistry Original Research Physical Chemistry Polymer Sciences Spectrum analysis Sustainable Development |
| title | Green one-pot preparation of carbon dots (CD)-embedded cellulose transparent film for Fe3+ indicator using ionic liquid |
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