Characterizing and Quantifying African Dust Transport and Deposition to South America: Implications for the Phosphorus Budget in the Amazon Basin

• Published in: Global biogeochemical cycles 2020-09, Vol.34 (9), p.n/a
• Main Authors: Prospero, Joseph M., Barkley, Anne E., Gaston, Cassandra J., Gatineau, Alexandre, Campos y Sansano, Arthur, Panechou, Kathy
• Format: Article
• Language: English
• Subjects: Aerosol measurements; Aerosol transport; Aerosols; Amazon Basin; Atmospheric particulates; Biomass; Biomass burning; Burning; Carbon cycle; Carbon dioxide; Carbon dioxide atmospheric concentrations; Chemical transport; Climate change; Deposition; Dust; Dust storms; Dust transport; Estimates; Fertility; Global warming; Heart; mineral dust; Mineral nutrients; Nutrient loss; Nutrients; Offsets; Particulate matter; Phosphorus; Physical properties; PM10; Precipitation chemistry; Questions; Rain; Rainfall; Rainfall-climatic change relationships; River basins; Soil; Soil erosion; Soil fertility; Soil loss; Soil nutrients; Soils; South America; Trade winds; Transport; Tropical climate; Weathering
• ISSN: 0886-6236; 1944-9224
• DOI: 10.1029/2020GB006536

Soils in the Amazon Basin are deficient in phosphorus, essential to soil fertility. Previous studies suggested that African mineral dust deposited to Amazonian soils served as an important source of phosphorus that enhances soil fertility. These studies lacked the quantitative measurements essential to validate estimates. Here we present daily measurements of mineral dust and PM10 carried in the trade winds at Cayenne, French Guiana, during 2002–2017. MERRA‐2 model dust concentrations showed excellent agreement with measurements over this period. Consequently, we used MERRA‐2 to estimate temporal and spatial deposition rates to Amazonia. Our annual deposition rate, 8–10 Tg dust, is substantially lower than previous estimates. Deposition rates are greatest over the northern and northeastern regions of South America. In contrast, rates are low in central Amazonia. Our results raise questions about the impact of African dust on soil fertility in Amazonia. However, African aerosol transport carries other aerosol species that could play a role in soil fertility, including biomass‐burning products known to contain substantial concentrations of phosphorus. Our study highlights the need for more measurements of aerosol and precipitation chemistry over wider expanses of South America in order to better characterize aerosol chemical and physical properties, to identify aerosol sources, and to constrain model estimates. We show that over 2002–2017 dust transport to South America was negatively correlated to rainfall over the Sahel in North Africa. Long‐term monitoring is needed to capture changes in transport from Africa that might occur as a result of climate change. Plain Language Summary The Amazon Basin plays a major role in climate by removing huge quantities of carbon dioxide (CO2) from the atmosphere and storing the carbon in vegetation. This removal partially offsets the impact of CO2 emitted by humans and the consequent rate of global warming. There is a concern about decreasing soil fertility in the Amazon Basin because of the loss of phosphorus, an essential plant nutrient, due to intense tropical weathering and biomass burning. Previous work suggested that large quantities of dust are transported from Africa to South America every year and deposited to the Amazon. Dust contains phosphorus and other nutrients that could mitigate soil losses and increase Amazonian soil fertility. However, estimates of the amount of dust carried to the Amazon are uncertain b