Controlling the Surface Organization of Conjugated Donor-Acceptor Polymers by their Aggregation in Solution

The aggregation of conjugated polymers is found to have a significant influence on the surface organization of deposited films. Difluorobenzothiadiazole‐based polymers show a strong pre‐aggregation in solution, but the addition of 1,2,4‐trichlorobenzene efficiently reduces such aggregates, leading t...

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Published in:Advanced materials (Weinheim) 2016-11, Vol.28 (42), p.9430-9438
Main Authors: Li, Mengmeng, An, Cunbin, Marszalek, Tomasz, Baumgarten, Martin, Yan, He, Müllen, Klaus, Pisula, Wojciech
Format: Article
Language:English
Subjects:
Addition polymerization
Agglomeration
Aggregates
Control surfaces
organic field-effect transistors
Organizations
Orientation
polymer aggregation
Polymers
self-assembly
solution processing
surface organization
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cited_by cdi_FETCH-LOGICAL-c4160-cf92e3a9799fb7c9fb932e7b12d3c07fb418d0ff124e39fef351fcb142eeb8803
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container_end_page 9438
container_issue 42
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container_title Advanced materials (Weinheim)
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creator Li, Mengmeng
An, Cunbin
Marszalek, Tomasz
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Müllen, Klaus
Pisula, Wojciech
description The aggregation of conjugated polymers is found to have a significant influence on the surface organization of deposited films. Difluorobenzothiadiazole‐based polymers show a strong pre‐aggregation in solution, but the addition of 1,2,4‐trichlorobenzene efficiently reduces such aggregates, leading to the transition of the surface organization from edge‐ to face‐on orientation in deposited films.
doi_str_mv 10.1002/adma.201602660
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source Wiley-Blackwell Read & Publish Collection
subjects Addition polymerization
Agglomeration
Aggregates
Control surfaces
organic field-effect transistors
Organizations
Orientation
polymer aggregation
Polymers
self-assembly
solution processing
surface organization
title Controlling the Surface Organization of Conjugated Donor-Acceptor Polymers by their Aggregation in Solution
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