A New Class of Lasing Materials: Intrinsic Stimulated Emission from Nonlinear Optically Active Metal–Organic Frameworks

Blue‐color stimulated emission with low threshold power is observed from In‐ and Zn‐MOFs, which feature a highly fluorescent chromophore densely packed and rigidly linked to the metal‐ion centers in the solid state. The density‐of‐states and transition dipole moments are calculated and the stimulate...

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Bibliographic Details
Published in:Advanced materials (Weinheim) 2017-05, Vol.29 (17), p.n/a
Main Authors: Medishetty, Raghavender, Nalla, Venkatram, Nemec, Lydia, Henke, Sebastian, Mayer, David, Sun, Handong, Reuter, Karsten, Fischer, Roland A.
Format: Article
Language:English
Subjects:
blue emission
Color
Density of states
Dipole moments
Fluorescence
hybrid materials
Lasing
Materials science
Metal-organic frameworks
nonlinear optics
Optical activity
Solid state
Stimulated emission
two‐photon excited fluorescence
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Summary:Blue‐color stimulated emission with low threshold power is observed from In‐ and Zn‐MOFs, which feature a highly fluorescent chromophore densely packed and rigidly linked to the metal‐ion centers in the solid state. The density‐of‐states and transition dipole moments are calculated and the stimulated emission phenomenon is correlated with these properties.
ISSN:0935-9648
1521-4095
DOI:10.1002/adma.201605637