Cycling performance of layered oxide cathode materials for sodium-ion batteries

Layered oxide is a promising cathode material for sodium-ion batteries because of its high-capacity, high operating voltage, and simple synthesis. Cycling performance is an important criterion for evaluating the application prospects of batteries. However, facing challenges, including phase transiti...

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Bibliographic Details
Published in:International journal of minerals, metallurgy and materials metallurgy and materials, 2024-07, Vol.31 (7), p.1720-1744
Main Authors: Wu, Jinpin, Tian, Junhang, Sun, Xueyi, Zhuang, Weidong
Format: Article
Language:English
Subjects:
Alternative energy
Batteries
Cathodes
Ceramics
Characterization and Evaluation of Materials
Chemistry and Materials Science
Composites
Concentration gradient
Corrosion and Coatings
Cycles
Doping
Electric vehicles
Electrode materials
Electrolytes
Energy consumption
Energy resources
Entropy
Environmental impact
Glass
Invited Review
Lithium
Materials Science
Metallic Materials
Metallurgy
Natural Materials
Phase transitions
Retention
Science
Sodium
Sodium-ion batteries
Surfaces and Interfaces
Thin Films
Tribology
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Summary:Layered oxide is a promising cathode material for sodium-ion batteries because of its high-capacity, high operating voltage, and simple synthesis. Cycling performance is an important criterion for evaluating the application prospects of batteries. However, facing challenges, including phase transitions, ambient stability, side reactions, and irreversible anionic oxygen activity, the cycling performance of layered oxide cathode materials still cannot meet the application requirements. Therefore, this review proposes several strategies to address these challenges. First, bulk doping is introduced from three aspects: cationic single doping, anionic single doping, and multi-ion doping. Second, homogeneous surface coating and concentration gradient modification are reviewed. In addition, methods such as mixed structure design, particle engineering, high-entropy material construction, and integrated modification are proposed. Finally, a summary and outlook provide a new horizon for developing and modifying layered oxide cathode materials.
ISSN:1674-4799
1869-103X
DOI:10.1007/s12613-023-2776-5