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Optical spectroscopy study of charge density wave order in Sr3Rh4Sn13 and (Sr0.5Ca0.5)3Rh4Sn13

We perform optical spectroscopy measurement on single-crystal samples of Sr 3 Rh 4 Sn 13 and (Sr 0.5 Ca 0.5 ) 3 Rh 4 Sn 13 . Formation of CDW energy gap was clearly observed for both single-crystal samples when they undergo the phase transitions. The existence of residual Drude components in σ 1 ( ω...

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Bibliographic Details
Published in:Science China. Physics, mechanics & astronomy mechanics & astronomy, 2017-04, Vol.60 (4), p.047011, Article 047011
Main Authors: Ban, W. J., Wang, H. P., Tseng, C. W., Kuo, C. N., Lue, C. S., Wang, N. L.
Format: Article
Language:English
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Summary:We perform optical spectroscopy measurement on single-crystal samples of Sr 3 Rh 4 Sn 13 and (Sr 0.5 Ca 0.5 ) 3 Rh 4 Sn 13 . Formation of CDW energy gap was clearly observed for both single-crystal samples when they undergo the phase transitions. The existence of residual Drude components in σ 1 ( ω ) below T CDW indicates that the Fermi surface is only partially gapped in the CDW state. The obtained value of 2Δ/ k B T CDW is roughly 13 for both Sr 3 Rh 4 Sn 13 and (Sr 0.5 Ca 0.5 ) 3 Rh 4 Sn 13 compounds, which is considerably larger than the mean-field value based on the weak-coupling BCS theory. The measurements provide optical evidence for the strong coupling characteristics of the CDW phase transition.
ISSN:1674-7348
1869-1927
DOI:10.1007/s11433-017-9007-0