Novel Perovskite Solar Cell Architecture Featuring Efficient Light Capture and Ultrafast Carrier Extraction

A new perovskite solar cell (PSC) structure with a functionalized interface between perovskite and a hole transport material has been proposed in this report. The short circuit current density of PSC was notably enhanced with the novel architecture (with an increase of 8.7%), and a power conversion...

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Published in:ACS applied materials & interfaces 2017-07, Vol.9 (28), p.23624-23634
Main Authors: Yu, Yu, Lei, Lei, Yang, Songwang, Xie, Junjie, Shao, Jun, Cao, Qipeng, Zhang, Sheng, Ni, Xiaojie, Ye, Bangjiao, Liu, Yan
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cited_by cdi_FETCH-LOGICAL-a330t-6d6c333dc4891518806b2bcc6d0c0fb270f334f19da13ae73c889f9d75a1c9463
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container_end_page 23634
container_issue 28
container_start_page 23624
container_title ACS applied materials & interfaces
container_volume 9
creator Yu, Yu
Lei, Lei
Yang, Songwang
Xie, Junjie
Shao, Jun
Cao, Qipeng
Zhang, Sheng
Ni, Xiaojie
Ye, Bangjiao
Liu, Yan
description A new perovskite solar cell (PSC) structure with a functionalized interface between perovskite and a hole transport material has been proposed in this report. The short circuit current density of PSC was notably enhanced with the novel architecture (with an increase of 8.7%), and a power conversion efficiency (PCE) of 16.93% was achieved. With the increased perovskite/hole conductor interface, hysteresis suppression was observed. The advantages of this structure in light-harvesting efficiency, trap density, and carrier separation rate were proved by various characterization and analysis studies. It is noteworthy that a PCE of 14.67% was achieved with poly­(3-hexyl-thiophene), which to our knowledge is the highest performing PSC based on this material.
doi_str_mv 10.1021/acsami.7b03666
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title Novel Perovskite Solar Cell Architecture Featuring Efficient Light Capture and Ultrafast Carrier Extraction
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