Single-Ion Recycling Reactions

A single ion is enough: Ion reaction rates and reaction product branching ratios could be determined through repeated regeneration of the original target ion by photodissociation after each reaction. The product molecule was identified through nondestructive mass spectrometry. Finally, the target io...

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Bibliographic Details
Published in:Angewandte Chemie International Edition 2012-08, Vol.51 (32), p.7960-7962
Main Authors: Hansen, Anders K., Sørensen, Magnus A., Staanum, Peter F., Drewsen, Michael
Format: Article
Language:English
Subjects:
actinoids
ion-molecule reactions
isotope effects
laser chemistry
low-temperature physics
Mass spectrometry
Photodissociation
Pictures
Reaction products
Recycling
Regeneration
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Summary:A single ion is enough: Ion reaction rates and reaction product branching ratios could be determined through repeated regeneration of the original target ion by photodissociation after each reaction. The product molecule was identified through nondestructive mass spectrometry. Finally, the target ion was regenerated through photodissociation of the molecular ion (see picture).
ISSN:1433-7851
1521-3773
DOI:10.1002/anie.201203550