Surface-Plasmon-Enhanced Photodriven CO sub(2) Reduction Catalyzed by Metal-Organic-Framework-Derived Iron Nanoparticles Encapsulated by Ultrathin Carbon Layers

Highly efficient utilization of solar light with an excellent reduction capacity is achieved for plasmonic Fe nanostructures. By carbon layer coating, the optimized catalyst exhibits enhanced selectivity and stability applied to the solar-driven reduction of CO sub(2) into CO. The surface-plasmon ef...

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Bibliographic Details
Published in:Advanced materials (Weinheim) 2016-05, Vol.28 (19), p.3703-3710
Main Authors: Zhang, Huabin, Wang, Tao, Wang, Junjie, Liu, Huimin, Dao, Thang Duy, Li, Mu, Liu, Guigao, Meng, Xianguang, Chang, Kun, Shi, Li, Nagao, Tadaaki, Ye, Jinhua
Format: Article
Language:English
Subjects:
Carbon
Carbon dioxide
Carbon monoxide
Encapsulation
Iron
Nanoparticles
Plasmonics
Reduction
Online Access:Get full text
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Summary:Highly efficient utilization of solar light with an excellent reduction capacity is achieved for plasmonic Fe nanostructures. By carbon layer coating, the optimized catalyst exhibits enhanced selectivity and stability applied to the solar-driven reduction of CO sub(2) into CO. The surface-plasmon effect of iron particles is proposed to excite CO sub(2) molecules, and thereby facilitates the final reaction activity.
ISSN:0935-9648
1521-4095
DOI:10.1002/adma.201505187