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Improving the Stability and Efficiency of Perovskite Solar Cells by Controlling the Crystallization Active Layer with Binary Anti-solvent
In this study, a hybrid anti-solvent treatment was used to prepare high-quality MA 0.9 FA 0.1 PbI 3 perovskite film, and perovskite solar cells (PSCs) with carbon counter electrodes of high stability and high efficiency were fabricated. Different ratios of chlorobenzene (CB) and toluene (TL) were ut...
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| Published in: | Chemical research in Chinese universities 2024, Vol.40 (6), p.1160-1170 |
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| Main Authors: | , , , , , , |
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| Language: | English |
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| container_end_page | 1170 |
| container_issue | 6 |
| container_start_page | 1160 |
| container_title | Chemical research in Chinese universities |
| container_volume | 40 |
| creator | Chen, Diandian Bala, Hari Zhang, Bowen Zhao, Zhiyong Zhao, Yunpeng Cheng, Fei Wen, Yingjie |
| description | In this study, a hybrid anti-solvent treatment was used to prepare high-quality MA
0.9
FA
0.1
PbI
3
perovskite film, and perovskite solar cells (PSCs) with carbon counter electrodes of high stability and high efficiency were fabricated. Different ratios of chlorobenzene (CB) and toluene (TL) were utilized as binary anti-solvent, and dropwise addition was initiated within spin-coating perovskite film. By optimizing the ratio of CB and TL, the formation process of perovskite film was effectively controlled and the crystallinity and coverage of the perovskite film were improved. The carbon electrode PSCs composed of MA
0.9
FA
0.1
PbI
3
film treated with anti-solvent exhibited a maximum power conversion efficiency (PCE) of 12.21% under air atmosphere conditions, which was higher than that of the PSCs of MA
0.9
FA
0.1
PbI
3
film without anti-solvent treatment. Finally, PSCs showed that the device still exhibits 90% of the initial efficiency after being stored in the air for 100 d, which shows excellent stability. |
| doi_str_mv | 10.1007/s40242-024-4049-x |
| format | article |
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0.9
FA
0.1
PbI
3
perovskite film, and perovskite solar cells (PSCs) with carbon counter electrodes of high stability and high efficiency were fabricated. Different ratios of chlorobenzene (CB) and toluene (TL) were utilized as binary anti-solvent, and dropwise addition was initiated within spin-coating perovskite film. By optimizing the ratio of CB and TL, the formation process of perovskite film was effectively controlled and the crystallinity and coverage of the perovskite film were improved. The carbon electrode PSCs composed of MA
0.9
FA
0.1
PbI
3
film treated with anti-solvent exhibited a maximum power conversion efficiency (PCE) of 12.21% under air atmosphere conditions, which was higher than that of the PSCs of MA
0.9
FA
0.1
PbI
3
film without anti-solvent treatment. Finally, PSCs showed that the device still exhibits 90% of the initial efficiency after being stored in the air for 100 d, which shows excellent stability.</description><identifier>ISSN: 1005-9040</identifier><identifier>EISSN: 2210-3171</identifier><identifier>DOI: 10.1007/s40242-024-4049-x</identifier><language>eng</language><publisher>Changchun: Jilin University and The Editorial Department of Chemical Research in Chinese Universities</publisher><subject>Analytical Chemistry ; Carbon ; Chemistry ; Chemistry and Materials Science ; Chemistry/Food Science ; Chlorobenzene ; Crystallization ; Electrodes ; Energy conversion efficiency ; Inorganic Chemistry ; Maximum power ; Organic Chemistry ; Perovskites ; Photovoltaic cells ; Physical Chemistry ; Solar cells ; Solvents ; Spin coating ; Stability ; Toluene</subject><ispartof>Chemical research in Chinese universities, 2024, Vol.40 (6), p.1160-1170</ispartof><rights>Jilin University, The Editorial Department of Chemical Research in Chinese Universities and Springer-Verlag GmbH 2024</rights><rights>Jilin University, The Editorial Department of Chemical Research in Chinese Universities and Springer-Verlag GmbH 2024.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><cites>FETCH-LOGICAL-c268t-515638a8814a700206db268bd736342faa5ede343bd6939c84167119e31937273</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,27924,27925</link.rule.ids></links><search><creatorcontrib>Chen, Diandian</creatorcontrib><creatorcontrib>Bala, Hari</creatorcontrib><creatorcontrib>Zhang, Bowen</creatorcontrib><creatorcontrib>Zhao, Zhiyong</creatorcontrib><creatorcontrib>Zhao, Yunpeng</creatorcontrib><creatorcontrib>Cheng, Fei</creatorcontrib><creatorcontrib>Wen, Yingjie</creatorcontrib><title>Improving the Stability and Efficiency of Perovskite Solar Cells by Controlling the Crystallization Active Layer with Binary Anti-solvent</title><title>Chemical research in Chinese universities</title><addtitle>Chem. Res. Chin. Univ</addtitle><description>In this study, a hybrid anti-solvent treatment was used to prepare high-quality MA
0.9
FA
0.1
PbI
3
perovskite film, and perovskite solar cells (PSCs) with carbon counter electrodes of high stability and high efficiency were fabricated. Different ratios of chlorobenzene (CB) and toluene (TL) were utilized as binary anti-solvent, and dropwise addition was initiated within spin-coating perovskite film. By optimizing the ratio of CB and TL, the formation process of perovskite film was effectively controlled and the crystallinity and coverage of the perovskite film were improved. The carbon electrode PSCs composed of MA
0.9
FA
0.1
PbI
3
film treated with anti-solvent exhibited a maximum power conversion efficiency (PCE) of 12.21% under air atmosphere conditions, which was higher than that of the PSCs of MA
0.9
FA
0.1
PbI
3
film without anti-solvent treatment. Finally, PSCs showed that the device still exhibits 90% of the initial efficiency after being stored in the air for 100 d, which shows excellent stability.</description><subject>Analytical Chemistry</subject><subject>Carbon</subject><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Chemistry/Food Science</subject><subject>Chlorobenzene</subject><subject>Crystallization</subject><subject>Electrodes</subject><subject>Energy conversion efficiency</subject><subject>Inorganic Chemistry</subject><subject>Maximum power</subject><subject>Organic Chemistry</subject><subject>Perovskites</subject><subject>Photovoltaic cells</subject><subject>Physical Chemistry</subject><subject>Solar cells</subject><subject>Solvents</subject><subject>Spin coating</subject><subject>Stability</subject><subject>Toluene</subject><issn>1005-9040</issn><issn>2210-3171</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2024</creationdate><recordtype>article</recordtype><recordid>eNp1kMtOxCAYhYnRxPHyAO5IXKPcStvl2IyXZBJN1DWhLXUYOzACM059A99aTDWu3BxC-M75fw4AZwRfEIzzy8Ax5RQlQRzzEu32wIRSghEjOdkHkwRlqMQcH4KjEJYYs1IIPgGfd6u1d1tjX2BcaPgYVW16EweobAtnXWcao20zQNfBB53A8GpiwlyvPKx03wdYD7ByNnrX978plR9CVOn-oaJxFk6baLYaztWgPXw3cQGvjFV-gFMbDQqu32obT8BBp_qgT3_OY_B8PXuqbtH8_uaums5RQ0URUUYywQpVFISrHGOKRVunh7rNmWCcdkplutWMs7oVJSubghORE1JqRkqW05wdg_MxN_37baNDlEu38TaNlIzQghYZLkSiyEg13oXgdSfX3qzSzpJg-d24HBuXSeR343KXPHT0hMTaF-3_kv83fQGm3ITl</recordid><startdate>2024</startdate><enddate>2024</enddate><creator>Chen, Diandian</creator><creator>Bala, Hari</creator><creator>Zhang, Bowen</creator><creator>Zhao, Zhiyong</creator><creator>Zhao, Yunpeng</creator><creator>Cheng, Fei</creator><creator>Wen, Yingjie</creator><general>Jilin University and The Editorial Department of Chemical Research in Chinese Universities</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope></search><sort><creationdate>2024</creationdate><title>Improving the Stability and Efficiency of Perovskite Solar Cells by Controlling the Crystallization Active Layer with Binary Anti-solvent</title><author>Chen, Diandian ; Bala, Hari ; Zhang, Bowen ; Zhao, Zhiyong ; Zhao, Yunpeng ; Cheng, Fei ; Wen, Yingjie</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c268t-515638a8814a700206db268bd736342faa5ede343bd6939c84167119e31937273</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2024</creationdate><topic>Analytical Chemistry</topic><topic>Carbon</topic><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Chemistry/Food Science</topic><topic>Chlorobenzene</topic><topic>Crystallization</topic><topic>Electrodes</topic><topic>Energy conversion efficiency</topic><topic>Inorganic Chemistry</topic><topic>Maximum power</topic><topic>Organic Chemistry</topic><topic>Perovskites</topic><topic>Photovoltaic cells</topic><topic>Physical Chemistry</topic><topic>Solar cells</topic><topic>Solvents</topic><topic>Spin coating</topic><topic>Stability</topic><topic>Toluene</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Chen, Diandian</creatorcontrib><creatorcontrib>Bala, Hari</creatorcontrib><creatorcontrib>Zhang, Bowen</creatorcontrib><creatorcontrib>Zhao, Zhiyong</creatorcontrib><creatorcontrib>Zhao, Yunpeng</creatorcontrib><creatorcontrib>Cheng, Fei</creatorcontrib><creatorcontrib>Wen, Yingjie</creatorcontrib><collection>CrossRef</collection><jtitle>Chemical research in Chinese universities</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Chen, Diandian</au><au>Bala, Hari</au><au>Zhang, Bowen</au><au>Zhao, Zhiyong</au><au>Zhao, Yunpeng</au><au>Cheng, Fei</au><au>Wen, Yingjie</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Improving the Stability and Efficiency of Perovskite Solar Cells by Controlling the Crystallization Active Layer with Binary Anti-solvent</atitle><jtitle>Chemical research in Chinese universities</jtitle><stitle>Chem. Res. Chin. Univ</stitle><date>2024</date><risdate>2024</risdate><volume>40</volume><issue>6</issue><spage>1160</spage><epage>1170</epage><pages>1160-1170</pages><issn>1005-9040</issn><eissn>2210-3171</eissn><abstract>In this study, a hybrid anti-solvent treatment was used to prepare high-quality MA
0.9
FA
0.1
PbI
3
perovskite film, and perovskite solar cells (PSCs) with carbon counter electrodes of high stability and high efficiency were fabricated. Different ratios of chlorobenzene (CB) and toluene (TL) were utilized as binary anti-solvent, and dropwise addition was initiated within spin-coating perovskite film. By optimizing the ratio of CB and TL, the formation process of perovskite film was effectively controlled and the crystallinity and coverage of the perovskite film were improved. The carbon electrode PSCs composed of MA
0.9
FA
0.1
PbI
3
film treated with anti-solvent exhibited a maximum power conversion efficiency (PCE) of 12.21% under air atmosphere conditions, which was higher than that of the PSCs of MA
0.9
FA
0.1
PbI
3
film without anti-solvent treatment. Finally, PSCs showed that the device still exhibits 90% of the initial efficiency after being stored in the air for 100 d, which shows excellent stability.</abstract><cop>Changchun</cop><pub>Jilin University and The Editorial Department of Chemical Research in Chinese Universities</pub><doi>10.1007/s40242-024-4049-x</doi><tpages>11</tpages></addata></record> |
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| ispartof | Chemical research in Chinese universities, 2024, Vol.40 (6), p.1160-1170 |
| issn | 1005-9040 2210-3171 |
| language | eng |
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| subjects | Analytical Chemistry Carbon Chemistry Chemistry and Materials Science Chemistry/Food Science Chlorobenzene Crystallization Electrodes Energy conversion efficiency Inorganic Chemistry Maximum power Organic Chemistry Perovskites Photovoltaic cells Physical Chemistry Solar cells Solvents Spin coating Stability Toluene |
| title | Improving the Stability and Efficiency of Perovskite Solar Cells by Controlling the Crystallization Active Layer with Binary Anti-solvent |
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