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Correlation between the valence state of cerium and the magnetic transition in Ce(Ru sub(1-x) Fe sub(x)) sub(2) Al sub(10) studied by resonant x-ray emission spectroscopy
The correlation between the 4f-conduction electron (c-f) hybridization and the transition temperature T sub(0) into the unconventional antiferromagnetically (AFM) ordered state in Ce(Ru sub(1-x) Fe sub(x)) sub(2)Al sub(10) has been investigated. The impact of pressure on the crystal structure and th...
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Published in: | Physical review. B, Condensed matter and materials physics Condensed matter and materials physics, 2014-03, Vol.89 (12) |
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Main Authors: | , , , , , , , , , , , |
Format: | Article |
Language: | English |
Subjects: | |
Online Access: | Get full text |
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Summary: | The correlation between the 4f-conduction electron (c-f) hybridization and the transition temperature T sub(0) into the unconventional antiferromagnetically (AFM) ordered state in Ce(Ru sub(1-x) Fe sub(x)) sub(2)Al sub(10) has been investigated. The impact of pressure on the crystal structure and the electronic structure has been measured using x-ray diffraction and resonant x-ray emission spectroscopy at the Ce L sub(3) absorption edge in a diamond anvil cell. Our results show that the lattice spacings imply some correlation with the disappearance of T sub(0). Analyses of the measured valence states, however, show only a weak correlation with the corresponding critical disappearance of the AFM order within experimental errors. Our results may be explained by a scenario based on the Kondo-Heisenberg model beyond the conventional Doniach phase diagram. |
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ISSN: | 1098-0121 1550-235X |