Hexabromocyclododecane Flame Retardant Isomers in Sediments from Detroit River and Lake Erie of the Laurentian Great Lakes of North America

Sediments collected in 2004 from along the Detroit River (n = 19) and across all of Lake Erie (n = 18) were analyzed for isomers of the flame retardant chemical, hexabromocyclododecane (HBCD), using liquid chromatography-tandem mass spectrometry. Sediment samples had ΣHBCD concentrations ranging fro...

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Published in:Bulletin of environmental contamination and toxicology 2015-07, Vol.95 (1), p.31-36
Main Authors: Letcher, Robert J., Lu, Zhe, Chu, Shaogang, Haffner, G. Douglas, Drouillard, Ken, Marvin, Christopher H., Ciborowski, Jan J. H.
Format: Article
Language:English
Subjects:
Aquatic Pollution
Basins
Chemical contaminants
Chromatography, Liquid
Contaminated sediments
Contamination
Earth and Environmental Science
Ecotoxicology
Environment
Environmental Chemistry
Environmental Health
Environmental Monitoring - methods
Flame retardants
Flame Retardants - analysis
Freshwater
Geologic Sediments - chemistry
Great Lakes Region
Hydrocarbons, Brominated - analysis
Hydrocarbons, Brominated - chemistry
Isomerism
Isomers
Lake Erie
Lakes
Lakes - chemistry
Liquid chromatography
Mass Spectrometry
Pollution
Rivers
Rivers - chemistry
Sediment samplers
Sediments
Sludge
Soil Science & Conservation
Toxicity
Waste Water Technology
Wastewater treatment plants
Water analysis
Water Management
Water Pollutants, Chemical - analysis
Water Pollutants, Chemical - chemistry
Water pollution
Water Pollution Control
Water sampling
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container_title Bulletin of environmental contamination and toxicology
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creator Letcher, Robert J.
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Haffner, G. Douglas
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Marvin, Christopher H.
Ciborowski, Jan J. H.
description Sediments collected in 2004 from along the Detroit River (n = 19) and across all of Lake Erie (n = 18) were analyzed for isomers of the flame retardant chemical, hexabromocyclododecane (HBCD), using liquid chromatography-tandem mass spectrometry. Sediment samples had ΣHBCD concentrations ranging from not detected to 1.6 ng/g d.w. γ-HBCD (56 %–100 % of ΣHBCDs) was the predominate isomer, observed in 7 of 19 samples from the Detroit River and 6 of 18 samples from Lake Erie (all within the western basin). α-HBCD was found in 4 Detroit River and 2 Lake Erie western basin sites, while β-HBCD was only in two Detroit River samples. High ΣHBCD concentrations (>100 ng/g d.w.) were found in two sludge samples from two Windsor, ON, wastewater treatment plants that feed into the Detroit River upstream. HBCD contamination into the Detroit River is a major input vector into Lake Erie and with an apparent sediment dilution effect moving towards the eastern basin.
doi_str_mv 10.1007/s00128-015-1491-y
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ispartof Bulletin of environmental contamination and toxicology, 2015-07, Vol.95 (1), p.31-36
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source Springer Nature
subjects Aquatic Pollution
Basins
Chemical contaminants
Chromatography, Liquid
Contaminated sediments
Contamination
Earth and Environmental Science
Ecotoxicology
Environment
Environmental Chemistry
Environmental Health
Environmental Monitoring - methods
Flame retardants
Flame Retardants - analysis
Freshwater
Geologic Sediments - chemistry
Great Lakes Region
Hydrocarbons, Brominated - analysis
Hydrocarbons, Brominated - chemistry
Isomerism
Isomers
Lake Erie
Lakes
Lakes - chemistry
Liquid chromatography
Mass Spectrometry
Pollution
Rivers
Rivers - chemistry
Sediment samplers
Sediments
Sludge
Soil Science & Conservation
Toxicity
Waste Water Technology
Wastewater treatment plants
Water analysis
Water Management
Water Pollutants, Chemical - analysis
Water Pollutants, Chemical - chemistry
Water pollution
Water Pollution Control
Water sampling
title Hexabromocyclododecane Flame Retardant Isomers in Sediments from Detroit River and Lake Erie of the Laurentian Great Lakes of North America
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