Synthesis, Structure and Properties of Donor-acceptor-type [4]Dendralenes

[4]Dendralene and its analogs possessing both strongly electron-donating 1,3-dithiol-2-ylidenes and electron-accepting dicyanomethylidenes (2b–4b) were successfully synthesized. X-ray structure analysis revealed that 2b adopts a nonplanar structure, in which half units of 2b are significantly inclin...

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Published in:Chemistry letters 2022-05, Vol.51 (5), p.581-584
Main Authors: Matsumoto, Yuya, Matsuda, Rina, Yoshimura, Aya, Shirahata, Takashi, Misaki, Yohji
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Language:English
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Electrons
Oxidation
Structural analysis
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Matsuda, Rina
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Misaki, Yohji
description [4]Dendralene and its analogs possessing both strongly electron-donating 1,3-dithiol-2-ylidenes and electron-accepting dicyanomethylidenes (2b–4b) were successfully synthesized. X-ray structure analysis revealed that 2b adopts a nonplanar structure, in which half units of 2b are significantly inclined to each other. Cyclic voltammograms of 2b–4b consisted of one pair of two-electron oxidation waves and one pair of one-electron reduction waves.
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subjects Electrons
Oxidation
Structural analysis
title Synthesis, Structure and Properties of Donor-acceptor-type [4]Dendralenes
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