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An integrated quantum material testbed with multi-resolution photoemission spectroscopy
We present the development of a multi-resolution photoemission spectroscopy (MRPES) setup, which probes quantum materials in energy, momentum, space, and time. This versatile setup integrates three light sources in one photoemission setup and can conveniently switch between traditional angle-resolve...
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Published in: | Review of scientific instruments 2021-11, Vol.92 (11), p.113907-113907 |
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container_title | Review of scientific instruments |
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creator | Yan, Chenhui Green, Emanuel Fukumori, Riku Protic, Nikola Lee, Seng Huat Fernandez-Mulligan, Sebastian Raja, Rahim Erdakos, Robin Mao, Zhiqiang Yang, Shuolong |
description | We present the development of a multi-resolution photoemission spectroscopy (MRPES) setup, which probes quantum materials in energy, momentum, space, and time. This versatile setup integrates three light sources in one photoemission setup and can conveniently switch between traditional angle-resolved photoemission spectroscopy (ARPES), time-resolved ARPES (trARPES), and micrometer-scale spatially resolved ARPES. It provides a first-time all-in-one solution to achieve an energy resolution of |
doi_str_mv | 10.1063/5.0072979 |
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This versatile setup integrates three light sources in one photoemission setup and can conveniently switch between traditional angle-resolved photoemission spectroscopy (ARPES), time-resolved ARPES (trARPES), and micrometer-scale spatially resolved ARPES. It provides a first-time all-in-one solution to achieve an energy resolution of <4 meV, a time resolution of <35 fs, and a spatial resolution of ∼10 μm in photoemission spectroscopy. Remarkably, we obtain the shortest time resolution among the trARPES setups using solid-state nonlinear crystals for frequency upconversion. Furthermore, this MRPES setup is integrated with a shadow-mask assisted molecular beam epitaxy system, which transforms the traditional photoemission spectroscopy into a quantum device characterization instrument. 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We demonstrate the functionalities of this novel quantum material testbed using FeSe/SrTiO3 thin films and MnBi4Te7 magnetic topological insulators.</description><subject>Energy resolution</subject><subject>Light sources</subject><subject>Molecular beam epitaxy</subject><subject>Photoelectric emission</subject><subject>Photoelectron spectroscopy</subject><subject>Scientific apparatus & instruments</subject><subject>Shadow masks</subject><subject>Spatial resolution</subject><subject>Spectrum analysis</subject><subject>Strontium titanates</subject><subject>Thin films</subject><subject>Topological insulators</subject><issn>0034-6748</issn><issn>1089-7623</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2021</creationdate><recordtype>article</recordtype><recordid>eNqdkF1LwzAUhoMoOKcX_oOCNyp0niZt2lyO4RcMvFG8DEl75jLapktSZf_ejAmClx4Ih5c8hDcPIZcZzDLg7K6YAZRUlOKITDKoRFpyyo7JBIDlKS_z6pSceb-BOEWWTcj7vE9MH_DDqYBNsh1VH8Yu6WJyRrVJQB90vPgyYZ10YxtM6tDbdgzG9smwtsFiZ7zfJz9gHZz1tR125-RkpVqPFz97St4e7l8XT-ny5fF5MV-mNeMQUs1AN0IoqDgVQLUuG8HyUkOuKqoxb3SGGjQthUJeaYac5nnTMNQrUesC2JRcH94dnN2OsayMbWpsW9WjHb2kHAoOECVE9OoPurGj62M7SQtRRDfxROrmQNXxJ97hSg7OdMrtZAZyr1gW8kdxZG8PrK9NUHsj_4M_rfsF5dCs2DdHZouV</recordid><startdate>20211101</startdate><enddate>20211101</enddate><creator>Yan, Chenhui</creator><creator>Green, Emanuel</creator><creator>Fukumori, Riku</creator><creator>Protic, Nikola</creator><creator>Lee, Seng Huat</creator><creator>Fernandez-Mulligan, Sebastian</creator><creator>Raja, Rahim</creator><creator>Erdakos, Robin</creator><creator>Mao, Zhiqiang</creator><creator>Yang, Shuolong</creator><general>American Institute of Physics</general><scope>AAYXX</scope><scope>CITATION</scope><scope>8FD</scope><scope>H8D</scope><scope>L7M</scope><scope>7X8</scope><orcidid>https://orcid.org/0000-0002-0005-8304</orcidid><orcidid>https://orcid.org/0000-0002-4920-3293</orcidid><orcidid>https://orcid.org/0000-0002-8200-9898</orcidid><orcidid>https://orcid.org/0000-0003-0896-4261</orcidid></search><sort><creationdate>20211101</creationdate><title>An integrated quantum material testbed with multi-resolution photoemission spectroscopy</title><author>Yan, Chenhui ; Green, Emanuel ; Fukumori, Riku ; Protic, Nikola ; Lee, Seng Huat ; Fernandez-Mulligan, Sebastian ; Raja, Rahim ; Erdakos, Robin ; Mao, Zhiqiang ; Yang, Shuolong</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c360t-b30bd99a0862902bb7d9347b04a82be4db1eb0b279ae68b3e6244dd3ebf9cb503</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2021</creationdate><topic>Energy resolution</topic><topic>Light sources</topic><topic>Molecular beam epitaxy</topic><topic>Photoelectric emission</topic><topic>Photoelectron spectroscopy</topic><topic>Scientific apparatus & instruments</topic><topic>Shadow masks</topic><topic>Spatial resolution</topic><topic>Spectrum analysis</topic><topic>Strontium titanates</topic><topic>Thin films</topic><topic>Topological insulators</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Yan, Chenhui</creatorcontrib><creatorcontrib>Green, Emanuel</creatorcontrib><creatorcontrib>Fukumori, Riku</creatorcontrib><creatorcontrib>Protic, Nikola</creatorcontrib><creatorcontrib>Lee, Seng Huat</creatorcontrib><creatorcontrib>Fernandez-Mulligan, Sebastian</creatorcontrib><creatorcontrib>Raja, Rahim</creatorcontrib><creatorcontrib>Erdakos, Robin</creatorcontrib><creatorcontrib>Mao, Zhiqiang</creatorcontrib><creatorcontrib>Yang, Shuolong</creatorcontrib><collection>CrossRef</collection><collection>Technology Research Database</collection><collection>Aerospace Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>MEDLINE - Academic</collection><jtitle>Review of scientific instruments</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Yan, Chenhui</au><au>Green, Emanuel</au><au>Fukumori, Riku</au><au>Protic, Nikola</au><au>Lee, Seng Huat</au><au>Fernandez-Mulligan, Sebastian</au><au>Raja, Rahim</au><au>Erdakos, Robin</au><au>Mao, Zhiqiang</au><au>Yang, Shuolong</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>An integrated quantum material testbed with multi-resolution photoemission spectroscopy</atitle><jtitle>Review of scientific instruments</jtitle><date>2021-11-01</date><risdate>2021</risdate><volume>92</volume><issue>11</issue><spage>113907</spage><epage>113907</epage><pages>113907-113907</pages><issn>0034-6748</issn><eissn>1089-7623</eissn><coden>RSINAK</coden><abstract>We present the development of a multi-resolution photoemission spectroscopy (MRPES) setup, which probes quantum materials in energy, momentum, space, and time. This versatile setup integrates three light sources in one photoemission setup and can conveniently switch between traditional angle-resolved photoemission spectroscopy (ARPES), time-resolved ARPES (trARPES), and micrometer-scale spatially resolved ARPES. It provides a first-time all-in-one solution to achieve an energy resolution of <4 meV, a time resolution of <35 fs, and a spatial resolution of ∼10 μm in photoemission spectroscopy. Remarkably, we obtain the shortest time resolution among the trARPES setups using solid-state nonlinear crystals for frequency upconversion. Furthermore, this MRPES setup is integrated with a shadow-mask assisted molecular beam epitaxy system, which transforms the traditional photoemission spectroscopy into a quantum device characterization instrument. We demonstrate the functionalities of this novel quantum material testbed using FeSe/SrTiO3 thin films and MnBi4Te7 magnetic topological insulators.</abstract><cop>Melville</cop><pub>American Institute of Physics</pub><doi>10.1063/5.0072979</doi><tpages>8</tpages><orcidid>https://orcid.org/0000-0002-0005-8304</orcidid><orcidid>https://orcid.org/0000-0002-4920-3293</orcidid><orcidid>https://orcid.org/0000-0002-8200-9898</orcidid><orcidid>https://orcid.org/0000-0003-0896-4261</orcidid></addata></record> |
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subjects | Energy resolution Light sources Molecular beam epitaxy Photoelectric emission Photoelectron spectroscopy Scientific apparatus & instruments Shadow masks Spatial resolution Spectrum analysis Strontium titanates Thin films Topological insulators |
title | An integrated quantum material testbed with multi-resolution photoemission spectroscopy |
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