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Lifetime measurement of the first vibrationally excited state of MgH super(+) in a cryogenic Paul Trap (CryPTEx)

A method is presented to measure the decay rate of the first excited vibrational state of polar molecular ions being part of a Coulomb crystal in a cryogenic linear Paul trap. Specifically, we have monitored the decay of the |v=1,J=1> sub(X) towards the |v=0,J=0> sub(X) level in MgH super(+) b...

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Published in:CPEM digest 2014-08, p.56-57
Main Authors: Versolato, O O, Schwarz, M, Hansen, A K, Gingell, AD, Windberger, A, Klosowski, L, Ullrich, J, Lopez-Urrutia, Crespo, Jensen, F, Drewsen, M
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creator Versolato, O O
Schwarz, M
Hansen, A K
Gingell, AD
Windberger, A
Klosowski, L
Ullrich, J
Lopez-Urrutia, Crespo
Jensen, F
Drewsen, M
description A method is presented to measure the decay rate of the first excited vibrational state of polar molecular ions being part of a Coulomb crystal in a cryogenic linear Paul trap. Specifically, we have monitored the decay of the |v=1,J=1> sub(X) towards the |v=0,J=0> sub(X) level in MgH super(+) by saturated laser excitation of the |v=0,J=2> sub(X) - |v=1,J=1> sub(X) transition followed by state selective resonance-enhanced two-photon dissociation out of the |v=0,J=2> sub(X) level. The technique can be extended to other simple molecular ions and it enables the determination, with an accuracy at the few percent level, of decay rates and thus absorption strengths.
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subjects Conferences
Coulomb friction
Crystals
Decay
Decay rate
Excitation
Lasers
Molecular ions
Vibrational states
title Lifetime measurement of the first vibrationally excited state of MgH super(+) in a cryogenic Paul Trap (CryPTEx)
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