Colloidal diffusion over a quasicrystalline-patterned surface

We report a systematic study of colloidal diffusion over a substrate with quasicrystalline-patterned holes. Silica spheres of diameter comparable to the hole diameter diffuse over the patterned substrate and experience a gravitational potential U(x, y). Using optical microscopy, we track the particl...

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Bibliographic Details
Published in:The Journal of chemical physics 2017-06, Vol.146 (21), p.214903-214903
Main Authors: Su, Yun, Lai, Pik-Yin, Ackerson, Bruce J., Cao, Xin, Han, Yilong, Tong, Penger
Format: Article
Language:English
Subjects:
Diffusion
Diffusion coefficient
Dwell time
Flat surfaces
Optical microscopy
Particle trajectories
Physics
Quasicrystals
Silicon dioxide
Substrates
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Summary:We report a systematic study of colloidal diffusion over a substrate with quasicrystalline-patterned holes. Silica spheres of diameter comparable to the hole diameter diffuse over the patterned substrate and experience a gravitational potential U(x, y). Using optical microscopy, we track the particle trajectories and find two distinct states: a trapped state when the particles are inside the holes and a free-diffusion state when they are on the flat surface outside the holes. The potential U(x, y) and dynamic properties of the diffusing particle, such as its mean dwell time, mean square displacement, and long-time diffusion coefficient D L , are measured simultaneously. The measured D L is in good agreement with the prediction of two theoretical models proposed for diffusion over a quasicrystal lattice. The experiment demonstrates the applications of this newly constructed potential landscape.
ISSN:0021-9606
1089-7690
DOI:10.1063/1.4984938