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Nitrated and oxygenated derivatives of polycyclic aromatic hydrocarbons in the ambient air of two French alpine valleys Part 2: Particle size distribution
The size distribution of polycyclic aromatic hydrocarbons (PAHs) and PAH derivatives was determined during the intensive sampling campaigns of the POVA (Pollution des Vallées Alpines) research programme, in two French alpine valleys, in winter and summer. The size distributions of PAHs, oxygenated P...
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| Published in: | Atmospheric environment 2008, Vol.42 (1), p.55-64 |
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| Main Authors: | , , , , |
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| Language: | English |
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| container_end_page | 64 |
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| container_title | Atmospheric environment |
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| creator | Albinet, A. Leoz-Garziandia, E. Budzinski, H. Villenave, E. Jaffrezo, J.-L. |
| description | The size distribution of polycyclic aromatic hydrocarbons (PAHs) and PAH derivatives was determined during the intensive sampling campaigns of the POVA (Pollution des Vallées Alpines) research programme, in two French alpine valleys, in winter and summer. The size distributions of PAHs, oxygenated PAHs (OPAHs) and nitrated PAHs (NPAHs) present large variations with year time and site type (traffic; suburban and rural). In general, these compounds were mainly associated (60–90%) with fine particles (
D
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| doi_str_mv | 10.1016/j.atmosenv.2007.10.008 |
| format | article |
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D
p<1.3
μm) in agreement with their release from sources (primary and/or secondary). The pollutant distributions with particle size were unimodal and centred at 0.85
μm both in the Chamonix and Maurienne valleys. The summer size distribution of NPAHs was centred at
D
p=2.75
μm. PAH, OPAH and NPAH super micrometre fractions were significantly larger in summer for most sites suggesting the existence of a second mode in that particle size range. A possible reason to explain this phenomenon is that aerosol was locally polluted and characterised by fine particles in winter whereas in summer, aerosol was more mixed and older with possibilities of adsorption of gaseous organic compounds at the surface of the pre-exiting particles. In summer, NPAHs were associated to a greater degree with the super micrometre fraction of the aerosol than the other categories of compounds.</description><identifier>ISSN: 1352-2310</identifier><identifier>ISSN: 0004-6981</identifier><identifier>EISSN: 1873-2844</identifier><identifier>DOI: 10.1016/j.atmosenv.2007.10.008</identifier><language>eng</language><publisher>Oxford: Elsevier Ltd</publisher><subject>Air. Soil. Water. Waste. Feeding ; Alpine valleys ; Applied sciences ; Atmospheric pollution ; Biological and medical sciences ; Earth Sciences ; Environment. Living conditions ; Exact sciences and technology ; Glaciology ; Medical sciences ; Nitrated polycyclic aromatic hydrocarbons ; Oxygenated polycyclic aromatic hydrocarbons ; Pollutants physicochemistry study: properties, effects, reactions, transport and distribution ; Pollution ; Polycyclic aromatic hydrocarbons ; POVA (Pollution des Vallées Alpines) ; Public health. Hygiene ; Public health. Hygiene-occupational medicine ; Sciences of the Universe ; Size distribution</subject><ispartof>Atmospheric environment, 2008, Vol.42 (1), p.55-64</ispartof><rights>2007 Elsevier Ltd</rights><rights>2008 INIST-CNRS</rights><rights>Distributed under a Creative Commons Attribution 4.0 International License</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c549t-97ea38109f8bf9e9d9b057ccb0aa0c80035dc7467ec4ffa5410323dec93091273</citedby><orcidid>0000-0002-7727-8647 ; 0000-0002-6921-5160 ; 0000-0001-5282-9011 ; 0000-0003-1028-9154</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>230,314,780,784,885,4024,27923,27924,27925</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=19962198$$DView record in Pascal Francis$$Hfree_for_read</backlink><backlink>$$Uhttps://insu.hal.science/insu-00375853$$DView record in HAL$$Hfree_for_read</backlink></links><search><creatorcontrib>Albinet, A.</creatorcontrib><creatorcontrib>Leoz-Garziandia, E.</creatorcontrib><creatorcontrib>Budzinski, H.</creatorcontrib><creatorcontrib>Villenave, E.</creatorcontrib><creatorcontrib>Jaffrezo, J.-L.</creatorcontrib><title>Nitrated and oxygenated derivatives of polycyclic aromatic hydrocarbons in the ambient air of two French alpine valleys Part 2: Particle size distribution</title><title>Atmospheric environment</title><description>The size distribution of polycyclic aromatic hydrocarbons (PAHs) and PAH derivatives was determined during the intensive sampling campaigns of the POVA (Pollution des Vallées Alpines) research programme, in two French alpine valleys, in winter and summer. The size distributions of PAHs, oxygenated PAHs (OPAHs) and nitrated PAHs (NPAHs) present large variations with year time and site type (traffic; suburban and rural). In general, these compounds were mainly associated (60–90%) with fine particles (
D
p<1.3
μm) in agreement with their release from sources (primary and/or secondary). The pollutant distributions with particle size were unimodal and centred at 0.85
μm both in the Chamonix and Maurienne valleys. The summer size distribution of NPAHs was centred at
D
p=2.75
μm. PAH, OPAH and NPAH super micrometre fractions were significantly larger in summer for most sites suggesting the existence of a second mode in that particle size range. A possible reason to explain this phenomenon is that aerosol was locally polluted and characterised by fine particles in winter whereas in summer, aerosol was more mixed and older with possibilities of adsorption of gaseous organic compounds at the surface of the pre-exiting particles. In summer, NPAHs were associated to a greater degree with the super micrometre fraction of the aerosol than the other categories of compounds.</description><subject>Air. Soil. Water. Waste. Feeding</subject><subject>Alpine valleys</subject><subject>Applied sciences</subject><subject>Atmospheric pollution</subject><subject>Biological and medical sciences</subject><subject>Earth Sciences</subject><subject>Environment. Living conditions</subject><subject>Exact sciences and technology</subject><subject>Glaciology</subject><subject>Medical sciences</subject><subject>Nitrated polycyclic aromatic hydrocarbons</subject><subject>Oxygenated polycyclic aromatic hydrocarbons</subject><subject>Pollutants physicochemistry study: properties, effects, reactions, transport and distribution</subject><subject>Pollution</subject><subject>Polycyclic aromatic hydrocarbons</subject><subject>POVA (Pollution des Vallées Alpines)</subject><subject>Public health. Hygiene</subject><subject>Public health. Hygiene-occupational medicine</subject><subject>Sciences of the Universe</subject><subject>Size distribution</subject><issn>1352-2310</issn><issn>0004-6981</issn><issn>1873-2844</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2008</creationdate><recordtype>article</recordtype><recordid>eNqNksFu1DAQhiMEEqXwCsgXOCDtMk6cOOZEVVGKtAIOcLYmzoT1ymsvtjcQHoWnJekWOLanscffzK_x_EXxnMOaA29e79aY9yGRH9clgJyTa4D2QXHGW1mtylaIh_O5qstVWXF4XDxJaQcAlVTyrPj90eaImXqGvmfh5_SN_M21p2hHzHakxMLADsFNZjLOGoYx7OcHw7ZTH4PB2AWfmPUsb4nhvrPkM0Mbl7L8I7CrSN5sGbqD9cRGdI6mxD5jzKx8cxOtccSS_UWstylH2x2zDf5p8WhAl-jZbTwvvl69-3J5vdp8ev_h8mKzMrVQeaUkYdVyUEPbDYpUrzqopTEdIIJp50Hr3kjRSDJiGLAWHKqy6smoChQvZXVevDr13aLTh2j3GCcd0Orri422Ph318ll1W1cjn-GXJ_gQw_cjpaz3NhlyDj2FY9IltCVvWnkPUEohBdwJctE2wEVzH7AWDSzSzQk0MaQUafg3FQe9WEbv9F_L6MUyS362zFz44lYBk0E3RPTGpv_VSjUlVwv39sTRvJbRUtTJzFs31NtIJus-2Luk_gAL_tza</recordid><startdate>2008</startdate><enddate>2008</enddate><creator>Albinet, A.</creator><creator>Leoz-Garziandia, E.</creator><creator>Budzinski, H.</creator><creator>Villenave, E.</creator><creator>Jaffrezo, J.-L.</creator><general>Elsevier Ltd</general><general>Elsevier Science</general><general>Elsevier</general><scope>IQODW</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7ST</scope><scope>C1K</scope><scope>SOI</scope><scope>7TG</scope><scope>7TV</scope><scope>KL.</scope><scope>1XC</scope><scope>VOOES</scope><orcidid>https://orcid.org/0000-0002-7727-8647</orcidid><orcidid>https://orcid.org/0000-0002-6921-5160</orcidid><orcidid>https://orcid.org/0000-0001-5282-9011</orcidid><orcidid>https://orcid.org/0000-0003-1028-9154</orcidid></search><sort><creationdate>2008</creationdate><title>Nitrated and oxygenated derivatives of polycyclic aromatic hydrocarbons in the ambient air of two French alpine valleys Part 2: Particle size distribution</title><author>Albinet, A. ; Leoz-Garziandia, E. ; Budzinski, H. ; Villenave, E. ; Jaffrezo, J.-L.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c549t-97ea38109f8bf9e9d9b057ccb0aa0c80035dc7467ec4ffa5410323dec93091273</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2008</creationdate><topic>Air. Soil. Water. Waste. Feeding</topic><topic>Alpine valleys</topic><topic>Applied sciences</topic><topic>Atmospheric pollution</topic><topic>Biological and medical sciences</topic><topic>Earth Sciences</topic><topic>Environment. Living conditions</topic><topic>Exact sciences and technology</topic><topic>Glaciology</topic><topic>Medical sciences</topic><topic>Nitrated polycyclic aromatic hydrocarbons</topic><topic>Oxygenated polycyclic aromatic hydrocarbons</topic><topic>Pollutants physicochemistry study: properties, effects, reactions, transport and distribution</topic><topic>Pollution</topic><topic>Polycyclic aromatic hydrocarbons</topic><topic>POVA (Pollution des Vallées Alpines)</topic><topic>Public health. Hygiene</topic><topic>Public health. Hygiene-occupational medicine</topic><topic>Sciences of the Universe</topic><topic>Size distribution</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Albinet, A.</creatorcontrib><creatorcontrib>Leoz-Garziandia, E.</creatorcontrib><creatorcontrib>Budzinski, H.</creatorcontrib><creatorcontrib>Villenave, E.</creatorcontrib><creatorcontrib>Jaffrezo, J.-L.</creatorcontrib><collection>Pascal-Francis</collection><collection>CrossRef</collection><collection>Environment Abstracts</collection><collection>Environmental Sciences and Pollution Management</collection><collection>Environment Abstracts</collection><collection>Meteorological & Geoastrophysical Abstracts</collection><collection>Pollution Abstracts</collection><collection>Meteorological & Geoastrophysical Abstracts - Academic</collection><collection>Hyper Article en Ligne (HAL)</collection><collection>Hyper Article en Ligne (HAL) (Open Access)</collection><jtitle>Atmospheric environment</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Albinet, A.</au><au>Leoz-Garziandia, E.</au><au>Budzinski, H.</au><au>Villenave, E.</au><au>Jaffrezo, J.-L.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Nitrated and oxygenated derivatives of polycyclic aromatic hydrocarbons in the ambient air of two French alpine valleys Part 2: Particle size distribution</atitle><jtitle>Atmospheric environment</jtitle><date>2008</date><risdate>2008</risdate><volume>42</volume><issue>1</issue><spage>55</spage><epage>64</epage><pages>55-64</pages><issn>1352-2310</issn><issn>0004-6981</issn><eissn>1873-2844</eissn><abstract>The size distribution of polycyclic aromatic hydrocarbons (PAHs) and PAH derivatives was determined during the intensive sampling campaigns of the POVA (Pollution des Vallées Alpines) research programme, in two French alpine valleys, in winter and summer. The size distributions of PAHs, oxygenated PAHs (OPAHs) and nitrated PAHs (NPAHs) present large variations with year time and site type (traffic; suburban and rural). In general, these compounds were mainly associated (60–90%) with fine particles (
D
p<1.3
μm) in agreement with their release from sources (primary and/or secondary). The pollutant distributions with particle size were unimodal and centred at 0.85
μm both in the Chamonix and Maurienne valleys. The summer size distribution of NPAHs was centred at
D
p=2.75
μm. PAH, OPAH and NPAH super micrometre fractions were significantly larger in summer for most sites suggesting the existence of a second mode in that particle size range. A possible reason to explain this phenomenon is that aerosol was locally polluted and characterised by fine particles in winter whereas in summer, aerosol was more mixed and older with possibilities of adsorption of gaseous organic compounds at the surface of the pre-exiting particles. In summer, NPAHs were associated to a greater degree with the super micrometre fraction of the aerosol than the other categories of compounds.</abstract><cop>Oxford</cop><pub>Elsevier Ltd</pub><doi>10.1016/j.atmosenv.2007.10.008</doi><tpages>10</tpages><orcidid>https://orcid.org/0000-0002-7727-8647</orcidid><orcidid>https://orcid.org/0000-0002-6921-5160</orcidid><orcidid>https://orcid.org/0000-0001-5282-9011</orcidid><orcidid>https://orcid.org/0000-0003-1028-9154</orcidid><oa>free_for_read</oa></addata></record> |
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| ispartof | Atmospheric environment, 2008, Vol.42 (1), p.55-64 |
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| language | eng |
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| source | ScienceDirect Freedom Collection 2022-2024 |
| subjects | Air. Soil. Water. Waste. Feeding Alpine valleys Applied sciences Atmospheric pollution Biological and medical sciences Earth Sciences Environment. Living conditions Exact sciences and technology Glaciology Medical sciences Nitrated polycyclic aromatic hydrocarbons Oxygenated polycyclic aromatic hydrocarbons Pollutants physicochemistry study: properties, effects, reactions, transport and distribution Pollution Polycyclic aromatic hydrocarbons POVA (Pollution des Vallées Alpines) Public health. Hygiene Public health. Hygiene-occupational medicine Sciences of the Universe Size distribution |
| title | Nitrated and oxygenated derivatives of polycyclic aromatic hydrocarbons in the ambient air of two French alpine valleys Part 2: Particle size distribution |
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