Loading…

Quantum yield of an emitter proximate to nanostructures: a quantitative understanding

Exciton-surface plasmon coupling is at the heart of the most elementary light-matter interactions and is a result of not only an intrinsic property of the emitter but that of emitter-environment interaction. Thus, change of electromagnetic environment, as in case of metallic nanoplasmonic structures...

Full description

Saved in:
Bibliographic Details
Published in:arXiv.org 2022-03
Main Author: Duan, J S
Format: Article
Language:English
Subjects:
Online Access:Get full text
Tags: Add Tag
No Tags, Be the first to tag this record!
cited_by
cites
container_end_page
container_issue
container_start_page
container_title arXiv.org
container_volume
creator Duan, J S
description Exciton-surface plasmon coupling is at the heart of the most elementary light-matter interactions and is a result of not only an intrinsic property of the emitter but that of emitter-environment interaction. Thus, change of electromagnetic environment, as in case of metallic nanoplasmonic structures and an emitter, significantly modifies the near field light-matter interaction, which leads to energy transfer in the form of exciton between metallic nanostructure and the emitter. However, this mechanism remains largely unexplored. Here, we developed and applied semi-classical electrodynamics theory and modeling techniques to analyze the energy transfer mechanism in exciton-surface plasmon coupling. The quantum efficiency of an emitter was investigated as a function of the location of the emitter with respect to nanoparticles and their assembles whose local plasmonic field modified by forming complex coupling modes as well as the local dielectric environment. The research provided a theoretical insight into fundamental science of nanophotonics and shed light on unprecedented applications in wide range fields such as ultra-low power lasers, quantum information processing, photovoltaics, photocatalysis, and chemical sensing.
format article
fullrecord <record><control><sourceid>proquest</sourceid><recordid>TN_cdi_proquest_journals_2638170454</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2638170454</sourcerecordid><originalsourceid>FETCH-proquest_journals_26381704543</originalsourceid><addsrcrecordid>eNqNjMsKwjAQRYMgWLT_MOC60CZ94VYUt4Kuy2CnktImNpmI_r0V_ABXd3HOuQsRSaWypM6lXInY-z5NU1lWsihUJK7ngIbDCG9NQwu2AzRAo2YmBw9nX3pEJmALBo317MKNgyO_A4Tpm2pG1k-CYFpyntG02tw3Ytnh4Cn-7Vpsj4fL_pTMj1Mgz01vgzMzamSp6qxK8yJX_1kfU1xCBg</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2638170454</pqid></control><display><type>article</type><title>Quantum yield of an emitter proximate to nanostructures: a quantitative understanding</title><source>ProQuest Publicly Available Content database</source><creator>Duan, J S</creator><creatorcontrib>Duan, J S</creatorcontrib><description>Exciton-surface plasmon coupling is at the heart of the most elementary light-matter interactions and is a result of not only an intrinsic property of the emitter but that of emitter-environment interaction. Thus, change of electromagnetic environment, as in case of metallic nanoplasmonic structures and an emitter, significantly modifies the near field light-matter interaction, which leads to energy transfer in the form of exciton between metallic nanostructure and the emitter. However, this mechanism remains largely unexplored. Here, we developed and applied semi-classical electrodynamics theory and modeling techniques to analyze the energy transfer mechanism in exciton-surface plasmon coupling. The quantum efficiency of an emitter was investigated as a function of the location of the emitter with respect to nanoparticles and their assembles whose local plasmonic field modified by forming complex coupling modes as well as the local dielectric environment. The research provided a theoretical insight into fundamental science of nanophotonics and shed light on unprecedented applications in wide range fields such as ultra-low power lasers, quantum information processing, photovoltaics, photocatalysis, and chemical sensing.</description><identifier>EISSN: 2331-8422</identifier><language>eng</language><publisher>Ithaca: Cornell University Library, arXiv.org</publisher><subject>Coupling ; Data processing ; Electrodynamics ; Emitters ; Energy transfer ; Excitons ; Nanoparticles ; Nanostructure ; Photovoltaic cells ; Quantum efficiency ; Quantum phenomena</subject><ispartof>arXiv.org, 2022-03</ispartof><rights>2022. This work is published under http://creativecommons.org/licenses/by-nc-nd/4.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License.</rights><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://www.proquest.com/docview/2638170454?pq-origsite=primo$$EHTML$$P50$$Gproquest$$Hfree_for_read</linktohtml><link.rule.ids>780,784,25753,37012,44590</link.rule.ids></links><search><creatorcontrib>Duan, J S</creatorcontrib><title>Quantum yield of an emitter proximate to nanostructures: a quantitative understanding</title><title>arXiv.org</title><description>Exciton-surface plasmon coupling is at the heart of the most elementary light-matter interactions and is a result of not only an intrinsic property of the emitter but that of emitter-environment interaction. Thus, change of electromagnetic environment, as in case of metallic nanoplasmonic structures and an emitter, significantly modifies the near field light-matter interaction, which leads to energy transfer in the form of exciton between metallic nanostructure and the emitter. However, this mechanism remains largely unexplored. Here, we developed and applied semi-classical electrodynamics theory and modeling techniques to analyze the energy transfer mechanism in exciton-surface plasmon coupling. The quantum efficiency of an emitter was investigated as a function of the location of the emitter with respect to nanoparticles and their assembles whose local plasmonic field modified by forming complex coupling modes as well as the local dielectric environment. The research provided a theoretical insight into fundamental science of nanophotonics and shed light on unprecedented applications in wide range fields such as ultra-low power lasers, quantum information processing, photovoltaics, photocatalysis, and chemical sensing.</description><subject>Coupling</subject><subject>Data processing</subject><subject>Electrodynamics</subject><subject>Emitters</subject><subject>Energy transfer</subject><subject>Excitons</subject><subject>Nanoparticles</subject><subject>Nanostructure</subject><subject>Photovoltaic cells</subject><subject>Quantum efficiency</subject><subject>Quantum phenomena</subject><issn>2331-8422</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2022</creationdate><recordtype>article</recordtype><sourceid>PIMPY</sourceid><recordid>eNqNjMsKwjAQRYMgWLT_MOC60CZ94VYUt4Kuy2CnktImNpmI_r0V_ABXd3HOuQsRSaWypM6lXInY-z5NU1lWsihUJK7ngIbDCG9NQwu2AzRAo2YmBw9nX3pEJmALBo317MKNgyO_A4Tpm2pG1k-CYFpyntG02tw3Ytnh4Cn-7Vpsj4fL_pTMj1Mgz01vgzMzamSp6qxK8yJX_1kfU1xCBg</recordid><startdate>20220310</startdate><enddate>20220310</enddate><creator>Duan, J S</creator><general>Cornell University Library, arXiv.org</general><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>ABUWG</scope><scope>AFKRA</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>DWQXO</scope><scope>HCIFZ</scope><scope>L6V</scope><scope>M7S</scope><scope>PIMPY</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PRINS</scope><scope>PTHSS</scope></search><sort><creationdate>20220310</creationdate><title>Quantum yield of an emitter proximate to nanostructures: a quantitative understanding</title><author>Duan, J S</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-proquest_journals_26381704543</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2022</creationdate><topic>Coupling</topic><topic>Data processing</topic><topic>Electrodynamics</topic><topic>Emitters</topic><topic>Energy transfer</topic><topic>Excitons</topic><topic>Nanoparticles</topic><topic>Nanostructure</topic><topic>Photovoltaic cells</topic><topic>Quantum efficiency</topic><topic>Quantum phenomena</topic><toplevel>online_resources</toplevel><creatorcontrib>Duan, J S</creatorcontrib><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Materials Science &amp; Engineering Collection</collection><collection>ProQuest Central (Alumni)</collection><collection>ProQuest Central</collection><collection>ProQuest Central Essentials</collection><collection>AUTh Library subscriptions: ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Central</collection><collection>SciTech Premium Collection</collection><collection>ProQuest Engineering Collection</collection><collection>Engineering Database</collection><collection>ProQuest Publicly Available Content database</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>ProQuest Central China</collection><collection>Engineering collection</collection></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Duan, J S</au><format>book</format><genre>document</genre><ristype>GEN</ristype><atitle>Quantum yield of an emitter proximate to nanostructures: a quantitative understanding</atitle><jtitle>arXiv.org</jtitle><date>2022-03-10</date><risdate>2022</risdate><eissn>2331-8422</eissn><abstract>Exciton-surface plasmon coupling is at the heart of the most elementary light-matter interactions and is a result of not only an intrinsic property of the emitter but that of emitter-environment interaction. Thus, change of electromagnetic environment, as in case of metallic nanoplasmonic structures and an emitter, significantly modifies the near field light-matter interaction, which leads to energy transfer in the form of exciton between metallic nanostructure and the emitter. However, this mechanism remains largely unexplored. Here, we developed and applied semi-classical electrodynamics theory and modeling techniques to analyze the energy transfer mechanism in exciton-surface plasmon coupling. The quantum efficiency of an emitter was investigated as a function of the location of the emitter with respect to nanoparticles and their assembles whose local plasmonic field modified by forming complex coupling modes as well as the local dielectric environment. The research provided a theoretical insight into fundamental science of nanophotonics and shed light on unprecedented applications in wide range fields such as ultra-low power lasers, quantum information processing, photovoltaics, photocatalysis, and chemical sensing.</abstract><cop>Ithaca</cop><pub>Cornell University Library, arXiv.org</pub><oa>free_for_read</oa></addata></record>
fulltext fulltext
identifier EISSN: 2331-8422
ispartof arXiv.org, 2022-03
issn 2331-8422
language eng
recordid cdi_proquest_journals_2638170454
source ProQuest Publicly Available Content database
subjects Coupling
Data processing
Electrodynamics
Emitters
Energy transfer
Excitons
Nanoparticles
Nanostructure
Photovoltaic cells
Quantum efficiency
Quantum phenomena
title Quantum yield of an emitter proximate to nanostructures: a quantitative understanding
url http://sfxeu10.hosted.exlibrisgroup.com/loughborough?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2024-12-24T18%3A20%3A21IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest&rft_val_fmt=info:ofi/fmt:kev:mtx:book&rft.genre=document&rft.atitle=Quantum%20yield%20of%20an%20emitter%20proximate%20to%20nanostructures:%20a%20quantitative%20understanding&rft.jtitle=arXiv.org&rft.au=Duan,%20J%20S&rft.date=2022-03-10&rft.eissn=2331-8422&rft_id=info:doi/&rft_dat=%3Cproquest%3E2638170454%3C/proquest%3E%3Cgrp_id%3Ecdi_FETCH-proquest_journals_26381704543%3C/grp_id%3E%3Coa%3E%3C/oa%3E%3Curl%3E%3C/url%3E&rft_id=info:oai/&rft_pqid=2638170454&rft_id=info:pmid/&rfr_iscdi=true