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The first polyoxoniobate-templated silver cluster with temperature-dependent luminescent emission
The compound [(Nb 6 O 19 )@Ag 34 ( t BuC&z.tbd;C) 24 (CH 3 COO) 2 ] (Ag 34 ) was synthesized using the solvothermal method combined with volatilization. This was the first case, to the best of our knowledge, of isolating a silver cluster containing a polyoxoniobate (PONb) template. The luminesce...
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| Published in: | Chemical communications (Cambridge, England) England), 2023-03, Vol.59 (2), p.2927-293 |
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| Main Authors: | , , , |
| Format: | Article |
| Language: | English |
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| cited_by | cdi_FETCH-LOGICAL-c337t-be6e90c2e272391d815d674e94fef76115af8282195c1905a57317e5f87e35ec3 |
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| cites | cdi_FETCH-LOGICAL-c337t-be6e90c2e272391d815d674e94fef76115af8282195c1905a57317e5f87e35ec3 |
| container_end_page | 293 |
| container_issue | 2 |
| container_start_page | 2927 |
| container_title | Chemical communications (Cambridge, England) |
| container_volume | 59 |
| creator | Biao Wu Li, Xin-Xiong Zheng, Shou-Tian Xie, Jianping |
| description | The compound [(Nb
6
O
19
)@Ag
34
(
t
BuC&z.tbd;C)
24
(CH
3
COO)
2
] (Ag
34
) was synthesized using the solvothermal method combined with volatilization. This was the first case, to the best of our knowledge, of isolating a silver cluster containing a polyoxoniobate (PONb) template. The luminescence, solution behavior and solid-state stability of Ag
34
were studied in detail. Electrospray ionization mass spectrometry indicated that Ag
34
can maintain the integrity of its skeleton in solution. Detection of temperature could be a potential application of its unique luminescent behavior. We expect this work to inspire further fabrications of PONb-templated high-nuclearity silver clusters.
A polyoxoniobate-templated silver nanocluster was first obtained. The compound not only shows good chemical stability but also exhibits interesting temperature-dependent luminescent emission. |
| doi_str_mv | 10.1039/d3cc00128h |
| format | article |
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6
O
19
)@Ag
34
(
t
BuC&z.tbd;C)
24
(CH
3
COO)
2
] (Ag
34
) was synthesized using the solvothermal method combined with volatilization. This was the first case, to the best of our knowledge, of isolating a silver cluster containing a polyoxoniobate (PONb) template. The luminescence, solution behavior and solid-state stability of Ag
34
were studied in detail. Electrospray ionization mass spectrometry indicated that Ag
34
can maintain the integrity of its skeleton in solution. Detection of temperature could be a potential application of its unique luminescent behavior. We expect this work to inspire further fabrications of PONb-templated high-nuclearity silver clusters.
A polyoxoniobate-templated silver nanocluster was first obtained. The compound not only shows good chemical stability but also exhibits interesting temperature-dependent luminescent emission.</description><identifier>ISSN: 1359-7345</identifier><identifier>EISSN: 1364-548X</identifier><identifier>DOI: 10.1039/d3cc00128h</identifier><identifier>PMID: 36799226</identifier><language>eng</language><publisher>England: Royal Society of Chemistry</publisher><subject>Clusters ; Mass spectrometry ; Temperature dependence</subject><ispartof>Chemical communications (Cambridge, England), 2023-03, Vol.59 (2), p.2927-293</ispartof><rights>Copyright Royal Society of Chemistry 2023</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c337t-be6e90c2e272391d815d674e94fef76115af8282195c1905a57317e5f87e35ec3</citedby><cites>FETCH-LOGICAL-c337t-be6e90c2e272391d815d674e94fef76115af8282195c1905a57317e5f87e35ec3</cites><orcidid>0000-0002-3254-5799 ; 0000-0002-9903-2699 ; 0000-0002-3365-9747</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,27922,27923</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/36799226$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Biao Wu</creatorcontrib><creatorcontrib>Li, Xin-Xiong</creatorcontrib><creatorcontrib>Zheng, Shou-Tian</creatorcontrib><creatorcontrib>Xie, Jianping</creatorcontrib><title>The first polyoxoniobate-templated silver cluster with temperature-dependent luminescent emission</title><title>Chemical communications (Cambridge, England)</title><addtitle>Chem Commun (Camb)</addtitle><description>The compound [(Nb
6
O
19
)@Ag
34
(
t
BuC&z.tbd;C)
24
(CH
3
COO)
2
] (Ag
34
) was synthesized using the solvothermal method combined with volatilization. This was the first case, to the best of our knowledge, of isolating a silver cluster containing a polyoxoniobate (PONb) template. The luminescence, solution behavior and solid-state stability of Ag
34
were studied in detail. Electrospray ionization mass spectrometry indicated that Ag
34
can maintain the integrity of its skeleton in solution. Detection of temperature could be a potential application of its unique luminescent behavior. We expect this work to inspire further fabrications of PONb-templated high-nuclearity silver clusters.
A polyoxoniobate-templated silver nanocluster was first obtained. The compound not only shows good chemical stability but also exhibits interesting temperature-dependent luminescent emission.</description><subject>Clusters</subject><subject>Mass spectrometry</subject><subject>Temperature dependence</subject><issn>1359-7345</issn><issn>1364-548X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><recordid>eNpdkc1Lw0AQxRdRrFYv3pWAFxGi-5HN7h6lflQoeKngLaSbCU1JsnF3o_a_d2NrBecyD-bH4_EGoTOCbwhm6rZgWmNMqFzuoSPC0iTmiXzbHzRXsWAJH6Fj51Y4DOHyEI1YKpSiND1C-XwJUVlZ56PO1GvzZdrKLHIPsYemq4MoIlfVH2AjXffOh_1Z-WU0XMHmvrcQF9BBW0Dro7pvqhacHjQ0lXOVaU_QQZnXDk63e4xeHx_mk2k8e3l6ntzNYs2Y8PECUlBYU6CCMkUKSXiRigRUUkIpUkJ4XkoqKVFcE4V5zgUjAngpBTAOmo3R1ca3s-a9B-ezEEBDXectmN5lVMiEyQSnKqCX_9CV6W0b0g0U41ISRgN1vaG0Nc5ZKLPOVk1u1xnB2VB8ds8mk5_ipwG-2Fr2iwaKHfrbdADON4B1enf9-xz7BhlsiL4</recordid><startdate>20230307</startdate><enddate>20230307</enddate><creator>Biao Wu</creator><creator>Li, Xin-Xiong</creator><creator>Zheng, Shou-Tian</creator><creator>Xie, Jianping</creator><general>Royal Society of Chemistry</general><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>L7M</scope><scope>7X8</scope><orcidid>https://orcid.org/0000-0002-3254-5799</orcidid><orcidid>https://orcid.org/0000-0002-9903-2699</orcidid><orcidid>https://orcid.org/0000-0002-3365-9747</orcidid></search><sort><creationdate>20230307</creationdate><title>The first polyoxoniobate-templated silver cluster with temperature-dependent luminescent emission</title><author>Biao Wu ; Li, Xin-Xiong ; Zheng, Shou-Tian ; Xie, Jianping</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c337t-be6e90c2e272391d815d674e94fef76115af8282195c1905a57317e5f87e35ec3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>Clusters</topic><topic>Mass spectrometry</topic><topic>Temperature dependence</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Biao Wu</creatorcontrib><creatorcontrib>Li, Xin-Xiong</creatorcontrib><creatorcontrib>Zheng, Shou-Tian</creatorcontrib><creatorcontrib>Xie, Jianping</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>MEDLINE - Academic</collection><jtitle>Chemical communications (Cambridge, England)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Biao Wu</au><au>Li, Xin-Xiong</au><au>Zheng, Shou-Tian</au><au>Xie, Jianping</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>The first polyoxoniobate-templated silver cluster with temperature-dependent luminescent emission</atitle><jtitle>Chemical communications (Cambridge, England)</jtitle><addtitle>Chem Commun (Camb)</addtitle><date>2023-03-07</date><risdate>2023</risdate><volume>59</volume><issue>2</issue><spage>2927</spage><epage>293</epage><pages>2927-293</pages><issn>1359-7345</issn><eissn>1364-548X</eissn><abstract>The compound [(Nb
6
O
19
)@Ag
34
(
t
BuC&z.tbd;C)
24
(CH
3
COO)
2
] (Ag
34
) was synthesized using the solvothermal method combined with volatilization. This was the first case, to the best of our knowledge, of isolating a silver cluster containing a polyoxoniobate (PONb) template. The luminescence, solution behavior and solid-state stability of Ag
34
were studied in detail. Electrospray ionization mass spectrometry indicated that Ag
34
can maintain the integrity of its skeleton in solution. Detection of temperature could be a potential application of its unique luminescent behavior. We expect this work to inspire further fabrications of PONb-templated high-nuclearity silver clusters.
A polyoxoniobate-templated silver nanocluster was first obtained. The compound not only shows good chemical stability but also exhibits interesting temperature-dependent luminescent emission.</abstract><cop>England</cop><pub>Royal Society of Chemistry</pub><pmid>36799226</pmid><doi>10.1039/d3cc00128h</doi><tpages>4</tpages><orcidid>https://orcid.org/0000-0002-3254-5799</orcidid><orcidid>https://orcid.org/0000-0002-9903-2699</orcidid><orcidid>https://orcid.org/0000-0002-3365-9747</orcidid></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 1359-7345 |
| ispartof | Chemical communications (Cambridge, England), 2023-03, Vol.59 (2), p.2927-293 |
| issn | 1359-7345 1364-548X |
| language | eng |
| recordid | cdi_proquest_journals_2783588132 |
| source | Royal Society of Chemistry |
| subjects | Clusters Mass spectrometry Temperature dependence |
| title | The first polyoxoniobate-templated silver cluster with temperature-dependent luminescent emission |
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