1,3,5-Trithian Mediated Formation of Two New One-Dimensional Silver Coordination Polymers and Investigation of Their Optical Features

To study the photoluminescence property of simple silver(I) coordination compounds constructed by 1,3,5-trithian ( 3S ), two new silver(I) polymers, namely, [Ag( 3S ) (9-AnCO 2 )] ∞ ( I , 9-AnCO 2  = anthracene carboxylate), and [Ag 2 ( 3S )(Ph 2 PO 2 ) 2 ] ∞ ( II , Ph 2 PO 2  = diphenylphosphinate)...

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Published in:Journal of cluster science 2023-09, Vol.34 (5), p.2737-2742
Main Authors: Wang, Ling-Xiao, Cheng, Xun, Zhang, Jing-Wen, Hou, Lin-Lin, Liu, Kuan-Guan
Format: Article
Language:English
Subjects:
Absorption spectra
Acids
Anthracene
Brief Communication
Brightening
Catalysis
Chemistry
Chemistry and Materials Science
Cooling
Coordination compounds
Coordination polymers
Crystals
Fourier transforms
Infrared analysis
Infrared spectroscopy
Inorganic Chemistry
Ligands
Molecular structure
Nanochemistry
Optical properties
Photoluminescence
Physical Chemistry
Polymers
Room temperature
Silver
Single crystals
Solid state
Solvents
Thermal analysis
Thermogravimetric analysis
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Cheng, Xun
Zhang, Jing-Wen
Hou, Lin-Lin
Liu, Kuan-Guan
description To study the photoluminescence property of simple silver(I) coordination compounds constructed by 1,3,5-trithian ( 3S ), two new silver(I) polymers, namely, [Ag( 3S ) (9-AnCO 2 )] ∞ ( I , 9-AnCO 2  = anthracene carboxylate), and [Ag 2 ( 3S )(Ph 2 PO 2 ) 2 ] ∞ ( II , Ph 2 PO 2  = diphenylphosphinate), have been prepared and investigated by single-crystal X-ray diffraction (SXRD), fourier-transform infrared spectroscopy (FT-IR), thermal gravimetric analysis (TGA), solid-state UV–vis absorption spectra (SUV) and photoluminescence spectroscopy (PL). Polymer I represents an electroneutral one-dimensional polymer bridging only by 3S . Polymer II represents an electroneutral one-dimensional polymer co-bridging by 3S and diphenylphosphinate. Both polymers show bright emission at room temperature in the solid-state, cyan light for I, and green light for II . The Aggregation-induced Emission (AIE) phenomenon of II is also observed when gradually adding the weakly polar solvent (ether) to its CH 3 CN solvent. Our work shows that 3S is an excellent ligand for constructing new luminous coordination compounds.
doi_str_mv 10.1007/s10876-023-02413-y
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subjects Absorption spectra
Acids
Anthracene
Brief Communication
Brightening
Catalysis
Chemistry
Chemistry and Materials Science
Cooling
Coordination compounds
Coordination polymers
Crystals
Fourier transforms
Infrared analysis
Infrared spectroscopy
Inorganic Chemistry
Ligands
Molecular structure
Nanochemistry
Optical properties
Photoluminescence
Physical Chemistry
Polymers
Room temperature
Silver
Single crystals
Solid state
Solvents
Thermal analysis
Thermogravimetric analysis
title 1,3,5-Trithian Mediated Formation of Two New One-Dimensional Silver Coordination Polymers and Investigation of Their Optical Features
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