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Indium-doped ZnO nanoparticle effects on the optical and electrical characterization under dark and illumination of OFET: application for optoelectronics and nonvolatile memory devices

Organic field-effect transistors (OFETs), based on poly(3-hexylthiophene) (P3HT) enriched by indium-doped zinc oxide (IZO) nanoparticles as an active layer, were successfully prepared by the spin-coating method. We report a significant impact of IZO nanoparticles on the P3HT carrier mobility, which...

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Bibliographic Details
Published in:Journal of materials science 2024-08, Vol.59 (32), p.15435-15448
Main Authors: Jdir, M., Erouel, M., Ba, M., Chouiref, L., El Beji, M., Mansouri, S., El Mir, L.
Format: Article
Language:English
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Summary:Organic field-effect transistors (OFETs), based on poly(3-hexylthiophene) (P3HT) enriched by indium-doped zinc oxide (IZO) nanoparticles as an active layer, were successfully prepared by the spin-coating method. We report a significant impact of IZO nanoparticles on the P3HT carrier mobility, which can be controlled by IZO-level loading. The X-ray diffraction and the UV–visible analysis conducted on P3HT/IZO nanocomposite thin films showed an enhancement of the conjugated chain length. Moreover, the improvement of the P3HT properties resulted in an increase in the polymer crystallinity and a reduction of the trap density. A particular result was illustrated corresponding to the enhancement of the carrier mobility and I ON / I OFF ratio in the devices based on hybrid nanocomposite. The significant hysteresis observed in this device, which depends on IZO content and illumination under ambient conditions and renders these OFETs promising for various optoelectronic and nonvolatile memory applications. Graphical abstract
ISSN:0022-2461
1573-4803
DOI:10.1007/s10853-024-10079-8