Performance of a gaseous detector based energy dispersive X-ray fluorescence imaging system: Analysis of human teeth treated with dental amalgam

• Published in: Spectrochimica acta. Part B: Atomic spectroscopy 2013-08, Vol.86, p.115-122
• Main Authors: Silva, A.L.M., Figueroa, R., Jaramillo, A., Carvalho, M.L., Veloso, J.F.C.A.
• Format: Article
• Language: English
• Subjects: Constituents; Dental amalgams; Drift; Elemental map distribution; Energy dispersive; Energy dispersive X-ray fluorescence; Gaseous detector; Human; Imaging; Imaging system; Mercury (metal); Teeth; Teeth analysis
• ISSN: 0584-8547; 1873-3565
• DOI: 10.1016/j.sab.2013.03.005

Energy dispersive X-ray fluorescence (EDXRF) imaging systems are of great interest in many applications of different areas, once they allow us to get images of the spatial elemental distribution in the samples. The detector system used in this study is based on a micro patterned gas detector, named Micro-Hole and Strip Plate. The full field of view system, with an active area of 28×28mm2 presents some important features for EDXRF imaging applications, such as a position resolution below 125μm, an intrinsic energy resolution of about 14% full width at half maximum for 5.9keV X-rays, and a counting rate capability of 0.5MHz. In this work, analysis of human teeth treated by dental amalgam was performed by using the EDXRF imaging system mentioned above. The goal of the analysis is to evaluate the system capabilities in the biomedical field by measuring the drift of the major constituents of a dental amalgam, Zn and Hg, throughout the tooth structures. The elemental distribution pattern of these elements obtained during the analysis suggests diffusion of these elements from the amalgam to teeth tissues. •Demonstration of an EDXRF imaging system based on a 2D-MHSP detector for biological analysis•Evaluation of the drift of the dental amalgam constituents, throughout the teeth•Observation of Hg diffusion, due to hydroxyapatite crystal defects that compose the teeth tissues