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Hyperfine Structure in the OD ESR Spectra of Recombining Charge Pairs in Doped Polyethylene Matrices
The hyperfine structure has been resolved in the optically detected electron spin resonance (OD ESR) spectra of radical ion pairs generated by ionizing radiation at a low dopant concentration in a solid polyethylene matrix at room temperature. The different organic molecules that can capture electro...
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| Published in: | Applied magnetic resonance 2018-04, Vol.49 (4), p.345-355 |
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| Main Authors: | , , , , , , |
| Format: | Article |
| Language: | English |
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| cited_by | cdi_FETCH-LOGICAL-c316t-883fd69a142937e64ba6c4bde4bd73ea1dc514c452ec351900919b1582625e353 |
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| cites | cdi_FETCH-LOGICAL-c316t-883fd69a142937e64ba6c4bde4bd73ea1dc514c452ec351900919b1582625e353 |
| container_end_page | 355 |
| container_issue | 4 |
| container_start_page | 345 |
| container_title | Applied magnetic resonance |
| container_volume | 49 |
| creator | Verkhovlyuk, V. N. Borovkov, V. I. Bagryansky, V. A. Zikirin, S. B. Taratayko, A. I. Anisimov, O. A. Molin, Yu. N. |
| description | The hyperfine structure has been resolved in the optically detected electron spin resonance (OD ESR) spectra of radical ion pairs generated by ionizing radiation at a low dopant concentration in a solid polyethylene matrix at room temperature. The different organic molecules that can capture electrons and holes were used as the dopants. The spin-lattice relaxation times
T
1
for radical ions of dopants were estimated to be tens of microseconds. The temperature dependence of OD ESR signal intensity indicates the diffusion-assisted mechanism of recombination of radical ion pairs in polyethylene. |
| doi_str_mv | 10.1007/s00723-018-0978-1 |
| format | article |
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T
1
for radical ions of dopants were estimated to be tens of microseconds. The temperature dependence of OD ESR signal intensity indicates the diffusion-assisted mechanism of recombination of radical ion pairs in polyethylene.</description><identifier>ISSN: 0937-9347</identifier><identifier>EISSN: 1613-7507</identifier><identifier>DOI: 10.1007/s00723-018-0978-1</identifier><language>eng</language><publisher>Vienna: Springer Vienna</publisher><subject>Atoms and Molecules in Strong Fields ; Charged particles ; Dopants ; Electron paramagnetic resonance ; Electron spin ; Hydrocarbons ; Hyperfine structure ; Ion pairs ; Ionizing radiation ; Laser Matter Interaction ; Magnetic fields ; Organic Chemistry ; Original Paper ; Physical Chemistry ; Physics ; Physics and Astronomy ; Polyethylene ; Polyethylenes ; Polymers ; Radiation ; Radicals ; Room temperature ; Solid State Physics ; Spectra ; Spectroscopy/Spectrometry ; Spin resonance ; Spin-lattice relaxation ; Temperature dependence ; X-rays</subject><ispartof>Applied magnetic resonance, 2018-04, Vol.49 (4), p.345-355</ispartof><rights>Springer-Verlag GmbH Austria, part of Springer Nature 2018</rights><rights>Springer-Verlag GmbH Austria, part of Springer Nature 2018.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c316t-883fd69a142937e64ba6c4bde4bd73ea1dc514c452ec351900919b1582625e353</citedby><cites>FETCH-LOGICAL-c316t-883fd69a142937e64ba6c4bde4bd73ea1dc514c452ec351900919b1582625e353</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,27923,27924</link.rule.ids></links><search><creatorcontrib>Verkhovlyuk, V. N.</creatorcontrib><creatorcontrib>Borovkov, V. I.</creatorcontrib><creatorcontrib>Bagryansky, V. A.</creatorcontrib><creatorcontrib>Zikirin, S. B.</creatorcontrib><creatorcontrib>Taratayko, A. I.</creatorcontrib><creatorcontrib>Anisimov, O. A.</creatorcontrib><creatorcontrib>Molin, Yu. N.</creatorcontrib><title>Hyperfine Structure in the OD ESR Spectra of Recombining Charge Pairs in Doped Polyethylene Matrices</title><title>Applied magnetic resonance</title><addtitle>Appl Magn Reson</addtitle><description>The hyperfine structure has been resolved in the optically detected electron spin resonance (OD ESR) spectra of radical ion pairs generated by ionizing radiation at a low dopant concentration in a solid polyethylene matrix at room temperature. The different organic molecules that can capture electrons and holes were used as the dopants. The spin-lattice relaxation times
T
1
for radical ions of dopants were estimated to be tens of microseconds. The temperature dependence of OD ESR signal intensity indicates the diffusion-assisted mechanism of recombination of radical ion pairs in polyethylene.</description><subject>Atoms and Molecules in Strong Fields</subject><subject>Charged particles</subject><subject>Dopants</subject><subject>Electron paramagnetic resonance</subject><subject>Electron spin</subject><subject>Hydrocarbons</subject><subject>Hyperfine structure</subject><subject>Ion pairs</subject><subject>Ionizing radiation</subject><subject>Laser Matter Interaction</subject><subject>Magnetic fields</subject><subject>Organic Chemistry</subject><subject>Original Paper</subject><subject>Physical Chemistry</subject><subject>Physics</subject><subject>Physics and Astronomy</subject><subject>Polyethylene</subject><subject>Polyethylenes</subject><subject>Polymers</subject><subject>Radiation</subject><subject>Radicals</subject><subject>Room temperature</subject><subject>Solid State Physics</subject><subject>Spectra</subject><subject>Spectroscopy/Spectrometry</subject><subject>Spin resonance</subject><subject>Spin-lattice relaxation</subject><subject>Temperature dependence</subject><subject>X-rays</subject><issn>0937-9347</issn><issn>1613-7507</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2018</creationdate><recordtype>article</recordtype><recordid>eNp1kDFPwzAQhS0EEqXwA9gsMQd8cRLHI2oLRQK1amG2HOfSpmqTYDtD_j2ugsTEcHfL-97dPULugT0CY-LJhRbziEEeMSnyCC7IBDLgkUiZuCQTJrmIJE_ENblx7sAYpDmICSmXQ4e2qhukW29743uLtG6o3yNdzeliu6HbDo23mrYV3aBpT0Xd1M2Ozvba7pCudW3dmZi3HZZ03R4H9PvhiMHxQ3tbG3S35KrSR4d3v3NKvl4Wn7Nl9L56fZs9v0eGQ-ajPOdVmUkNSRyuxSwpdGaSosRQgqOG0qSQmCSN0fAUJGMSZBEeibM4RZ7yKXkYfTvbfvfovDq0vW3CShVLEBK4SHhQwagytnXOYqU6W5-0HRQwdQ5TjWGqEKY6h6kgMPHIuKBtdmj_nP-HfgD_EnYZ</recordid><startdate>20180401</startdate><enddate>20180401</enddate><creator>Verkhovlyuk, V. 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N.</au><au>Borovkov, V. I.</au><au>Bagryansky, V. A.</au><au>Zikirin, S. B.</au><au>Taratayko, A. I.</au><au>Anisimov, O. A.</au><au>Molin, Yu. N.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Hyperfine Structure in the OD ESR Spectra of Recombining Charge Pairs in Doped Polyethylene Matrices</atitle><jtitle>Applied magnetic resonance</jtitle><stitle>Appl Magn Reson</stitle><date>2018-04-01</date><risdate>2018</risdate><volume>49</volume><issue>4</issue><spage>345</spage><epage>355</epage><pages>345-355</pages><issn>0937-9347</issn><eissn>1613-7507</eissn><abstract>The hyperfine structure has been resolved in the optically detected electron spin resonance (OD ESR) spectra of radical ion pairs generated by ionizing radiation at a low dopant concentration in a solid polyethylene matrix at room temperature. The different organic molecules that can capture electrons and holes were used as the dopants. The spin-lattice relaxation times
T
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| subjects | Atoms and Molecules in Strong Fields Charged particles Dopants Electron paramagnetic resonance Electron spin Hydrocarbons Hyperfine structure Ion pairs Ionizing radiation Laser Matter Interaction Magnetic fields Organic Chemistry Original Paper Physical Chemistry Physics Physics and Astronomy Polyethylene Polyethylenes Polymers Radiation Radicals Room temperature Solid State Physics Spectra Spectroscopy/Spectrometry Spin resonance Spin-lattice relaxation Temperature dependence X-rays |
| title | Hyperfine Structure in the OD ESR Spectra of Recombining Charge Pairs in Doped Polyethylene Matrices |
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