Building premium secondary reaction field with a miniaturized capsule catalyst to realize efficient synthesis of a liquid fuel directly from syngas

Herein, we report a new miniaturized capsule catalyst, Co/SiO 2 -M-Z 6ET , which is different from routine capsule catalysts, has a smaller core size and has stronger Brønsted acidity. The premium secondary reaction field and the significant capsule size effect on Co/SiO 2 -M-Z 6ET were demonstrated...

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Bibliographic Details
Published in:Catalysis science & technology 2017, Vol.7 (10), p.1996-2000
Main Authors: Yamane, Noriyuki, Wang, Yang, Li, Jie, He, Yingluo, Zhang, Peipei, Nguyen, Letrunghieu, Tan, Li, Ai, Peipei, Peng, Xiaobo, Wang, Ye, Yang, Guohui, Tsubaki, Noritatsu
Format: Article
Language:English
Subjects:
Buildings
Catalysis
Catalysts
Gasoline
Silicon dioxide
Size effects
Synthesis
Synthetic fuels
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Summary:Herein, we report a new miniaturized capsule catalyst, Co/SiO 2 -M-Z 6ET , which is different from routine capsule catalysts, has a smaller core size and has stronger Brønsted acidity. The premium secondary reaction field and the significant capsule size effect on Co/SiO 2 -M-Z 6ET were demonstrated using a model compound of n -hexadecane ( n -C 16 ). Furthermore, a striking gasoline selectivity of 72% was facilely obtained from FT synthesis.
ISSN:2044-4753
2044-4761
DOI:10.1039/C7CY00224F