Hybrid Transverse Magneto‐Thermoelectric Cooling in Artificially Tilted Multilayers

• Published in: Advanced energy materials 2024-01, Vol.14 (3), p.n/a
• Main Authors: Uchida, Ken‐ichi, Hirai, Takamasa, Ando, Fuyuki, Sepehri‐Amin, Hossein
• Format: Article
• Language: English
• Subjects: artificially tilted multilayers; Conductors; Ettingshausen effect; lock‐in thermography; Magnetic fields; Magnetization; magneto‐Peltier effect; Multilayers; Permanent magnets; Thermoelectric cooling; Thermography; Transport phenomena; transverse thermoelectrics
• ISSN: 1614-6832; 1614-6840
• DOI: 10.1002/aenm.202302375

In artificially tilted multilayers comprising two different conductors that are alternately and obliquely stacked, transverse thermoelectric conversion occurs, in which charge and heat currents are interconverted in the orthogonal direction. Although transverse thermoelectric conversion also occurs in homogeneous materials as an intrinsic transport phenomenon owing to the effects of magnetic fields, magnetization, and spins on conduction carriers, such magneto‐thermoelectric effects are investigated independently of thermoelectrics for artificially tilted multilayers. Here, this study shows that the synergy of these different principles improves the performance of transverse thermoelectric conversion. Using lock‐in thermography techniques, transverse thermoelectric conversion processes are visualized in artificially tilted multilayers and the experiments clarify how nonuniform charge currents are converted into orthogonal heat currents. Through the measurements of temperature change under magnetic fields, the contributions of the magneto‐thermoelectric effects are quantified in the artificially tilted multilayers and magnetically enhanced hybrid transverse thermoelectric cooling is demonstrated. By replacing one of the conductors in the multilayer with permanent magnets, the same functionality is obtained even in the absence of magnetic fields, paving the way for the creation of “thermoelectric permanent magnets” that exhibit efficient transverse thermoelectric conversion together with spontaneous magnetization. This study provides a new material design guideline for transverse thermoelectrics. To realize versatile thermal management technologies, a novel method for improving transverse thermoelectric conversion performance by utilizing magneto‐transport phenomena in artificially tilted multilayers is developed and demonstrated. This work integrates transverse thermoelectrics, spin caloritronics, and permanent magnet materials, which are studied independently, contributing to the creation of interdisciplinary materials science and device technologies that utilize heat and magnetism.