Nanoimprinted Exciton-Polaritons Metasurfaces: Cost-Effective, Large-Scale, High Homogeneity, and Room Temperature Operation

Exciton-polaritons represent a promising platform that combines the strengths of both photonic and electronic systems for future optoelectronic devices. However, their application is currently limited to laboratory research due to the high cost and complexity of fabrication methods, which are not co...

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Bibliographic Details
Published in:arXiv.org 2024-03
Main Authors: Nguyen Ha My Dang, Bouteyre, Paul, Trippé-Allard, Gaëlle, Chevalier, Céline, Deleporte, Emmanuelle, Drouard, Emmanuel, Seassal, Christian, Hai Son Nguyen
Format: Article
Language:English
Subjects:
CMOS
Electronic systems
Excitons
Homogeneity
Low cost
Optoelectronic devices
Perovskites
Polaritons
Room temperature
Substrates
Thin films
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Summary:Exciton-polaritons represent a promising platform that combines the strengths of both photonic and electronic systems for future optoelectronic devices. However, their application is currently limited to laboratory research due to the high cost and complexity of fabrication methods, which are not compatible with the mature CMOS technology developed for microelectronics. In this work, we develop an innovative, low-cost, and CMOS-compatible method for fabricating large surface polaritonic devices. This is achieved by direct patterning of a halide-perovskite thin film via thermal nanoimprint. As a result, we observe highly homogeneous polaritonic modes of quality factor \(Q\approx 300\) at room temperature across a centimetric scale. Impressively, the process provides high reproducibility and fidelity, as the same mold can be reused more than 10 times to imprint the perovskite layer on different types of substrates. Our results could pave the way for the production of low-cost integrated polaritonic devices operating at room temperature.
ISSN:2331-8422