Development of a framework catalyst for photocatalytic hydrogen evolution

The controlled self-assembly of a catalyst module composed of a Rh( ii ) paddle-wheel dimer bearing 1,8-naphthalimide-based moieties afforded a novel heterogeneous framework catalyst (FC-1). The framework catalyst exhibited long-lived activity for photocatalytic hydrogen production from water and wa...

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Bibliographic Details
Published in:Chemical communications (Cambridge, England) England), 2018, Vol.54 (1), p.1174-1177
Main Authors: Chinapang, Pondchanok, Okamura, Masaya, Itoh, Takahiro, Kondo, Mio, Masaoka, Shigeyuki
Format: Article
Language:English
Subjects:
Catalysis
Catalysts
Catalytic activity
Hydrogen evolution
Hydrogen production
Photocatalysis
Self-assembly
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Summary:The controlled self-assembly of a catalyst module composed of a Rh( ii ) paddle-wheel dimer bearing 1,8-naphthalimide-based moieties afforded a novel heterogeneous framework catalyst (FC-1). The framework catalyst exhibited long-lived activity for photocatalytic hydrogen production from water and was easily reused without considerable loss of catalytic activity. The self-assembly of a catalyst module afforded a novel framework catalyst with long-lived activity and reusability for photocatalytic hydrogen production.
ISSN:1359-7345
1364-548X
DOI:10.1039/c7cc08013a