Loading…
Rashba Interaction and Local Magnetic Moments in a Graphene-BN Heterostructure Intercalated with Au
We intercalate a van der Waals heterostructure of graphene and hexagonal boron nitride with Au, by encapsulation, and show that the Au at the interface is two dimensional. Charge transfer upon current annealing indicates the redistribution of the Au and induces splitting of the graphene band structu...
Saved in:
Published in: | Physical review letters 2016-08, Vol.117 (7), p.076603-076603, Article 076603 |
---|---|
Main Authors: | , , , , , , |
Format: | Article |
Language: | English |
Subjects: | |
Citations: | Items that this one cites Items that cite this one |
Online Access: | Get full text |
Tags: |
Add Tag
No Tags, Be the first to tag this record!
|
cited_by | cdi_FETCH-LOGICAL-c344t-6bcfe98c1aa8929e405762251e7035e848ae13fb34bdb09278d8049944e8b8513 |
---|---|
cites | cdi_FETCH-LOGICAL-c344t-6bcfe98c1aa8929e405762251e7035e848ae13fb34bdb09278d8049944e8b8513 |
container_end_page | 076603 |
container_issue | 7 |
container_start_page | 076603 |
container_title | Physical review letters |
container_volume | 117 |
creator | O'Farrell, E C T Tan, J Y Yeo, Y Koon, G K W Özyilmaz, B Watanabe, K Taniguchi, T |
description | We intercalate a van der Waals heterostructure of graphene and hexagonal boron nitride with Au, by encapsulation, and show that the Au at the interface is two dimensional. Charge transfer upon current annealing indicates the redistribution of the Au and induces splitting of the graphene band structure. The effect of an in-plane magnetic field confirms that the splitting is due to spin splitting and that the spin polarization is in the plane, characteristic of a Rashba interaction with a magnitude of approximately 25 meV. Consistent with the presence of an intrinsic interfacial electric field we show that the splitting can be enhanced by an applied displacement field in dual gated samples. A giant negative magnetoresistance, up to 75%, and a field induced anomalous Hall effect at magnetic fields |
doi_str_mv | 10.1103/PhysRevLett.117.076603 |
format | article |
fullrecord | <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_miscellaneous_1835656748</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>1835656748</sourcerecordid><originalsourceid>FETCH-LOGICAL-c344t-6bcfe98c1aa8929e405762251e7035e848ae13fb34bdb09278d8049944e8b8513</originalsourceid><addsrcrecordid>eNqNkU1PwkAQhjdGI4j-BbJHL8XZ7nY_jkgUSPAjRM_NdjtIDbTY3Wr495YUjUdPk7zzPjOZeQkZMhgxBvzmeb33S_xcYAitoEagpAR-QvoMlIkUY-KU9AE4iwyA6pEL798BgMVSn5NerBLJjY77xC2tX2eWzsuAtXWhqEpqy5wuKmc39MG-lRgKRx-qLZbB06Lt0mltd2ssMbp9pDNsucqHunGhqbGb06I2YE6_irCm4-aSnK3sxuPVsQ7I6_3dy2QWLZ6m88l4ETkuRIhk5lZotGPWahMbFJAoGccJQwU8QS20RcZXGRdZnoGJlc41CGOEQJ3phPEBue7m7urqo0Ef0m3hHW42tsSq8SnTPJGJVEL_w8qETDTTB6vsrK6909e4Snd1sbX1PmWQHrJI_2TRCirtsmjB4XFHk20x_8V-ns-_Af3Dh3M</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>1814658188</pqid></control><display><type>article</type><title>Rashba Interaction and Local Magnetic Moments in a Graphene-BN Heterostructure Intercalated with Au</title><source>American Physical Society:Jisc Collections:APS Read and Publish 2023-2025 (reading list)</source><creator>O'Farrell, E C T ; Tan, J Y ; Yeo, Y ; Koon, G K W ; Özyilmaz, B ; Watanabe, K ; Taniguchi, T</creator><creatorcontrib>O'Farrell, E C T ; Tan, J Y ; Yeo, Y ; Koon, G K W ; Özyilmaz, B ; Watanabe, K ; Taniguchi, T</creatorcontrib><description>We intercalate a van der Waals heterostructure of graphene and hexagonal boron nitride with Au, by encapsulation, and show that the Au at the interface is two dimensional. Charge transfer upon current annealing indicates the redistribution of the Au and induces splitting of the graphene band structure. The effect of an in-plane magnetic field confirms that the splitting is due to spin splitting and that the spin polarization is in the plane, characteristic of a Rashba interaction with a magnitude of approximately 25 meV. Consistent with the presence of an intrinsic interfacial electric field we show that the splitting can be enhanced by an applied displacement field in dual gated samples. A giant negative magnetoresistance, up to 75%, and a field induced anomalous Hall effect at magnetic fields <1 T are observed. These demonstrate that the hybridized Au has a magnetic moment and suggests the proximity to the formation of a collective magnetic phase. These effects persist close to room temperature.</description><identifier>ISSN: 0031-9007</identifier><identifier>EISSN: 1079-7114</identifier><identifier>DOI: 10.1103/PhysRevLett.117.076603</identifier><identifier>PMID: 27563982</identifier><language>eng</language><publisher>United States</publisher><subject>Boron nitride ; Charge transfer ; Electric fields ; Graphene ; Heterostructures ; Magnetic fields ; Magnetic moment ; Splitting</subject><ispartof>Physical review letters, 2016-08, Vol.117 (7), p.076603-076603, Article 076603</ispartof><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c344t-6bcfe98c1aa8929e405762251e7035e848ae13fb34bdb09278d8049944e8b8513</citedby><cites>FETCH-LOGICAL-c344t-6bcfe98c1aa8929e405762251e7035e848ae13fb34bdb09278d8049944e8b8513</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,777,781,27905,27906</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/27563982$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>O'Farrell, E C T</creatorcontrib><creatorcontrib>Tan, J Y</creatorcontrib><creatorcontrib>Yeo, Y</creatorcontrib><creatorcontrib>Koon, G K W</creatorcontrib><creatorcontrib>Özyilmaz, B</creatorcontrib><creatorcontrib>Watanabe, K</creatorcontrib><creatorcontrib>Taniguchi, T</creatorcontrib><title>Rashba Interaction and Local Magnetic Moments in a Graphene-BN Heterostructure Intercalated with Au</title><title>Physical review letters</title><addtitle>Phys Rev Lett</addtitle><description>We intercalate a van der Waals heterostructure of graphene and hexagonal boron nitride with Au, by encapsulation, and show that the Au at the interface is two dimensional. Charge transfer upon current annealing indicates the redistribution of the Au and induces splitting of the graphene band structure. The effect of an in-plane magnetic field confirms that the splitting is due to spin splitting and that the spin polarization is in the plane, characteristic of a Rashba interaction with a magnitude of approximately 25 meV. Consistent with the presence of an intrinsic interfacial electric field we show that the splitting can be enhanced by an applied displacement field in dual gated samples. A giant negative magnetoresistance, up to 75%, and a field induced anomalous Hall effect at magnetic fields <1 T are observed. These demonstrate that the hybridized Au has a magnetic moment and suggests the proximity to the formation of a collective magnetic phase. These effects persist close to room temperature.</description><subject>Boron nitride</subject><subject>Charge transfer</subject><subject>Electric fields</subject><subject>Graphene</subject><subject>Heterostructures</subject><subject>Magnetic fields</subject><subject>Magnetic moment</subject><subject>Splitting</subject><issn>0031-9007</issn><issn>1079-7114</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2016</creationdate><recordtype>article</recordtype><recordid>eNqNkU1PwkAQhjdGI4j-BbJHL8XZ7nY_jkgUSPAjRM_NdjtIDbTY3Wr495YUjUdPk7zzPjOZeQkZMhgxBvzmeb33S_xcYAitoEagpAR-QvoMlIkUY-KU9AE4iwyA6pEL798BgMVSn5NerBLJjY77xC2tX2eWzsuAtXWhqEpqy5wuKmc39MG-lRgKRx-qLZbB06Lt0mltd2ssMbp9pDNsucqHunGhqbGb06I2YE6_irCm4-aSnK3sxuPVsQ7I6_3dy2QWLZ6m88l4ETkuRIhk5lZotGPWahMbFJAoGccJQwU8QS20RcZXGRdZnoGJlc41CGOEQJ3phPEBue7m7urqo0Ef0m3hHW42tsSq8SnTPJGJVEL_w8qETDTTB6vsrK6909e4Snd1sbX1PmWQHrJI_2TRCirtsmjB4XFHk20x_8V-ns-_Af3Dh3M</recordid><startdate>20160812</startdate><enddate>20160812</enddate><creator>O'Farrell, E C T</creator><creator>Tan, J Y</creator><creator>Yeo, Y</creator><creator>Koon, G K W</creator><creator>Özyilmaz, B</creator><creator>Watanabe, K</creator><creator>Taniguchi, T</creator><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope><scope>7U5</scope><scope>8FD</scope><scope>H8D</scope><scope>L7M</scope></search><sort><creationdate>20160812</creationdate><title>Rashba Interaction and Local Magnetic Moments in a Graphene-BN Heterostructure Intercalated with Au</title><author>O'Farrell, E C T ; Tan, J Y ; Yeo, Y ; Koon, G K W ; Özyilmaz, B ; Watanabe, K ; Taniguchi, T</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c344t-6bcfe98c1aa8929e405762251e7035e848ae13fb34bdb09278d8049944e8b8513</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2016</creationdate><topic>Boron nitride</topic><topic>Charge transfer</topic><topic>Electric fields</topic><topic>Graphene</topic><topic>Heterostructures</topic><topic>Magnetic fields</topic><topic>Magnetic moment</topic><topic>Splitting</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>O'Farrell, E C T</creatorcontrib><creatorcontrib>Tan, J Y</creatorcontrib><creatorcontrib>Yeo, Y</creatorcontrib><creatorcontrib>Koon, G K W</creatorcontrib><creatorcontrib>Özyilmaz, B</creatorcontrib><creatorcontrib>Watanabe, K</creatorcontrib><creatorcontrib>Taniguchi, T</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>Technology Research Database</collection><collection>Aerospace Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Physical review letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>O'Farrell, E C T</au><au>Tan, J Y</au><au>Yeo, Y</au><au>Koon, G K W</au><au>Özyilmaz, B</au><au>Watanabe, K</au><au>Taniguchi, T</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Rashba Interaction and Local Magnetic Moments in a Graphene-BN Heterostructure Intercalated with Au</atitle><jtitle>Physical review letters</jtitle><addtitle>Phys Rev Lett</addtitle><date>2016-08-12</date><risdate>2016</risdate><volume>117</volume><issue>7</issue><spage>076603</spage><epage>076603</epage><pages>076603-076603</pages><artnum>076603</artnum><issn>0031-9007</issn><eissn>1079-7114</eissn><abstract>We intercalate a van der Waals heterostructure of graphene and hexagonal boron nitride with Au, by encapsulation, and show that the Au at the interface is two dimensional. Charge transfer upon current annealing indicates the redistribution of the Au and induces splitting of the graphene band structure. The effect of an in-plane magnetic field confirms that the splitting is due to spin splitting and that the spin polarization is in the plane, characteristic of a Rashba interaction with a magnitude of approximately 25 meV. Consistent with the presence of an intrinsic interfacial electric field we show that the splitting can be enhanced by an applied displacement field in dual gated samples. A giant negative magnetoresistance, up to 75%, and a field induced anomalous Hall effect at magnetic fields <1 T are observed. These demonstrate that the hybridized Au has a magnetic moment and suggests the proximity to the formation of a collective magnetic phase. These effects persist close to room temperature.</abstract><cop>United States</cop><pmid>27563982</pmid><doi>10.1103/PhysRevLett.117.076603</doi><tpages>1</tpages></addata></record> |
fulltext | fulltext |
identifier | ISSN: 0031-9007 |
ispartof | Physical review letters, 2016-08, Vol.117 (7), p.076603-076603, Article 076603 |
issn | 0031-9007 1079-7114 |
language | eng |
recordid | cdi_proquest_miscellaneous_1835656748 |
source | American Physical Society:Jisc Collections:APS Read and Publish 2023-2025 (reading list) |
subjects | Boron nitride Charge transfer Electric fields Graphene Heterostructures Magnetic fields Magnetic moment Splitting |
title | Rashba Interaction and Local Magnetic Moments in a Graphene-BN Heterostructure Intercalated with Au |
url | http://sfxeu10.hosted.exlibrisgroup.com/loughborough?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-01-19T18%3A18%3A39IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_cross&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Rashba%20Interaction%20and%20Local%20Magnetic%20Moments%20in%20a%20Graphene-BN%20Heterostructure%20Intercalated%20with%20Au&rft.jtitle=Physical%20review%20letters&rft.au=O'Farrell,%20E%20C%20T&rft.date=2016-08-12&rft.volume=117&rft.issue=7&rft.spage=076603&rft.epage=076603&rft.pages=076603-076603&rft.artnum=076603&rft.issn=0031-9007&rft.eissn=1079-7114&rft_id=info:doi/10.1103/PhysRevLett.117.076603&rft_dat=%3Cproquest_cross%3E1835656748%3C/proquest_cross%3E%3Cgrp_id%3Ecdi_FETCH-LOGICAL-c344t-6bcfe98c1aa8929e405762251e7035e848ae13fb34bdb09278d8049944e8b8513%3C/grp_id%3E%3Coa%3E%3C/oa%3E%3Curl%3E%3C/url%3E&rft_id=info:oai/&rft_pqid=1814658188&rft_id=info:pmid/27563982&rfr_iscdi=true |