Latitudinal variation of the effect of aviation NOx emissions on atmospheric ozone and methane and related climate metrics

• Published in: Atmospheric environment (1994) 2013-01, Vol.64, p.1-9
• Main Authors: Köhler, M.O., Rädel, G., Shine, K.P., Rogers, H.L., Pyle, J.A.
• Format: Article
• Language: English
• Subjects: Aircraft; Aircraft emissions; altitude; Applied sciences; atmospheric chemistry; Atmospheric pollution; Atmospherics; aviation; climate; Climate metrics; Climatology. Bioclimatology. Climate change; Earth, ocean, space; Emission; Emission analysis; emissions; Exact sciences and technology; External geophysics; global warming; Greenhouse gases; guanosine triphosphate; Latitude; Meteorology; Methane; Nitrogen oxides; Ozone; Pollution; Pollution sources. Measurement results; Radiative forcing; Radio frequencies; temperature; Transports
• ISSN: 1352-2310; 1873-2844
• DOI: 10.1016/j.atmosenv.2012.09.013

We evaluate the response to regional and latitudinal changes in aircraft NOx emissions using several climate metrics (radiative forcing (RF), Global Warming Potential (GWP), Global Temperature change Potential (GTP)). Global chemistry transport model integrations were performed with sustained perturbations in regional aircraft and aircraft-like NOx emissions. The RF due to the resulting ozone and methane changes is then calculated. We investigate the impact of emission changes for specific geographical regions (approximating to USA, Europe, India and China) and cruise altitude emission changes in discrete latitude bands covering both hemispheres. We find that lower latitude emission changes (per Tg N) cause ozone and methane RFs that are about a factor of 6 larger than those from higher latitude emission changes. The net RF is positive for all experiments. The meridional extent of the RF is larger for low latitude emissions. GWPs for all emission changes are positive, with tropical emissions having the largest values; the sign of the GTP depends on the choice of time horizon. ► Global model study on climate response to regional/latitudinal aircraft NOx changes. ► RF impacts from O3 and CH4 are larger for changes at lower than at higher latitudes. ► GWPs for all latitudes are positive whereas the GTP can exhibit a change in sign.