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A highly permeable graphene oxide membrane with fast and selective transport nanochannels for efficient carbon capture

Ultrathin graphene oxide membranes using borate as both crosslinker of GO nanosheets and facilitated transport carrier of CO 2 are designed and fabricated. The membranes exhibited high CO 2 permeance up to 650 GPU and a CO 2 /CH 4 selectivity of 75, due to the rational manipulation of the interlayer...

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Published in:Energy & environmental science 2016-10, Vol.9 (1), p.317-3112
Main Authors: Wang, Shaofei, Wu, Yingzhen, Zhang, Ning, He, Guangwei, Xin, Qingping, Wu, Xingyu, Wu, Hong, Cao, Xingzhong, Guiver, Michael D, Jiang, Zhongyi
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creator Wang, Shaofei
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description Ultrathin graphene oxide membranes using borate as both crosslinker of GO nanosheets and facilitated transport carrier of CO 2 are designed and fabricated. The membranes exhibited high CO 2 permeance up to 650 GPU and a CO 2 /CH 4 selectivity of 75, due to the rational manipulation of the interlayer nanochannel size, sufficient facilitated transport carriers and high water content. Tailored physicochemical microenvironments in stacked graphene oxide nanochannels give membranes with fast and highly selective CO 2 transport.
doi_str_mv 10.1039/c6ee01984f
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source Royal Society of Chemistry:Jisc Collections:Royal Society of Chemistry Read and Publish 2022-2024 (reading list)
subjects Carbon dioxide
Carriers
Graphene
Membranes
Moisture content
Nanostructure
Oxides
Transport
title A highly permeable graphene oxide membrane with fast and selective transport nanochannels for efficient carbon capture
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